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Ionization of acetylene by linearly-polarized, vacuum ultraviolet (VUV) laser pulses is modelled using time-dependent density functional theory. Several laser wavelengths are considered including one that produces direct ionization to the…

原子物理 · 物理学 2017-04-24 Daniel Dundas , Peter Mulholland , Abigail Wardlow , Alejandro de la Calle

The single ionization of noble gas atoms by the combined action of XUV attopulses and an infrared laser field is theoretically investigated by means of a non-perturbative model that under certain approximations gives closed-form expressions…

原子物理 · 物理学 2015-12-21 D. I. R. Boll , O. A. Fojón

We show that the correlation dynamics in coherently excited doubly excited resonances of helium can be followed in real time by two-photon interferometry. This approach promises to map the evolution of the two-electron wave packet onto…

量子物理 · 物理学 2013-05-24 J. Feist , S. Nagele , C. Ticknor , B. I. Schneider , L. A. Collins , J. Burgdörfer

We report on a kinematically complete experiment on strong field double ionization of helium using laser pulses with a wavelength of 394\,nm and intensities of $3.5-5.7\times10^{14}\,W/cm^2$. Our experiment reaches the most complete level…

Multiphoton ionization of sodium by femtosecond laser pulses of 800 nm wavelength in the range of laser peak intensities entering over-the-barrier ionization domain is studied. Photoelectron momentum distributions and the energy spectra are…

原子物理 · 物理学 2021-02-24 A. Bunjac , D. B. Popovic , N. S. Simonovic

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

原子物理 · 物理学 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a…

原子物理 · 物理学 2015-05-28 Feng He , Camilo Ruiz , Andreas Becker , Uwe Thumm

This paper presents measurements of the energy radiated by the lower solar atmosphere, at optical, UV, and EUV wavelengths, during an X-class solar flare (SOL2011-02-15T01:56) in response to an injection of energy assumed to be in the form…

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

We present a table-top extreme ultraviolet (XUV) beamline for measuring time- and frequency-resolved XUV excited optical luminescence (XEOL) with additional femtosecond-resolution XUV transient absorption spectroscopy functionality. XUV…

We demonstrate an accurate phase retrieval of XUV atomic ionization by streaking the photoelectron in a circularly polarized IR laser field. The streaking phase can then be converted to the atomic time delay containing the Wigner and…

Pulses of extreme ultraviolet (XUV) light, with wavelengths between 10 and 100$\,$nm, can be used to image and excite ultra-fast phenomena such as the motion of atomic electrons. Here we show that the illumination of plasma with…

等离子体物理 · 物理学 2018-08-24 T. G. Blackburn , A. A. Gonoskov , M. Marklund

Pump-probe photoionization has been used to map the relaxation processes taking place from highly vibrationally excited levels of the S2 state of azulene, populated directly or via internal conversion from the S4 state. Photoelectron…

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

We investigate the influence of relativistic nondipole effects on the photoelectron spectra of argon, particularly in the low kinetic energy region (0 eV - 5 eV). In our experiment, we use intense linearly polarised 800 nm laser pulse to…

原子物理 · 物理学 2022-03-14 Nida Haram , Han Xu , Igor Ivanov , Dashavir Chetty , Igor Litvinyuk , R. T. Sang

Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…

We theoretically study how time- and angle-resolved photoemission spectroscopy can be applied for imaging coherent electron dynamics in molecules. We consider a process in which a pump pulse triggers coherent electronic dynamics in a…

光学 · 物理学 2018-12-11 Daria Popova-Gorelova , Jochen Küpper , Robin Santra

We propose a continuous variable quantum state tomography protocol of electrons which result from the ionization of atoms or molecules by the absorption of extreme ultraviolet light pulses. Our protocol is benchmarked against a direct…

In this paper, we report the results of measurements of the intensities and delays of super-radiance decays from excited helium atoms at multiple wavelengths. The experiment was performed using extreme ultraviolet radiation produced by the…

Intense extreme-ultraviolet (XUV) pulses enable the investigation of XUV-induced nonlinear processes and are a prerequisite for the development of attosecond pump - attosecond probe experiments. While highly nonlinear processes in the XUV…