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We report measurements of the specific heat and magnetization of single crystal samples of the spin-1/2 kagome compound ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ (herbertsmithite), a promising quantum spin-liquid candidate, in high magnetic fields and…

We report 17O NMR measurements in the S=1/2 Cu2+ kagome antiferromagnet Herbertsmithite ZnCu3(OH)6Cl2 down to 45mK in magnetic fields ranging from 2T to 12T. While Herbertsmithite displays a gapless spin-liquid behavior in zero field, we…

强关联电子 · 物理学 2013-09-09 M. Jeong , F. Bert , P. Mendels , F. Duc , J. C. Trombe , M. A. de Vries , A. Harrison

We present transverse field muon spin rotation/relaxation measurements on single crystals of the spin-1/2 kagome antiferromagnet Herbertsmithite. We find that the spins are more easily polarized when the field is perpendicular to the kagome…

强关联电子 · 物理学 2015-05-20 Oren Ofer , Amit Keren , Jess H. Brewer , Tianheng H. Han , Young S. Lee

The magnetization process of an S=1/2 antiferromagnet on the kagome lattice, [Cu_3(titmb)_2(OCOCH_3)_6]H_2O {titmb= 1,3,5-tris(imidazol-1-ylmethyl)-2,4,6 trimethylbenzene} has been measured at very low temperatures in both pulsed and steady…

We present magnetization measurements on oriented powder of ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ along and perpendicular to the orienting field. We find a dramatic difference in the magnetization between the two directions. It is biggest at low…

强关联电子 · 物理学 2009-04-21 Oren Ofer , Amit Keren

The dc-magnetization of the unique S=1/2 kagome antiferromagnet Herbertsmithite has been measured down to 0.1K. No sign of spin freezing is observed in agreement with former muSR and ac-susceptibility results. The low temperature magnetic…

强关联电子 · 物理学 2009-11-13 F. Bert , S. Nakamae , F. Ladieu , D. L'Hôte , P. Bonville , F. Duc , J. -C. Trombe , P. Mendels

Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel…

强关联电子 · 物理学 2017-01-06 A. Zorko , M. Herak , M. Gomilšek , J. van Tol , M. Velázquez , P. Khuntia , F. Bert , P. Mendels

The magnetization of two spin-1/2 kagome antiferromagnets, volborthite and vesignieite, has been measured in pulsed magnetic fields up to 68 T. A magnetization plateau is observed for each compound near the highest magnetic field.…

强关联电子 · 物理学 2015-05-27 Yoshihiko Okamoto , Masashi Tokunaga , Hiroyuki Yoshida , Akira Matsuo , Koichi Kindo , Zenji Hiroi

We present a Raman spectroscopic investigation of the Herbertsmithite ZnCu3(OH)6Cl2, the first realization of a Heisenberg s=1/2 antiferromagnet on a perfect kagome lattice. The magnetic excitation spectrum of this compound is dominated by…

Herbertsmithite, ZnCu3(OH)6Cl2, is the prototype candidate for a spin liquid behavior on a geometrically perfect kagome lattice. Its discovery and the absence of any evidence for spin-freezing down to the lowest probed temperature to-date…

强关联电子 · 物理学 2015-05-28 P. Mendels , F. Bert

The magnetization process of the orthogonal-dimer antiferromagnet SrCu2(BO3)2 is investigated in high magnetic fields of up to 118 T. A 1/2 plateau is clearly observed in the field range 84 to 108 T in addition to 1/8, 1/4 and 1/3 plateaux…

The magnetization process of the spin-S Heisenberg antiferromagnet on the kagome lattice is studied by the numerical-diagonalization method. Our numerical-diagonalization data for small finite-size clusters with S=1, 3/2, 2, and 5/2 suggest…

材料科学 · 物理学 2015-05-27 Hiroki Nakano , Toru Sakai

We investigate the structural and magnetic properties of BaNi$_3$(AsO$_4$)$_2$(OH)$_2$, focusing on its spin-1 kagome lattice and the intricate coexistence of ferromagnetic and antiferromagnetic interactions. Powder x-ray diffraction…

强关联电子 · 物理学 2025-08-14 Yuya Haraguchi , Jun-ichi Yamaura , Akira Matsuo , Koichi Kindo , Hiroko Aruga Katori

A recently discovered kagome antiferromagnet $\rm{Y}_3\rm{Cu}_9(\rm{OH})_{19}\rm{Cl}_8$ has attracted significant interest due to its unique kagome lattice structure and magnetic properties. The kagome lattice has three types of exchange…

强关联电子 · 物理学 2024-09-27 Kazu Bodaiji , Katsuhiro Morita , Yoshiyuki Fukumoto

We have performed magnetization measurements at high magnetic fields of up to 53 T on single crystals of a uranium heavy-fermion compound U$_2$Zn$_{17}$ grown by the Bridgman method. In the antiferromagnetic state below the N\'{e}el…

High-field electron spin resonance (ESR) measurements have been performed on vesignieite BaCu$_3$V$_2$O$_8$(OH)$_2$, which is considered as a nearly ideal model substance of $S$=1/2 kagome antiferromagnet, in the temperature region from 1.9…

A spin-1/2 Heisenberg model on honeycomb lattice is investigated by doing triplon analysis and quantum Monte Carlo calculations. This model, inspired by Cu$_2$(pymca)$_3$(ClO$_4$), has three different antiferromagnetic exchange interactions…

强关联电子 · 物理学 2021-09-15 Meghadeepa Adhikary , Arnaud Ralko , Brijesh Kumar

We clarify the existence of several magnetization plateaux for the kagome $S=1/2$ antiferromagnetic Heisenberg model in a magnetic field. Using approximate or exact localized magnon eigenstates, we are able to describe in a similar manner…

强关联电子 · 物理学 2013-10-30 Sylvain Capponi , Oleg Derzhko , Andreas Honecker , Andreas M. Läuchli , Johannes Richter

The frustration of antiferromagnetic interactions on the loosely connected kagome lattice associated to the enhancement of quantum fluctuations for S=1/2 spins was acknowledged long ago as a keypoint to stabilize novel ground states of…

强关联电子 · 物理学 2011-03-16 Philippe Mendels , Fabrice Bert

Herbertsmithite is known as the archetype of a S=1/2 nearest-neighbor Heisenberg antiferromagnet on the Kagom\'e lattice, theoretically presumed to be a quantum gapless spin liquid. However, more and more experiments reveal that the model…

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