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We investigate the interplay between lattice symmetry, phonons, and magnetism in the quasi-one-dimensional ladder compound BaFe$_2$S$_3$ by combining polarized synchrotron infrared spectroscopy, hybrid-functional density functional theory…

We investigated the magnetic and magnetoelastic properties of MnSc$_2$Se$_4$ single crystals at low temperature under a magnetic field directed along the crystallographic [111] axis. The magnetization data at low temperature show a linear…

强关联电子 · 物理学 2024-10-29 J. Sourd , Y. Skourski , L. Prodan , V. Tsurkan , A. Miyata , J. Wosnitza , S. Zherlitsyn

The vibrational structure of chromium germanium telluride (Cr$_2$Ge$_2$Te$_6$, CGT) is investigated and a strong spin-phonon coupling is revealed. The measured high-resolution Raman scattering (RS) spectra are composed of the 10…

Magnetic nanoparticles of gamma-Fe2O3 coated by organic molecules and suspended in liquid and solid matrices, as well as a non-diluted magnetic fluid have been studied by electron magnetic resonance (EMR) at 77-380 K. Slightly asymmetric…

材料科学 · 物理学 2009-11-11 N. Noginova , F. Chen , T. Weaver , E. P. Giannelis , A. B. Bourlinos , V. A. Atsarkin

We report ac susceptibility and high-frequency electron spin resonance (ESR) measurements on the geometrically frustrated compound Ba$_3$NbFe$_3$Si$_2$O$_{14}$ with the N\'{e}el temperature $T_N=27 K$. An unusually large…

强关联电子 · 物理学 2011-08-10 K. -Y. Choi , Z. -X. Wang , A. Ozarowski , J. van Tol , H. D. Zhou , C. R. Wiebe , N. S. Dalal

When magnons and phonons, the fundamental quasiparticles of the solid, are coupled to one another, they form a new hybrid quasi-particle, leading to novel phenomena and interesting applications. Despite its wide-ranging importance, however,…

We have investigated crystal field and phonon dynamics of the multiferroic orthoferrite DyFeO$_3$ via polarized infrared spectroscopy. Reflectance of single crystals was measured in the far- to mid-infrared spectral range at range of…

强关联电子 · 物理学 2013-02-14 A. D. LaForge , J. Whalen , T. Siegrist , A. P. Ramirez , Z. Schlesinger

Since thermal fluctuations become more important as dimensions shrink, it is expected that low-dimensional magnets are more sensitive to lattice distortions and phonons than bulk systems are. Here we present a fully relativistic…

材料科学 · 物理学 2022-04-06 Banasree Sadhukhan , Anders Bergman , Yaroslav O. Kvashnin , Johan Hellsvik , Anna Delin

Lattice dynamics and magnetic excitations are investigated to elucidate the origin of magneto-dielectric effects in the S=1/2 two-dimensional quantum spin compound K$_2$V$_3$O$_8$. We find evidence for lattice instabilities at 110 K and 60…

强关联电子 · 物理学 2015-06-04 K. -Y. Choi , P. Lemmens , V. P. Gnezdilov , B. C. Sales , M. D. Lumsden

The strong coupling between spin, lattice and electronic degrees of freedom in magnetic materials can produce interesting phenomena, including multiferroic and magnetodielectric (MD) behavior, and exotic coupled excitations, such as…

强关联电子 · 物理学 2019-05-08 A. Sethi , J. E. Slimak , T. Kolodiazhnyi , S. L. Cooper

We report a giant linear magnetoelectric coupling in strained BiMnO3 thin films in which the disorder associated with an islanded morphology gives rise to extrinsic relaxor ferroelectricity that is not present in bulk centrosymmetric…

材料科学 · 物理学 2016-04-13 Patrick R. Mickel , Hyoungjeen Jeen , Pradeep Kumar , Amlan Biswas , Arthur F. Hebard

Polycrystalline ceramic samples and a single crystal of EuTiO3 have been investigated by Raman spectroscopy in the temperature range 80-300 K. Although synchrotron XRD data clearly indicated the cubic to tetragonal phase transition around…

材料科学 · 物理学 2021-04-21 P. Pappas , E. Liarokapis , M. Calamiotou , A. Bussmann-Holder

We apply the density-functional theory to study various phases (including non-magnetic (NM), anti-ferromagnetic (AFM), and ferromagnetic (FM)) in monolayer magnetic chromium triiodide (CrI$_3$), a recently fabricated 2D magnetic material.…

介观与纳米尺度物理 · 物理学 2018-10-17 Lucas Webster , Liangbo Liang , Jia-An Yan

The temperature dependence of eigenfrequencies and intensities of the IR active modes has been investigated for the antiferromagnetic chromium spinel compounds CdCr2O4, ZnCr2O4, ZnCr2S4, ZnCr2Se4, and HgCr2S4 by IR spectroscopy for…

强关联电子 · 物理学 2007-07-05 T. Rudolf , Ch. Kant , F. Mayr , J. Hemberger , V. Tsurkan , A. Loidl

Magnetic excitations in layered magnetic materials that can be thinned down the two-dimensional (2D) monolayer limit are of high interest from a fundamental point of view and for applications perspectives. Raman scattering has played a…

介观与纳米尺度物理 · 物理学 2023-02-20 Amit Pawbake , Thomas Pelini , Nathan P. Wilson , Kseniia Mosina , Zdenek Sofer , Rolf Heid , Clement Faugeras

Motivated by the possibility of an intermediate U(1) quantum spin liquid phase in out-of-plane magnetic fields and enhanced magnetic fluctuations in exfoliated {\alpha}-RuCl3 flakes, we study magneto-Raman spectra of exfoliated multilayer…

We theoretically study origins of the ferroelectricity in the multiferroic phases of the rare-earth (R) Mn perovskites, RMnO3, by constructing a realistic spin model including the spin-phonon coupling, which reproduces the entire…

强关联电子 · 物理学 2011-02-21 Masahito Mochizuki , Nobuo Furukawa , Naoto Nagaosa

We employ polarization-resolved Raman spectroscopy and first-principles phonon calculations to study the lattice dynamics and spin-phonon coupling in the kagome spin ice compound HoAgGe. Upon cooling, HoAgGe shows transitions from a…

强关联电子 · 物理学 2025-03-11 Shangfei Wu , Lingxiao Zhao , Wei Song , Mingshu Tan , Feng Jin , Tianping Ying , Jia-Xin Yin , Qingming Zhang

In condensed matter physics broken symmetries and emergence of quasi-particles are intimately linked to each other. Whenever a symmetry is broken, it leaves its fingerprints, and that may be observed indirectly via its influence on the…

材料科学 · 物理学 2020-01-15 Birender Singh , Sunil Kumar , Pradeep Kumar

We investigated complex magnetic properties of multifunctional LaCrO3-LaFeO3 system. The magnetic measurements substantiate the presence of competing complex magnetic ordering against temperature, showing paramagnetic to ferrimagnetic…

强关联电子 · 物理学 2019-08-20 Brajesh Tiwari , Ambesh Dixit , M. S. Ramachandra Rao