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Pyroelectric current and magnetoelectric coupling measurements on polycrystalline samples of the quadruple perovskite (LaMn$_{3}$)Mn$_{4}$O$_{12}$ give evidence of ferroelectricity driven by the antiferromagnetic ordering of the $B$-site…

We have systematically investigated the magnetic properties and magnetocaloric effect (MCE) in $R$MnO$_3$ ($R$$=$Dy, Tb, Ho and Yb) single crystals. Above a critical value of applied field ($H_c$), $R$MnO$_3$ undergo a first-order…

强关联电子 · 物理学 2011-12-23 A. Midya , S. N. Das , P. Mandal , S. Pandya , V. Ganesan

We present a simple theory for structural transitions in displacive ferroelectrics of the perovskite type. In our theory, the competition between the elastic energy cost for the displacement of the homopolar ion from the centrosymmetric…

材料科学 · 物理学 2007-05-23 K. Sheshadri , Rangan Lahiri Pushan Ayyub , Shobo Bhattacharya

Investigation of the electronic and spin structure in double perovskites is recently attracting significant attention, mainly driven by their unique multifunctional properties and other underlying charge and spin dynamics. Herein, using…

材料科学 · 物理学 2023-07-18 R. Hissariya , R. Sharma , S. K. Mishra

Orthorhombic HoMnO3 is a multiferroic in which Mn antiferromagnetic order induces ferroelectricity. A second transition occurs within the multiferroic phase, in which a strong enhancement of the ferroelectric polarization occurs…

强关联电子 · 物理学 2021-01-04 Y. W. Windsor , M. Ramakrishnan , L. Rettig , A. Alberca , T. Lippert , C. W. Schneider , U. Staub

Magnetic and ferroelectric properties of layered geometrically frustrated cluster compound FeTe$_2$O$_5$Br were investigated with single-crystal neutron diffraction and dielectric measurements. Incommensurate amplitude modulated magnetic…

材料科学 · 物理学 2009-10-01 M. Pregelj , O. Zaharko , A. Zorko , Z. Kutnjak , P. Jeglic , P. J. Brown , M. Jagodic , Z. Jaglicic , H. Berger , D. Arcon

We have discovered strong magnetoelectric (ME) effects in the single chiral-helical magnetic state of single-crystalline langasite Ba3NbFe3Si2O14 that is crystallographically chiral. The ferroelectric polarization, predominantly aligned…

强关联电子 · 物理学 2014-03-26 Nara Lee , Young Jai Choi , Sang-Wook Cheong

Epitaxial CaMnO3 films grown with 2.3% tensile strain on (001)-oriented LaAlO3 substrates are found to be incipiently ferroelectric below 25 K. Optical second harmonic generation (SHG) was used for the detection of the incipient…

材料科学 · 物理学 2015-06-05 T. Günter , E. Bousquet , A. David , Ph. Boullay , Ph. Ghosez , W. Prellier , M. Fiebig

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

材料科学 · 物理学 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

Sm$_2$Ti$_2$O$_7$, a member of rare-earth titanate pyrochlores, exhibits dipolar-octupolar antiferromagnetism below $T_N$ = 0.35 K. We observed two ferroelectric transitions at 182 ($T_{FE1}$) and 52 K ($T_{FE2}$), significantly higher than…

材料科学 · 物理学 2024-07-30 S. Mukherjee , O. Ivashko , S. Majumdar , A. Kumar , S. Giri

By means of magnetic, specific heat and pyroelectric measurements, we report on magnetic ferroelectricity in the quadruple perovskite \namno, characterized by a canted antiferromagnetic (AFM) CE structure. Surprisingly, ferroelectricity is…

A dielectric anomaly has been found near the incommensurate to commensurate antiferromagnetic phase transition (TN2=230 K) in YBaCuFeO5 ceramics, a compound which crystallizes in an ordered perovskite structure. The existence of electric…

材料科学 · 物理学 2009-03-13 B. Kundys , A. Maignan , Ch. Simon

Magneto-dielectric spectra of La0.95Ca0.05CoO3 covering the crossover of spin states reveals strong coupling of its spin and dipolar degrees of freedom. Signature of spin-state transition at 30K clearly manifests in magnetization, supported…

材料科学 · 物理学 2016-02-29 Suchita Pandey , Jitender Kumar , A. M. Awasthi

Polarization induced spin switching of atoms in magnetic materials opens for possibilities to design and develop advanced spintronic devices, in particular, storage devices where the magnetic state can be controlled by an electric field. We…

材料科学 · 物理学 2018-10-09 Indukuru Ramesh Reddy , Peter M. Oppeneer , Kartick Tarafder

Crystal and magnetic structures of the high-pressure stabilized perovskite phase of TlMnO3 have been studied by neutron powder diffraction. The crystal structure involves two types of primary structural distortions: a+b-b-octahedral tilting…

强关联电子 · 物理学 2019-03-07 Dmitry D. Khalyavin , Pascal Manuel , Wei Yi , Alexei A. Belik

Experiments have been performed to measure magnetoelectric properties of room temperature spirally ordered Sr3Co2Fe24O41 hexaferrite slabs. The measured properties include the magnetic permeability, the magnetization and the strain all as a…

材料科学 · 物理学 2015-06-03 Khabat Ebnabbasi , Carmine Vittoria , Allan Widom

We investigate the crystal structure in multiferroic tetragonal perovskite Sr$_{1/2}$Ba$_{1/2}$MnO$_3$ with high accuracy of the order of 10$^{-3}$ Angstrom for an atomic displacement. The large atomic displacement for Mn ion from the…

材料科学 · 物理学 2020-07-15 D. Okuyama , K. Yamauchi , H. Sakai , Y. Taguchi , Y. Tokura , K. Sugimoto , T. J. Sato , T. Oguchi

The coupling between localized spins and phonons can lead to shifts in the dielectric constant of insulating materials at magnetic ordering transitions. Studies on isostructural SeCuO3 (ferromagnetic) and TeCuO3 (antiferromagnetic)…

材料科学 · 物理学 2009-04-14 G. Lawes , T. Kimura , C. M. Varma , M. A. Subramanian , R. J. Cava , A. P. Ramirez

SmCrO$_3$ single crystals were successfully grown utilizing the high-pressure optical floating-zone method and their crystal structure, magnetization behavior, and magnetic phase diagrams were thoroughly investigated. Magnetic studies were…

Observation of ferroelectricity among non-d0 systems, which was believed for a long time an unrealistic concept, led to various proposals for the mechanisms to explain the same (i.e. magnetically induced ferroelectricity) during last…