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Magnetic double perovskite compounds provide a fertile playground to explore interesting electronic and magnetic properties. By complementary macroscopic characterizations, neutron powder diffraction measurements and first-principles…

强关联电子 · 物理学 2024-04-03 Cheng Su , Xu-Tao Zeng , Kaitong Sun , Denis Sheptyakov , Ziyu Chen , Xian-Lei Sheng , Haifeng Li , Wentao Jin

Recent experiments on the Co-based $d^7$ honeycomb materials BaCo$_2$(AsO$_4$)$_2$ and BaCo$_2$(PO$_4$)$_2$ have drawn renewed interest to XXZ models with competing interactions beyond the nearest neighbor exchange. While the case of…

强关联电子 · 物理学 2023-01-02 Yoshito Watanabe , Simon Trebst , Ciarán Hickey

In a recent letter [Phys. Rev. Lett. {\bf 82}, 1012 (1999)] it was found that the Tb$^{3+}$ magnetic moments in the Tb$_2$Ti$_2$O$_7$ pyrochlore lattice of corner-sharing tetrahedra remain in a {\it collective paramagnetic} state down to…

无序系统与神经网络 · 物理学 2009-10-31 M. J. P. Gingras , B. C. den Hertog , M. Faucher , J. S. Gardner , L. J. Chang , B. D. Gaulin , N. P. Raju , J. E. Greedan

Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

Li2MnO3 with a S=3/2 two-dimensional Mn honeycomb lattice has a Neel-type antiferromagnetic transition at TN=36 K with a broad maximum in the magnetic susceptibility at TM=48 K. We have investigated site percolation effects by replacing Mn…

强关联电子 · 物理学 2015-06-22 Sanghyun Lee , Junghwan Park , Jiyeon Kim , Kun-Pyo Hong , Youngmi Song , Je-Geun Park

The development of magnetoelectric materials requires chemical design strategies that integrate structural polarity with magnetic lattices capable of supporting competing spin interactions. Here, we demonstrate such an approach in the…

材料科学 · 物理学 2026-03-17 Faith O. Adeyemi , Xudong Huai , Mohamed Kandil , Pradip Karki , Wencan Jin , Thao T. Tran

Anti-site disordering in Sr2FeMoO6 double perovskites (containing Mo atoms at Fe positions, and viceversa) has recently been shown to have a dramatic influence in their magnetic and magnetotransport properties. In the present study, two…

We report a combined muon spin relaxation/rotation, bulk magnetization, neutron scattering, and transport study of the electronic properties of the pyrochlore iridate Nd2Ir2O7. We observe the onset of strongly hysteretic behavior in the…

Neutron diffraction, polarized neutron transmission, and small angle neutron scattering have been used to investigate the crystal structure and nature of the magnetic order in a polycrystalline sample of RuSr2Eu1.2Ce0.8Cu2O10. The sample…

超导电性 · 物理学 2009-11-11 J. W. Lynn , Y. Chen , Q. Huang , S. K. Goh , G. V. M. Williams , J. L. Tallon

Neutron diffraction studies have been carried out in the applied magnetic field H(//[011]) on a single crystal of pyrochlore ferromagnet Nd2Mo2O7, whose Hall resistivity(r_H) has been reported to have quite unusual magnetic field (H)- and…

Recently, layered honeycomb cobaltates have been predicted as a new promising system for realizing the Kitaev quantum spin liquid, a many-body quantum entangled ground state characterized by fractional excitations. However, these…

Examples of materials where an "order by disorder" mechanism is at play to select a particular ground state are scarce. It has recently been proposed, however, that the antiferromagnetic XY pyrochlore Er2Ti2O7, reveals a most convincing…

强关联电子 · 物理学 2015-06-23 S. Petit , J. Robert , S. Guitteny , P. Bonville , C. Decorse , J. Ollivier , H. Mutka , M. J. P. Gingras , I. Mirebeau

Recent theoretical studies have suggested that the low-energy Hamiltonian of honeycomb cobaltate systems could be dominated by anisotropic Kitaev interactions. Motivated by the theory, a honeycomb layered material Na$_{2}$Co$_{2}$TeO$_{6}$…

Ho2Ir3Si5 belongs to the family of three-dimensional (3D) R2Ir3Si5 (R = Lu, Er and Ho) compounds that exhibit a colossal first-order charge density wave (CDW) transition where there is a strong orthorhombic-to-triclinic distortion of the…

R2RhIn8 compounds (space group P4/mmm, R is a rare-earth element) belong to a large group of structurally related tetragonal materials which involves several heavy-fermion superconductors based on Ce. We have succeeded to grow single…

We report on the crystal structure of the quantum magnet (CuCl)LaNb2O7 that was controversially described with respect to its structural organization and magnetic behavior. Using high-resolution synchrotron powder x-ray diffraction,…

材料科学 · 物理学 2015-03-17 Alexander A. Tsirlin , Artem M. Abakumov , Gustaaf Van Tendeloo , Helge Rosner

Extensive experimental investigations of the magnetic structures and excitations in the XY pyrochlores have been carried out over the last decade. Three families of XY pyrochlores have emerged: Yb$_2B_2$O$_7$, Er$_2B_2$O$_7$, and, most…

强关联电子 · 物理学 2020-09-14 Alannah M. Hallas , Jonathan Gaudet , Bruce D. Gaulin

We report on the results of powder and single crystal neutron diffraction to investigate the magnetic order in YbCo$_2$Si$_2$ below the N\'eel temperature $T_{\rm N} = 1.7~$K in detail. Two different magnetically ordered phases can clearly…

强关联电子 · 物理学 2016-08-03 N. Mufti , K. Kaneko , A. Hoser , M. Gutmann , C. Geibel , C. Krellner , O. Stockert

We investigated the crystal structure, magnetic behavior, and optical properties of the layered honeycomb compound Na2Cu2TeO6. X-ray and neutron diffraction confirmed a monoclinic structure, with Cu ions arranged in dimerized chains.…

强关联电子 · 物理学 2025-08-25 Shubham Patil , S. D. Kaushik

Rare earth based cobalt-ruthenium double perovskites A$_2$CoRuO$_6$ (A = La, Pr, Nd and Sm) were synthesized and investigated for their structural and magnetic properties. All the compounds crystallize in the monoclinic $P2_1/n$ structure…

材料科学 · 物理学 2019-07-24 Manjil Das , Prabir Dutta , Saurav Giri , Subham Majumdar