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Cold collisions of light molecules are often dominated by a single partial wave resonance. For the rotational quenching of HD(v=1,j=2) by collisions with ground state para-H2, the process is dominated by a single L=2 partial wave resonance…

Full-dimensional quantum scattering calculations are reported for ro-vibrational transitions in HD+HD collisions using a highly accurate interaction potential for the H$_2$-H$_2$ system. Several near-resonant ro-vibrational transitions are…

原子物理 · 物理学 2026-03-06 Bikramaditya Mandal , Hubert Jóźwiak , Piotr Wcisło , Naduvalath Balakrishnan

We present numerical results for rate coefficients of reaction and vibrational quenching in the collision of H with D$_2(v,j)$ at cold and ultracold temperatures. We explore both ortho-D$_2(j\!=\!0)$ and para-D$_2(j\!=\!1)$ for several…

原子物理 · 物理学 2017-05-24 I. Simbotin , R. Côté

We report numerically exact quantum scattering calculations on magnetic Feshbach resonances in ultracold, strongly anisotropic atom-molecule [Rb($^2$S) + SrF($^2\Sigma^+$)] collisions based on state-of-the-art ab initio potential energy…

A close coupling quantum-mechanical calculation is performed for rotational energy transfer in a HD+HD collision at very low energy, down to the ultracold temperatures: $T \sim 10^{-8}$ K. A global six-dimensional H$_2$-H$_2$ potential…

化学物理 · 物理学 2015-06-03 Renat A. Sultanov , Dennis Guster , S. K. Adhikari

In collisions at ultralow temperatures, molecules will possess Feshbach resonances, foreign to ultracold atoms, whose virtual excited states consist of rotations of the molecules. We estimate the mean spacing and mean widths of these…

原子物理 · 物理学 2009-11-07 J. L. Bohn , A. V. Avdeenkov , M. P. Deskevich

A previously developed approach for the numerical treatment of two particles that are confined in a finite optical-lattice potential and interact via an arbitrary isotropic interaction potential has been extended to incorporate an…

量子气体 · 物理学 2014-12-10 Bruno Schulz , Simon Sala , Alejandro Saenz

We report a unique feature of magnetic field Feshbach resonances in which atoms collide with non-zero orbital angular momentum. P-wave ($l=1$) Feshbach resonances are split into two components depending on the magnitude of the resonant…

原子物理 · 物理学 2009-11-10 C. Ticknor , C. A. Regal , D. S. Jin , J. L. Bohn

Anisotropy is a fundamental property of particle interactions. It occupies a central role in cold and ultra-cold molecular processes, where long range forces have been found to significantly depend on orientation in ultra-cold polar…

Quantum scattering calculations are reported for the H+HCl(v,j=0) and H+DCl(v,j=0) collisions for vibrational levels v=0-2 of the diatoms. Calculations were performed for incident kinetic energies in the range 10-7 to 10-1 eV, for total…

化学物理 · 物理学 2009-11-10 P. F. Weck , N. Balakrishnan

We investigate the effect of temperature on resonant and antiresonant dynamics in a dilute atomic gas kicked periodically by a standing wave laser field. Our numerical calculations are based on a Monte Carlo method for an incoherent mixture…

原子物理 · 物理学 2008-07-17 M. Saunders , P. L. Halkyard , K. J. Challis , S. A. Gardiner

Ammonia is one of the most widely observed molecules in space, and many observations are able to resolve the hyperfine structure due to the electric quadrupole moment of the nitrogen nucleus. The observed spectra often display anomalies in…

星系天体物理 · 物理学 2023-09-06 J. Loreau , A. Faure , F. Lique , S. Demes , P. J. Dagdigian

We have observed and located more than 60 magnetic field-induced Feshbach resonances in ultracold collisions of ground-state $^{133}$Cs atoms. These resonances are associated with molecular states with up to four units of rotational angular…

软凝聚态物质 · 物理学 2007-05-23 Cheng Chin , Vladan Vuletic , Andrew J. Kerman , Steven Chu , Eite Tiesinga , Paul J. Leo , Carl J. Williams

New quantum scattering calculations for rotational deexcitation transitions of CO induced by H collisions using two CO-H potential energy surfaces (PESs) from Shepler et al. (2007) are reported. State-to-state rate coefficients are computed…

太阳与恒星天体物理 · 物理学 2015-06-15 Benhui Yang , P. C. Stancil , N. Balakrishnan , R. C. Forrey , J. M. Bowman

We calculate the interaction potential between N atoms and NH molecules and use it to investigate cold and ultracold collisions important for sympathetic cooling. The ratio of elastic to inelastic cross sections is large over a wide range…

化学物理 · 物理学 2011-02-23 Piotr S. Żuchowski , Jeremy M. Hutson

We consider the magnetically tunable Feshbach resonances that may exist in ultracold mixtures of molecules in $^2\Sigma$ states and alkali-metal atoms. We focus on Rb+CaF as a prototype system. There are likely to be Feshbach resonances…

原子物理 · 物理学 2023-06-05 Robert C. Bird , Michael R. Tarbutt , Jeremy M. Hutson

A (diatomic) shape resonance is a metastable state of a pair of colliding atoms quasi-bound by the centrifugal barrier imposed by the angular momentum involved in the collision. The temporary trapping of the atoms' scattering wavefunction…

Shape resonances in H$_2$, produced as reaction intermediates in the photolysis of H$_2$S precursor molecules, are measured in a half-collision approach. Before desintegrating into two ground state H atoms, the reaction is quenched by…

原子物理 · 物理学 2021-11-10 K. -F. Lai , E. J. Salumbides , W. Ubachs , M. Beyer

Two different ab initio potential energy surfaces are employed to investigate the efficiency of the rotational excitation channels for the polar molecular ion HeH$^+$ interacting with He atoms. We further use them to investigate the quantum…

Stereodynamics of cold collisions has become a fertile ground for quantized studies of molecular collisions and control of the collision outcome. A benchmark process for stereodynamic control is rotational transition in He+HD collisions.…

化学物理 · 物理学 2020-09-04 Masato Morita , Naduvalath Balakrishnan
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