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We propose a systematic approach to obtain various forms of insulating titanium oxynitrides Ti$_{n}$N$_{2}$O$_{2n-3}$ and we conduct a detailed study on its $n=2$ case, Ti$_{2}$N$_{2}$O. We study the energetics and the electronic structures…

材料科学 · 物理学 2019-03-06 Yuta Aoki , Sinisa Coh , Steven G. Louie , Marvin L. Cohen , Susumu Saito

Thin TiO2 films on quartz substrates were prepared by spin coating of undoped and metal-ion-doped Sol Gel precursors. These films were characterised by Scanning Electron Microscopy, Laser Raman Microspectroscopy, Xray Diffraction and UV Vis…

材料科学 · 物理学 2021-06-08 D. A. H. Hanaor , G. Triani , C. C. Sorrell

Titanium dioxide materials have been studied intensively and extensively due to photocatalytic applications. A long-standing open question is the energy band alignment of rutile and anatase TiO2 phases, which can affect the photocatalytic…

材料科学 · 物理学 2015-11-10 Daoyu Zhang , Minnan Yang , Shuai Dong

TiO2 is a wide band-gap semiconductor that has been intensively investigated for photocatalysis and water-spiting. However, weak light absorption in the visible region of the spectrum poses stringent limitation to its practical application.…

材料科学 · 物理学 2023-02-07 Fernando P. Sabino , Anderson Janotti

TiO$_2$ and SrTiO$_3$ are well known materials in the field of photocatalysis due to their exceptional electronic structure, high chemical stability, non-toxicity and low cost. However, owing to the wide band gap, these can be utilized only…

材料科学 · 物理学 2020-09-25 Manish Kumar , Pooja Basera , Shikha Saini , Saswata Bhattacharya

Photocatalysis, a promising solution for environmental challenges, relies on the generation and utilization of photogenerated charge carriers within photocatalysts. However, recombination of these carriers often limits efficiency.…

材料科学 · 物理学 2024-03-18 Mona Asadinamin , Aleksandar Živkovic , Nora H. De Leeuw , Steven P. Lewis

Titanium dioxide is a photocatalytic substance of great practical importance. However, with its bandgap in the ultraviolet (UV) regime, native forms (undoped) of TiO2 generally exhibits poor photocatalytic activities under visible light.…

化学物理 · 物理学 2013-12-04 Mingzheng Wang , Ka-Kit Yee , Biao Nie , Hua Cheng , Jian Lu , Linbao Luo , Zhengtao Xu , Yang Yang Li

Nanostructured TiO2 thin films were prepared by pulsed laser deposition (PLD) on indium doped tin oxide (ITO) substrates. Results from X-ray photoelectron spectroscopy (XPS) show that Ti 2p core level peaks shift toward the lower binding…

材料科学 · 物理学 2007-12-20 H. Lin , Abdul K. Rumaiz , Meghan Schulz , Demin Wang , Reza Rock , C. P. Huang , S. Ismat Shah

Titanium dioxide is one of the most widely investigated oxides. This is due to its broad range of applications, from catalysis to photocatalysis to photovoltaics. Despite this large interest, many of its bulk properties have been sparsely…

材料科学 · 物理学 2010-03-12 L. Chiodo , J. M. García-Lastra , D. J. Mowbray , A. Iacomino , A. Rubio

The rutile TiO$_2$ (110) surface reduced by the bridging oxygen vacancy, bridging hydroxyl group or Ti interstitial atom has been investigated by calculating their electronic structures using the density functional theory plus U method. It…

材料科学 · 物理学 2015-10-13 Daoyu Zhang , Minnan Yang , Shuai Dong

Surface fluorination of TiO$_2$ (F-TiO$_2$) has complicate photocatalytic behavior in degradation of organic compounds. This work attempts to establish an elegant scenario based on the band model to understand this behavior. Density…

材料科学 · 物理学 2017-11-21 Huimin Gao , Daoyu Zhang , Minnan Yang , Shuai Dong

Understanding the mechanism of the heterojunction is an important step towards controllable and tunable interfaces for photocatalytic and photovoltaic based devices. To this aim, we propose a thorough study of a double heterostructure…

计算物理 · 物理学 2019-04-04 Slimane Haffad

Photocatalytic reactions on TiO2 have recently gained an enormous resurgence because of various new strategies and findings that promise to drastically increase efficiency and specificity of such reactions by modifications of the titania…

应用物理 · 物理学 2020-04-13 Xuemei Zhou , Ning Liu , Patrik Schmuki

Using an organometallic precursor, TiO$_2$ coatings were fabricated on surfaces of quartz, zircon and rutile sands. X ray Diffraction, X ray Fluorescence, UV Vis spectroscopy and surface area measurement were used to characterise support…

材料科学 · 物理学 2021-06-08 Dorian A. H. Hanaor , Charles C. Sorrell

A template-free process for the synthesis of nanocrystalline TiO2 hierarchical microstructures by reactive Pulsed Laser Deposition (PLD) is here presented. By a proper choice of deposition parameters a fine control over the morphology of…

材料科学 · 物理学 2013-11-28 F. Di Fonzo , C. S. Casari , V. Russo , M. F. Brunella , A. Li Bassi , C. E. Bottani

Visible-light photocatalyst titanium dioxide (TiO2) was successfully prepared via a novel and facile single-mode microwave assisted synthesis process. In this one-step synthesis, Ti as target material selectively oxides in magnetic field…

应用物理 · 物理学 2022-02-04 Kunihiko Katoa , Sebastien Vaucher , Patrik Hoffmann , Yunzi Xin , Takashi Shirai

We perform first-principles calculations to investigate the band structure, density of states, optical absorption, and the imaginary part of dielectric function of Cu, Ag, and Au-doped anatase TiO2 in 72 atoms systems. The electronic…

材料科学 · 物理学 2015-08-10 Meili Guo , Jiulin Du

TiO2 nanotube arrays grown by anodization were coated with thin layers of polydopamine as visible light sensitizer. The PDA-coated TiO2 scaffolds were used as photocatalyst for selective oxidation of benzyl alcohol under monochromatic…

材料科学 · 物理学 2016-10-18 Jyotsna Tripathy , Gabriel Loget , Marco Altomare , Patrik Schmuki

Photoreforming is a clean photocatalytic technology for simultaneous plastic waste degradation and hydrogen fuel production, but there are still limited active and stable catalysts for this process. This work introduces the brookite…

材料科学 · 物理学 2024-08-21 Thanh Tam Nguyen , Kaveh Edalati

Here we investigate the band-level energetics of "black" hydrogenated titania in different polymorphs using in-situ photoelectrochemical measurements and XPS valence band measurements. We find that the conduction band of black rutile is…

化学物理 · 物理学 2020-04-27 Xuemei Zhou , Ewa Wierzbicka , Ning Liu , Patrik Schmuki
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