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Understanding the intricate relation between illumination and temperature in metallic nano-particles is crucial for elucidating the role of illumination in various physical processes which rely on plasmonic enhancement but are also…

化学物理 · 物理学 2023-03-31 Ieng-Wai Un , Yonatan Dubi , Yonatan Sivan

Recent experiments claimed that the enhancement of catalytic reaction rates occurs via the reduction of activation barriers driven by non-equilibrium (``hot'') electrons in plasmonic metal nanoparticles. These experiments place plasmonic…

化学物理 · 物理学 2020-04-22 Yonatan Sivan , Ieng Wai Un , Yonatan Dubi

Light absorption and scattering of plasmonic metal nanoparticles can lead to non-equilibrium charge carriers, intense electromagnetic near-fields, and heat generation, with promising applications in a vast range of fields, from chemical and…

光学 · 物理学 2020-08-27 Guillaume Baffou , Ivan Bordacchini , Andrea Baldi , Romain Quidant

It has been known for many years that metallic nanoparticles can catalyse various chemical reactions, both in the dark and under illumination, through different mechanisms. In the last decade or so, many claims of plasmon-assisted "hot"…

光学 · 物理学 2020-11-13 Yonatan Sivan , Yonatan Dubi

Plasmonic absorption of light can lead to significant local heating in metallic nanostructures, an effect that defines the sub-field of thermoplasmonics and has been leveraged in diverse applications from biomedical technology to…

介观与纳米尺度物理 · 物理学 2014-02-21 Joseph B. Herzog , Mark W. Knight , Douglas Natelson

Several chemical reactions catalyzed by plasmonic nanoparticles show enhanced rates under visible-light-excitation of the localized surface plasmon resonance of the nanoparticles. But it has been argued that there is an associated…

化学物理 · 物理学 2019-10-11 Prashant K. Jain

Multilayered metal-dielectric nanostructures display both strong plasmonic behavior and hyperbolic optical dispersion. The latter is responsible for the appearance of two separated radiative and non-radiative channels in the extinction…

The pulsed photothermal phenomenon due to optically absorbed energy, result from non-radiative decay mechanisms, which in nature, these imply the temporal change in the local free energy and thus a temporary change in the local temperature.…

介观与纳米尺度物理 · 物理学 2019-04-04 M. Rodríguez-Matus , C. Garcia-Segundo , Jean-Parick Connerade

Thermal relaxation of nanoscale magnetic islands, mimicking Ising macrospins, is indispensable for studies of geometrically frustrated artificial spin systems and low-energy nanomagnetic computation. Currently-used heating schemes based on…

介观与纳米尺度物理 · 物理学 2019-04-24 Matteo Pancaldi , Naëmi Leo , Paolo Vavassori

Understanding the interplay between illumination and the electron distribution in metallic nanostructures is a crucial step towards developing applications such as plasmonic photo-catalysis for green fuels, nano-scale photo-detection and…

光学 · 物理学 2019-07-23 Yonatan Dubi , Yonatan Sivan

The effect of the electron temperature on both the light absorption and the scattering by metal nanoparticles (MNs) with excitation of the surface plasmon electron vibrations is studied in the framework of the kinetic theory. The formulae…

介观与纳米尺度物理 · 物理学 2013-11-25 N. I. Grigorchuk

In numerous applications of energy harvesting via transformation of light into heat the focus recently shifted towards highly absorptive materials featuring nanoplasmons. It is currently established that noble metals-based absorptive…

光学 · 物理学 2013-01-22 Gustav Edman Jonsson , Vladimir Miljkovic , Alexandre Dmitriev

While the thermal and electromagnetic properties of plasmonic nanostructures are well understood, nanoscale thermometry still presents an experimental and theoretical challenge. Plasmonic structures can confine electromagnetic energy at the…

Current thermometry techniques lack the spatial resolution required to see the temperature gradients in typical, highly-scaled modern transistors. As a step toward addressing this problem, we have measured the temperature dependence of the…

介观与纳米尺度物理 · 物理学 2018-01-17 Matthew Mecklenburg , Brian Zutter , B. C. Regan

The excitation of plasmonic nanoparticles by ultrashort laser pulses sets in motion a complex ultrafast relaxation process involving the gradual re-equilibration of the system's electron gas, lattice and environment. One of the major…

Controlling the temperature in architectures involving nanoparticles and substrates is a key issue for applications involving micro and nanoscale heat transfer. We study the thermal behavior of a single nanoparticle interacting with a flat…

光学 · 物理学 2017-03-03 Houssem Kallel , Rémi Carminati , Karl Joulain

In this paper we use layer potentials and asymptotic analysis techniques to analyze the heat generation due to nanoparticles when illuminated at their plasmonic resonance. We consider arbitrary-shaped particles and both single and multiple…

偏微分方程分析 · 数学 2017-03-02 Habib Ammari , Francisco Romero , Matias Ruiz

Plasmonic nanoparticles (NPs) hold tremendous promise for catalyzing light-driven chemical reactions. The conventionally assumed detrimental absorption loss from plasmon damping can now be harvested to drive chemical transformations of the…

Plasmonic structures are renowned for their capability to efficiently convert light into heat at the nanoscale. However, despite the possibility to generate deep sub-wavelength electromagnetic hot spots, the formation of extremely localized…

Over the last few decades, extensive previous studies of the nonlinear response of metal nanoparticles report a wide variation of nonlinear coefficients, thus, revealing a highly confused picture of the underlying physics. This naturally…

光学 · 物理学 2020-10-28 Ieng Wai Un , Yoatan Sivan
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