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Manufacturing new soft materials with specific optical, mechanical and magnetic properties is a significant challenge. Assembling and manipulating colloidal particles at fluid interfaces is a promising way to make such materials. We use…

软凝聚态物质 · 物理学 2014-10-29 Gary B. Davies , Timm Krüger , Peter V. Coveney , Jens Harting , Fernando Bresme

We perform molecular dynamics simulations to understand the translational and rotational diffusion of Janus nanoparticles at the interface between two immiscible fluids. Considering spherical particles with different affinity to fluid…

流体动力学 · 物理学 2016-05-04 Hossein Rezvantalab , German Drazer , Shahab Shojaei-Zadeh

We propose a primitive model of Janus ellipsoids that represent particles with an ellipsoidal core and two semi-surfaces coded with dissimilar properties, for example, hydrophobicity and hydrophilicity, respectively. We investigate the…

软凝聚态物质 · 物理学 2015-03-19 Ya Liu , Wei Li , Toni Perez , J. D. Gunton , Genevieve Brett

Capillary interactions have emerged as a tool for the directed assembly of particles adsorbed at fluid-fluid interfaces, and play a role in controlling the mechanical properties of emulsions and foams. In this paper, following Davies et al.…

软凝聚态物质 · 物理学 2015-07-23 Gary B. Davies , Lorenzo Botto

Janus particles have attracted significant interest as building blocks for complex materials in recent years. Furthermore, capillary interactions have been identified as a promising tool for directed self-assembly of particles at…

软凝聚态物质 · 物理学 2015-03-13 Qingguang Xie , Gary B. Davies , Florian Günther , Jens Harting

Capillary interactions can be used to direct assembly of particles adsorbed at fluid-fluid interfaces. Precisely controlling the magnitude and direction of capillary interactions to assemble particles into favoured structures for materials…

软凝聚态物质 · 物理学 2016-07-11 Qingguang Xie , Gary B. Davies , Jens Harting

The equilibrium properties of a Janus fluid confined to a one-dimensional channel are exactly derived. The fluid is made of particles with two faces (active and passive), so that the pair interaction is that of hard spheres, except if the…

统计力学 · 物理学 2020-07-01 M. A. G. Maestre , A. Santos

Using large scale molecular dynamics simulations we study the orientational dynamics of a heated Janus particle which exhibits self-propulsion. The asymmetry in the microscopic interaction of the colloid with the solvent is implemented by…

软凝聚态物质 · 物理学 2018-11-14 Dipanjan Chakraborty

Colloidal assembly at fluid interfaces has a great potential for the bottom-up fabrication of novel structured materials. However, challenges remain in realizing controllable and tunable assembly of particles into diverse structures.…

软凝聚态物质 · 物理学 2020-12-29 Qingguang Xie , Jens Harting

We numerically investigate the propelled motions of a Janus particle in a periodically phase-separating binary fluid mixture. In this study, the surface of the particle tail prefers one of the binary fluid components and the particle head…

软凝聚态物质 · 物理学 2015-04-06 Takeaki Araki , Shintaro Fukai

Molecular dynamics simulations are carried out to study the translational and rotational diffusion of a single Janus particle immersed in a dense Lennard-Jones fluid. We consider a spherical particle with two hemispheres of different…

软凝聚态物质 · 物理学 2015-06-18 Ali Kharazmi , Nikolai V. Priezjev

If an active Janus particle is trapped at the interface between a liquid and a fluid, its self-propelled motion along the interface is affected by a net torque on the particle due to the viscosity contrast between the two adjacent fluid…

软凝聚态物质 · 物理学 2016-02-15 P. Malgaretti , M. N. Popescu , S. Dietrich

Using fluorescence microscopy we study the adsorption of single latex microparticles at a water/water interface between demixing aqueous solutions of polymers, generally known as a water-in-water emulsion. Similar microparticles at the…

软凝聚态物质 · 物理学 2018-05-23 Louis Keal , Carlos E. Colosqui , Hans Tromp , Cecile Monteux

The diffusion of a Janus rod-shaped nanoparticle in a dense Lennard-Jones fluid is studied using molecular dynamics (MD) simulations. The Janus particle is modeled as a rigid cylinder whose atoms on each half-side have different interaction…

软凝聚态物质 · 物理学 2017-07-31 Ali Kharazmi , Nikolai V. Priezjev

The interactions of autonomous microswimmers play an important role for the formation of collective states of motile active matter. We study them in detail for the common microswimmer-design of two-faced Janus spheres with hemispheres made…

软凝聚态物质 · 物理学 2021-08-09 Sven Auschra , Andreas Bregulla , Klaus Kroy , Frank Cichos

Self-assembly of Janus (or `patchy') particles is dependent on the precise interaction between neighbouring particles. Here, the orientations of two amphiphilic Janus spheres within a dimer in an explicit fluid are studied with high…

软凝聚态物质 · 物理学 2021-08-18 Sina Safaei , Caleb Todd , Jack Yarndley , Shaun Hendy , Geoff R. Willmott

A lattice gas simulation of water between a hydrophobic plate and a hydrophilic plate (a Janus interface) shows large fluctuations in the number of liquid cells in contact with the hydrophobic plate, and a power spectrum similar to the…

软凝聚态物质 · 物理学 2009-11-10 Thomas A. McCormick

The adsorption behavior of ions at liquid-vapor interfaces exhibits several unexpected yet generic features. In particular, energy and entropy are both minimum when the solute resides near the surface, for a variety of ions in a range of…

统计力学 · 物理学 2017-02-08 Suriyanarayanan Vaikuntanathan , Patrick R. Shaffer , Phillip L. Geissler

We study the effects of heterogeneity on interfacial pinning and hydrodynamic drag using molecular dynamics (MD) simulations of Janus nanospheres at a liquid/vapor interface. We construct the free energy landscape for this system, both in…

软凝聚态物质 · 物理学 2019-04-17 Joel Koplik , Charles Maldarelli

Based on extensive Monte Carlo simulations and analytical considerations we study the electrostatically driven adsorption of flexible polyelectrolyte chains onto charged Janus nanospheres. These net-neutral colloids are composed of two…

软凝聚态物质 · 物理学 2017-09-13 Sidney J. de Carvalho , Ralf Metzler , Andrey G. Cherstvy
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