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Excitons and their constituent charge carriers play the central role in electroluminescence mechanisms determining the ultimate performance of organic optoelectronic devices. The involved processes and their dynamics are often studied with…

We present a study of free carrier photo-generation and multi-carrier bound states, such as biexcitons and trions (ionized excitons), in semiconducting single-walled carbon nanotubes. Pump-and-probe measurements performed with fs pulses…

Doping substantially influences the electronic and photophysical properties of semiconducting single-wall carbon nanotubes (s-SWNTs). Although prior studies have noted that surplus charge carriers modify optical spectra and accelerate…

We propose a double channel mechanism for the formation of charged excitons (trions); they are formed through bi- and tri-molecular processes. This directly implies that both negatively and positively charged excitons coexist in a quantum…

材料科学 · 物理学 2009-09-29 M. T. Portella-Oberli , J. Berney , L. Kappei , F. Morier-Genoud , J. Szczytko , B. Deveaud

Optical excitation and control of excitonic wavepackets in organic molecules is the basis to energy conversion processes. To gain insights into such processes, it is essential to establish the relationship between the coherence timescales…

We have studied the coherent dynamics of injected electrons when they are either free or bounded both in excitons and in trions (charged excitons). We have considered a remotely doped asymmetric double quantum well where an excess of free…

材料科学 · 物理学 2009-11-10 P. Aceituno , A. Hernandez-Cabrera

Charged excitons, or trions, offering unique spin and charge degrees of freedom, have primarily been investigated in doped systems where charges are long considered indispensable. Here, we present an alternative route to ultra-efficient…

介观与纳米尺度物理 · 物理学 2026-02-17 N. Fang , U. Erkilic , Y. R. Chang , S. Fujii , D. Yamashita , C. F. Fong , S. Morito , K. Kanahashi , T. Taniguchi , K. Watanabe , K. Ueno , K. Nagashio , Y. K. Kato

Trions are excitonic species with a positive or negative charge, and thus, unlike neutral excitons, the flow of trions can generate a net detectable charge current. Trions under favourable doping conditions can be created in a coherent…

应用物理 · 物理学 2020-03-24 Sarthak Das , Sangeeth Kallatt , Nithin Abraham , Kausik Majumdar

Trions are charged excitons that form upon optical or electrical excitation of low-dimensional semiconductors in the presence of charge carriers (holes or electrons). Trion emission from semiconducting single-walled carbon nanotubes…

材料科学 · 物理学 2023-02-17 Sonja Wieland , Abdurrahman Ali El Yumin , Jan M. Gotthardt , Jana Zaumseil

We demonstrate exciton and charged exciton (trion) electroluminescence from frozen p-n junctions in networks of polymer-sorted, semiconducting (6,5) single-walled carbon nanotubes. Electrolyte-gating with an ionic liquid was employed to…

We report charged exciton (trion) formation dynamics in doped monolayer transition metal dichalcogenides (TMDs), specifically molybdenum diselenide (MoSe2), using resonant two-color pump-probe spectroscopy. When resonantly pumping the…

Monolayer phosphorene provides a unique two-dimensional (2D) platform to investigate the fundamental dynamics of excitons and trions (charged excitons) in reduced dimensions. However, owing to its high instability, unambiguous…

材料科学 · 物理学 2015-04-30 Jiong Yang , Renjing Xu , Jiajie Pei , Ye Win Myint , Fan Wang , Zhu Wang , Shuang Zhang , Zongfu Yu , Yuerui Lu

We studied the excitation density dependence of photoluminescence (PL) spectra of excitons and trions (charged excitons) in hole-doped single-walled carbon nanotubes. We found that the PL intensity of trions exhibited a strong nonlinear…

Multimodal device operations are essential to advancing the integration of 2D semiconductors in electronics, photonics, information and quantum technology. Precise control over carrier dynamics, particularly exciton generation and…

We present evidence of all optical trion generation and emission in undoped single walled carbon nanotubes (SWCNTs). Luminescence spectra, recorded on individual SWCNTs over a large CW excitation intensity range, show trion emission peaks…

介观与纳米尺度物理 · 物理学 2015-05-28 Silvia Santos , Bertrand Yuma , Stéphane Berciaud , Jonah Shaver , Mathieu Gallart , Pierre Gilliot , Laurent Cognet , Brahim Lounis

We report on the exciton and trion density dynamics in a single layer of MoSe$_2$, resonantly excited and probed using three-pulse four-wave mixing (FWM), at temperatures from 300K to 77K . A multi-exponential third-order response function…

介观与纳米尺度物理 · 物理学 2017-07-12 L. Scarpelli , F. Masia , E. M. Alexeev , F. Withers , A. I. Tartakovskii , K. S. Novoselov , W. Langbein

We report the first observation of trions (charged excitons), three-particle bound states consisting of one electron and two holes, in hole-doped carbon nanotubes at room temperature. When p-type dopants are added to carbon nanotube…

介观与纳米尺度物理 · 物理学 2013-08-26 Ryusuke Matsunaga , Kazunari Matsuda , Yoshihiko Kanemitsu

Strong Coulomb interaction in atomically-thin transition metal dichalcogenides makes these systems particularly promising for studies of excitonic physics. Of special interest are the manifestations of the charged excitons, also known as…

介观与纳米尺度物理 · 物理学 2020-08-26 M. M. Glazov

The possibility of electrical manipulation and detection of charged exciton (trion) before its radiative recombination makes it promising for excitonic devices. Using a few-layer graphene/monolayer WS$_{2}$/monolayer graphene vertical…

介观与纳米尺度物理 · 物理学 2019-04-04 Sangeeth Kallatt , Sarthak Das , Suman Chatterjee , Kausik Majumdar

We revisit low-temperature optical spectra of transition-metal dichalcogenide monolayers and point to a possible crystallization of electrons (or holes) at low to moderate charge densities. To calculate the excitonic spectra under such…

介观与纳米尺度物理 · 物理学 2023-08-16 Dinh Van Tuan , Hanan Dery
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