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Molecular dynamics simulations were employed to study the wetting behavior of nanoscale aqueous hydrophilic and hydrophobic Imidazolium based ionic liquid (IL) droplets on a solid graphite substrate subjected to the perpendicular electric…

软凝聚态物质 · 物理学 2020-12-09 Sanchari Bhattacharjee , Sandip Khan

In Molecular Dynamics (MD) simulations, interactions between water molecules and graphitic surfaces are often modeled as a simple Lennard-Jones potential between oxygen and carbon atoms. A possible method for tuning this parameter consists…

介观与纳米尺度物理 · 物理学 2015-06-03 Giulio Scocchi , Danilo Sergi , Claudio D'Angelo , Alberto Ortona

This work describes the behaviour of water molecules in 1-butyl-3-methylimidazolium tetrafluoroborate ionic liquid under nanoconfinement between graphene sheets. By means of molecular dynamics simulations, an adsorption of water molecules…

Ionic liquids (IL) are promising electrolytes for electrochemical applications due to their remarkable stability and high charge density. Molecular dynamics simulations are essential for better understanding the complex phenomena occurring…

Using dielectric spectroscopy and differential scanning calorimetry, we have performed a detailed investigation of the influence of water uptake on the translational and reorientational glassy dynamics in the typical ionic liquid…

材料科学 · 物理学 2017-01-23 P. Sippel , V. Dietrich , D. Reuter , M. Aumüller , P. Lunkenheimer , A. Loidl , S. Krohns

The interactions of a hydrophilic surface with water can significantly influence the characteristics of the liquid water interface. In this manuscript, we explore this influence by studying the molecular structure of liquid water at a…

软凝聚态物质 · 物理学 2022-09-19 Sucheol Shin , Adam P. Willard

In this work we present the dielectric behavior of water with a novel flexible model that improved all three sites water models Different concentrations of the ionic liquid 1- butyl-3-methylimidazolium [bmim]…

The fundamental understanding of intermolecular interactions of ionic liquids with water represents a vital extent in predicting ionic liquid properties. Intermolecular or noncovalent interactions were studied for 1,3-dimethyl imidazolium…

化学物理 · 物理学 2022-06-14 Oleg N. Starovoytov

The relation between wetting properties and geometric parameters of fractal surfaces are widely discussed on the literature and, however, there are still divergences on this topic. Here we propose a simple theoretical model to describe the…

软凝聚态物质 · 物理学 2024-06-14 Iara Patrícia da Silva Ramos , Cristina Gavazzoni , Davi Lazzari , Carolina Brito

Droplet impact is a fascinating phenomenon that occurs when a liquid droplet collides with a surface. It is not only a fundamental area of scientific inquiry but also has practical implications across many industries and natural systems.…

流体动力学 · 物理学 2026-03-27 Shubham Ganar , Arindam Das

Understanding how water wets graphene is critical for predicting and controlling its behaviour in nanofluidic, sensing, and energy applications. A key measure of wetting is the contact angle made by a liquid droplet against the surface, yet…

介观与纳米尺度物理 · 物理学 2026-05-04 Darren Wayne Lim , Xavier R. Advincula , William C. Witt , Angelos Michaelides , Fabian L. Thiemann , Christoph Schran

The interaction energy between a water molecule and graphitic structured clusters terminated by hydrogen atoms is analyzed by ab initio methods and decomposed into electrostatic, induction, Pauli repulsion, and correlation energy…

计算物理 · 物理学 2008-01-21 D. J. Wallace Geldart , I. Wayan Sudiarta , Glen Lesins , Petr Chylek

Hydrophobic solid-water interfaces underpin processes in nanofluidics, electrochemistry, and energy technologies. Microscopic insights into these systems are often inferred from our understanding of the air-water interface, which is assumed…

Ionic liquids (ILs) feature a tailorable and wide range of structural, chemical and electronic properties that make this class of materials suitable to a broad variety of forefront applications in next-generation electronics. Yet, their…

材料科学 · 物理学 2022-11-28 Irene Amiehe Essomba , Mauro Boero , Kerstin Falk , Guido Ori

We demonstrate droplet manipulation using electric signals to induce the liquid to wet or dewet on a hydrophilic conductive substrate in the air without adding layers. In this phenomenon, the contact angle changes more than 15{\deg} or…

流体动力学 · 物理学 2023-03-07 Lele Zhou , Rong Zhang , Hung-Ta Wang , Yifan Liu

The wetting dynamics of liquid particles, from coated droplets to soft capsules, holds significant technological interest. Motivated by the need to simulate liquid metal droplet with an oxidize surface layer, in this work we introduce a…

流体动力学 · 物理学 2024-02-14 Francesca Pelusi , Fabio Guglietta , Marcello Sega , Othmane Aouane , Jens Harting

The interaction of interfacial water with graphitic carbon at the atomic scale is studied as a function of the hydrophobicity of epitaxial graphene. High resolution X-ray reflectivity shows that the graphene-water contact angle is…

We study the wetting properties of water on silica surfaces using molecular dynamics (MD) simulations. To describe the intermolecular interaction between water and silica atoms, two types of interaction potential models are used: the…

软凝聚态物质 · 物理学 2016-10-12 E. Pafong , J. Geske , B. Drossel

In this work, we studied the wetting behavior of impinged and stagnant supercooled water nanodroplet at the atomistic scale using molecular dynamics simulations. We show that water droplet represents a retraction behavior from surface…

化学物理 · 物理学 2019-08-05 Amir Afshar , Dong Meng

We analyze and compare the structural, dynamical, and electronic properties of liquid water next to prototypical metals including Pt, graphite, and graphene. Our results are built on Born-Oppenheimer molecular dynamics (BOMD) generated…

材料科学 · 物理学 2017-08-09 Kevin Ryczko , Isaac Tamblyn
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