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A new light responsive arylazopyrazole (AAP) containing polymer matrix thin film is fabricated by spin-coating of different concentrations of the AAP azo dye into the polydimethylsiloxane (PDMS) polymer at 150C. The new AAP molecular switch…

Responsive foams and interfaces, are interesting for active materials that respond to external stimuli. We have used the photochromic reaction of a spiropyran surfactant to render interfacial, rising bubble as well as foaming properties…

Binding and phase behavior of oppositely charged polyelectrolytes and surfactants were studied in aqueous bulk solutions and at air-water interfaces. In particular, we have investigated the polyanion poly(sodium 4-styrenesulfonate) (NaPSS)…

软凝聚态物质 · 物理学 2020-07-16 Felix Schulze-Zachau , Björn Braunschweig

We use molecular dynamics simulations to study the thermodynamics and kinetics of alanine dipeptide isomerization at the air-water interface. Thermodynamically, we find an affinity of the dipeptide to the interface. This affinity arises…

统计力学 · 物理学 2022-01-10 Aditya N. Singh , David T. Limmer

Per- and polyfluoroalkyl substances are a class of synthetic chemical compounds widely used as coatings to lower surface energies. Yet the microscopic mechanisms of their weak interaction with water and organic compounds remain poorly…

化学物理 · 物理学 2026-04-06 Maximilian R. Becker , Ruben Cruz , Kenichi Ataka , Joachim Heberle , Roland R. Netz

This study of adsorption of normal alkanols at the oil/water interface with x-ray reflectivity and tensiometry demonstrates that the liquid to gas monolayer phase transition at the hexane/water interface is thermodynamically favorable only…

软凝聚态物质 · 物理学 2009-11-13 Aleksey M. Tikhonov , Mark L. Schlossman

The air-water interface is a highly prevalent phase boundary with a far-reaching impact on natural and industrial processes. Water molecules behave differently at the interface compared to the bulk, exhibiting anisotropic orientational…

The effect of increasing temperature on the structural stability and interactions of two kinds of Al/Zr (Al(1%wtSi)/Zr and Al(Pure)/Zr) multilayer mirrors are investigated. All Al/Zr multilayers annealed from 200^{\circ}C to 500^{\circ}C,…

材料科学 · 物理学 2015-06-11 Qi Zhong , Shuang Ma , Zhong Zhang , Runze Qi , Jia Li , Zhanshan Wang , Philippe Jonnard

The unique structural properties of interfacial water are at the heart of a vast range of important processes in electrochemistry, climate science, and biophysics. At interfaces, water molecules exhibit preferential orientations and an…

Herein, we present a series of isomerically pure, peripherically alkyl substituted, soluble and low aggregating azaphthalocyanines as well as their new, smaller hybrid homologues, the azasubphthalocyanines. The focus lies on the effect of…

Systematic exploration of amorphous ABC heterostructures revealed that nanoscale morphological modifications markedly improved their artificial bulk second-order susceptibility. These amorphous birefringent heterostructures were fabricated…

On-surface synthesis has paved the way towards the fabrication and characterization of conjugated carbon-based molecular materials that exhibit {\pi}-magnetism such as triangulenes. Aza-triangulene, a nitrogen-substituted derivative, was…

Transparent conducting oxides have recently gained great attention as CMOS-compatible materials for applications in nanophotonics due to their low optical loss, metal-like behavior, versatile/tailorable optical properties, and established…

光学 · 物理学 2015-07-27 N. Kinsey , C. DeVault , J. Kim , M. Ferrera , V. M. Shalaev , A. Boltasseva

Environmental oxidation has a great impact in tuning the physical, chemical and electronic properties of two-dimensional (2D) monolayers which can affect their practical applications in nanoscale engineering devices under ambient…

材料科学 · 物理学 2025-11-18 Soumendra Kumar Das , Prasanjit Samal , Brahmananda Chakraborty , Sridhar Sahu

Amino-silane-based surface passivation schemes are gaining attention in halide perovskite optoelectronics, with varying levels of success. We compare surface treatments using (3-aminopropyl)trimethoxysilane (APTMS) and…

材料科学 · 物理学 2025-09-05 Zixu Huang , Farhad Akrami , Junxiang Zhang , Stephen Barlow , Seth R. Marder , David S. Ginger

Entanglement control of qubits in a photoisomerizing molecule is studied in the context of an NMR quantum computer by taking azobenzene as an example. Azobenzene has two different isomers, {\it{}trans}-azobenzene (TAB) and…

量子物理 · 物理学 2010-04-07 Taiga Yasuda , Masahito Tada-Umezaki , Mikio Nakahara , Tomonari Wakabayashi

A systematic study of the electronic structure and optical properties of the thio-apatites Ba$_5$(VS$_{\alpha}$O$_{\beta}$)$_3$X (X= Cl, F, Br, I) is carried out through first principles density functional theory simulations. The band gap…

材料科学 · 物理学 2025-07-14 Smritijit Sen , Houria Kabbour

The adsorption of anions from aqueous solution on the air/water interface controls important heterogeneous chemistry in the atmosphere and is thought to have similar physics to anion adsorption at hydrophobic interfaces more generally.…

化学物理 · 物理学 2018-05-09 Yujin Tong , Igor Ying Zhang , R. Kramer Campen

Virtually all organic (opto)electronic devices rely on organic/inorganic interfaces with specific properties. These properties are, in turn, inextricably linked to the interface structure. Therefore, a change in structure can introduce a…

材料科学 · 物理学 2022-04-21 Lukas Hörmann , Andreas Jeindl , Oliver T. Hofmann

High entropy oxides (HEO) hold the potential to revolutionize the conventional material paradigms by leveraging high order of chemical disorder that induces highly desirable exotic phases for advanced applications. Here, we devise a…

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