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This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly…

强关联电子 · 物理学 2022-04-06 R. E. F. Silva , Igor V. Blinov , Alexey N. Rubtsov , O. Smirnova , M. Ivanov

A major challenge in condensed matter physics is active control of quantum phases. Dynamic control with pulsed electromagnetic fields can overcome energetic barriers enabling access to transient or metastable states that are not thermally…

Light-matter interactions in crystals are powerful tools that seamlessly allow both functionalities of sizeable bandgap modulation and non-invasive spectroscopy. While we often assume that the border between the two regimes of modulation…

We present a microscopic theory for ultrafast control of solids with high-intensity terahertz frequency optical pulses. When resonant with selected infrared-active vibrations, these pulses transiently modify the crystal structure and lead…

强关联电子 · 物理学 2014-07-15 Alaska Subedi , Andrea Cavalleri , Antoine Georges

Ultrafast time-resolved optical spectroscopy in high-temperature superconductors enables the direct real-time measurement of non-equilibrium quasiparticle recombination dynamics. In addition, it also gives detailed information about the…

超导电性 · 物理学 2007-05-23 D. Mihailovic , J. Demsar

We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase…

强关联电子 · 物理学 2014-01-15 I. Kezsmarki , R. Gaal , C. C. Homes , B. Sipos , H. Berger , S. Bordacs , G. Mihaly , L. Forro

We investigate the thermal-driven charge density wave (CDW) transition of two cubic superconducting intermetallic systems Lu(Pt1-xPdx)2In and (Sr1-xCax)3Ir4Sn13 by means of x-ray diffraction technique. A detailed analysis of the CDW…

强关联电子 · 物理学 2020-05-27 F. B. Carneiro , L. S. I. Veiga , J. R. L. Mardegan , R. Khan , C. Macchiutti , A. Lopez , E. M. Bittar

Using ultrashort laser pulses, it has become possible to probe the dynamics of long-range order in solids on microscopic timescales. In the conventional description of symmetry-broken phases within time-dependent Ginzburg-Landau theory, the…

强关联电子 · 物理学 2023-06-08 Antonio Picano , Francesco Grandi , Martin Eckstein

The transition between different states in manganites can be driven by various external stimuli. Controlling these transitions with light opens the possibility to investigate the microscopic path through which they evolve. We performed…

强关联电子 · 物理学 2014-01-17 L. Piazza , C. Ma , H. X. Yang , A. Mann , Y. Zhu , J. Q. Li , F. Carbone

Ongoing developments in ultrafast X-ray sources offer powerful new means of probing the com- plex non-adiabatically coupled structural and electronic dynamics of photoexcited molecules. These non-Born-Oppenheimer effects are governed by…

化学物理 · 物理学 2018-07-04 Simon P. Neville , Majed Chergui , Albert Stolow , Michael S. Schuurman

We report ultrafast reflectivity measurements of the dynamics of the order parameter of the charge density wave (CDW) in TbTe$_3$ under anisotropic strain. We observe an increase in the frequency of the amplitude mode with increasing…

强关联电子 · 物理学 2024-09-04 Soyeun Kim , Gal Orenstein , Anisha G. Singh , Ian R. Fisher , David A. Reis , Mariano Trigo

Engineering quantum phases using light is a novel route to designing functional materials, where light-induced superconductivity is a successful example. Although this phenomenon has been realized experimentally, especially for the…

超导电性 · 物理学 2021-11-23 Yao Wang , Tao Shi , Cheng-Chien Chen

Advances in attosecond core-level spectroscopies have successfully unlocked the fastest dynamics involving high-energy electrons. Yet, these techniques are not conventionally regarded as an appropriate probe for low-energy quasiparticle…

A number of intriguing phenomena, including exciton condensation, orbital ordering, and emergence of chirality, have been proposed to accompany charge-density-wave (CDW) formation in the layered transition metal dichalcogenide…

强关联电子 · 物理学 2025-02-18 Wei Wang , Patrick Liu , Lijun Wu , Jing Tao , Genda Gu , Alfred Zong , Yimei Zhu

Exciton polaritons based on atomically thin semiconductors are essential building blocks of quantum optoelectronic devices. Their properties are governed by an ultrafast and oscillatory energy transfer between their excitonic and photonic…

Ultrafast lasers ($< 500$ fs) have enabled laser-matter interactions at intensities exceeding $10^{18} \rm{Wcm}^{-2}$ with only millijoules of laser energy. However, as pulse durations become shorter, larger spectral bandwidths are…

Modern laser sources nowadays deliver ultrashort light pulses reaching few cycles in duration, high energies beyond the Joule level and peak powers exceeding several terawatt (TW). When such pulses propagate through optically-transparent…

光学 · 物理学 2007-09-27 L. Berge , S. Skupin , R. Nuter , J. Kasparian , J. -P. Wolf

Laser excitation has emerged as an effective tool for probing microscopic interactions and manipulating phases of matter. Among charge density wave (CDW) materials, 1T-TaS2 has garnered significant attention due to its diverse stacking…

材料科学 · 物理学 2025-02-26 Jin Zhang , Yang Yang , Jia Zhang , Mengxue Guan , Jiyu Xu , Kun Yang , Xinghua Shi , Sheng Meng

To understand complex physics of a system with strong electron electron interactions, it is ideal to control and monitor its properties while tuning an external electric field applied to the system. Indeed, complete electric field control…

The field of metamaterial research revolves around the idea of creating artificial media that interact with light in a way unknown from naturally occurring materials. This is commonly achieved by creating sub-wavelength lattices of…

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