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This paper introduces Spectral Incoherent Diffractive Imaging (SIDI) as a novel method for achieving dark-field imaging of nanostructures with heterogeneous oxidation states. With SIDI, shifts in photoemission profiles can be spatially…

光学 · 物理学 2023-12-25 Tamme Wollweber , Kartik Ayyer

X-ray diffraction studies of nanoporous gold face the poorly understood diffraction scenario where large coherent crystals are riddled with nanoscale holes. Theoretical considerations derived in this study show that the ligament size of the…

材料科学 · 物理学 2017-12-27 Matthias Graf , Bao-Nam Dinh Ngô , Jörg Weissmüller , Jürgen Markmann

Direct nanoimprinting provides a simple and high-throughput route for producing uniform nanopatterns at great precision and at low costs. However, applying this technique to crystalline metals has been considered as impossible due to…

介观与纳米尺度物理 · 物理学 2019-08-07 Ze Liu

X-ray free-electron lasers (XFELs) offer unique capabilities for measuring the structure and dynamics of biomolecules, helping us understand the basic building blocks of life. Notably, high-repetition-rate XFELs enable single particle…

计算机视觉与模式识别 · 计算机科学 2023-12-25 Jay Shenoy , Axel Levy , Frédéric Poitevin , Gordon Wetzstein

The short and intense pulses of the new X-ray free electron lasers, now operational or under construction, may make possible diffraction experiments on single molecule-sized objects with high resolution, before radiation damage destroys the…

数据分析、统计与概率 · 物理学 2012-04-11 Miklós Tegze , Gábor Bortel

Three-dimensional electron diffraction (3D ED) has emerged as a powerful method for solving the structures of sub-micron-sized particles down to nanoparticles. However, it faces technical challenges when applied to beam-sensitive samples or…

The classical method of determining the atomic structure of complex molecules by analyzing diffraction patterns is currently undergoing drastic developments. Modern techniques for producing extremely bright and coherent X-ray lasers allow a…

生物大分子 · 定量生物学 2015-10-12 Tomas Ekeberg , Stefan Engblom , Jing Liu

A differential interference contrast microscopy technique, which employs a photonic crystal fiber as a white-light source, is used to measure both the real and imaginary parts of the complex dielectric constant of single 10 and 15 nm gold…

材料科学 · 物理学 2009-11-11 Patrick Stoller , Volker Jacobsen , Vahid Sandoghdar

With X-ray free-electron lasers (XFELs), it is possible to determine the three-dimensional structure of noncrystalline nanoscale particles using X-ray single-particle imaging (SPI) techniques at room temperature. Classifying SPI scattering…

机器学习 · 计算机科学 2023-02-15 Cong Wang , Eric Florin , Hsing-Yin Chang , Jana Thayer , Chun Hong Yoon

Shape measurement of rod-shaped particles in fluids is an outstanding challenge with applications in characterising synthetic functional nanoparticles and in early warning detection of rod-shaped pathogens in water supplies. However, it is…

光学 · 物理学 2024-05-14 Yumeng Yin , Aurelien Trichet , Jiangrui Qian , Jason Smith

This paper describes an imaging microscopic technique based on heterodyne digital holography where subwavelength-sized gold colloids can be imaged in cell environment. Surface cellular receptors of 3T3 mouse fibroblasts are labeled with 40…

Nanoscale phase-control is one of the most powerful approaches to specifically tailor electrical fields in modern nanophotonics. Especially the precise sub-wavelength assembly of many individual nano-building-blocks has given rise to…

光学 · 物理学 2021-05-26 Lisa Saemisch , Niek F. van Hulst , Matz Liebel

The advent of X-ray Free Electron Lasers promises the possibility to determine the structure of individual particles such as microcrystallites, viruses and biomolecules from single-shot diffraction snapshots obtained before the particle is…

软凝聚态物质 · 物理学 2010-05-06 Brian Moths , Abbas Ourmazd

UV-Vis absorption spectroscopy is frequently used to characterize the size and shape of gold nanoparticles. We present a full-spectrum model that yields reliable results for the commonly encountered case of mixtures of spheres and rods in…

软凝聚态物质 · 物理学 2015-04-07 Kostyantyn Slyusarenko , Benjamin Abécassis , Patrick Davidson , Doru Constantin

Identifying the three-dimensional (3D) crystal-plane and strain-field distributions of nanocrystals is essential for optical, catalytic, and electronic applications. Here, we developed a methodology for visualizing the 3D information of…

A novel method for single-step, lithography-free, and large-scale laser writing of nanoparticle-based plasmonic structures has been developed. Changing energy of femtosecond laser pulses and thickness of irradiated gold film it is possible…

Live cell imaging using metallic nanoparticles as tags is an emerging technique to visualize long and highly dynamic processes due to the lack of photobleaching and high photon rate. However, the lack of excited states as compared to…

介观与纳米尺度物理 · 物理学 2011-01-12 H. E. Grecco , O. E. Martínez

The influence of delay-time between two sequential femtosecond pulses on the properties of nanoparticles obtained via laser ablation of gold in ethanol has been studied. The morphological and optical properties of the nanoparticles attained…

介观与纳米尺度物理 · 物理学 2010-08-03 E. Axente , M. Barberoglou , P. G. Kuzmin , E. Magoulakis , P. A. Loukakos , E. Stratakis , G. A. Shafeev , C. Fotakis

Materials modelling and processing require experiments to visualize and quantify how external excitations drive the evolution of deep subsurface structure and defects that determine properties. Today, 3D movies with ~100-nm resolution of…

Imaging of the optical properties of individual nanosystems beyond fluorescence can provide a wealth of information. However, the minute signals for absorption and dispersion are challenging to observe, and only specialized techniques…

光学 · 物理学 2015-09-10 Matthias Mader , Jakob Reichel , Theodor W. Hänsch , David Hunger