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Free electron beams such as those employed in electron microscopes have evolved into powerful tools to investigate photonic nanostructures with an unrivaled combination of spatial and spectral precision through the analysis of electron…

量子物理 · 物理学 2021-04-22 F. Javier García de Abajo , Valerio Di Giulio

This review discusses how low-energy, valence excitations created by swift electrons can render information on the optical response of structured materials with unmatched spatial resolution. Electron microscopes are capable of focusing…

材料科学 · 物理学 2012-11-13 F. J. Garcia de Abajo

This paper describes a method for the explicit reconstruction and visualization of various polarization ellipses from the intensities measured after a rotating polarizer. The state of polarization of a light beam is represented by the…

光学 · 物理学 2022-11-29 Ramonika Sengupta , Brijesh Tripathi , Asha Adhiya

High energy electron beams can now be routinely focused to 1-2 {\AA} and offer the ability to obtain vibrational information from materials using monochromated electron energy-loss spectroscopy (EELS) in a scanning transmission electron…

材料科学 · 物理学 2021-07-13 Kartik Venkatraman , Peter A. Crozier

We study the origin of the structure in the spin-polarized electron energy loss spectroscopy (SPEELS) spectra of ferromagnetic crystals. Our study is based on a 3d tight-binding Fe model, with constant onsite Coulomb repulsion U between…

材料科学 · 物理学 2009-10-31 R. Saniz , S. P. Apell

Orientation dependent electronic properties of wurtzite zinc oxide nanorods are characterized by aloof beam electron energy-loss spectroscopy (EELS) carried out in a scanning transmission electron microscope (STEM). The two key crystal…

材料科学 · 物理学 2021-10-06 Yao-Wen Yeh , Sobhit Singh , David Vanderbilt , Philip E. Batson

Progress in electron-beam spectroscopies has recently enabled the study of optical excitations with combined space, energy and time resolution in the nanometer, millielectronvolt and femtosecond domain, thus providing unique access into…

光学 · 物理学 2019-11-13 Albert Polman , Mathieu Kociak , F. Javier García de Abajo

We study strongly confined plasmons in ultrathin gold and silver films by simulating electron energy-loss spectroscopy (EELS). Plasmon dispersion relations are directly retrieved from the energy- and momentum-resolved loss probability under…

Spatially resolved electron energy-loss spectroscopy (EELS) in a scanning transmission electron microscope (STEM) has been used to investigate as fluidic phase in nanoubbles embedded in a metallic Pd90Pt10 matrix. Using the 1s->2p…

材料科学 · 物理学 2016-08-14 D. Taverna , M. Kociak , O. Stéphan , A. Fabre , E. Finot , B. Décamps , C. Colliex

Inelastic scattering of electrons incident on a solid surface is determined by the two properties: (i) electronic response of the target system and (ii) the detailed quantum-mechanical motion of the projectile electron inside and in the…

材料科学 · 物理学 2016-01-06 V. U. Nazarov , V. M. Silkin , E. E. Krasovskii

The study of electronic transitions within a molecule connected to the absorption or emission of light is a common task in the process of the design of new materials. The transitions are complex quantum mechanical processes and a detailed…

In the presence of a (time-dependent) macroscopic electric field the electron dynamics of dielectrics cannot be described by the time-dependent density only. We present a real-time formalism that has the density and the macroscopic…

材料科学 · 物理学 2016-07-27 M. Grüning , D. Sangalli , C. Attaccalite

In previous work a different and powerful, analytical, technique was used to get data, such as the absolute atom concentration (AAC), specimen thickness etc., from public domain boron nitride EELS spectrum collected under a collection…

材料科学 · 物理学 2020-09-24 Noureddine Hadji

A procedure is developed to rigorously decompose experimental loss spectra of medium-energy electrons reflected from solid surfaces into contributions due to surface and volume electronic excitations. This can be achieved by analysis of two…

材料科学 · 物理学 2009-11-11 Wolfgang S. M. Werner

Intensity noise cross-correlation of the polarization eigenstates of light emerging from an atomic vapor cell in the Hanle configuration allows one to perform high resolution spectroscopy with free- running semiconductor lasers. Such an…

原子物理 · 物理学 2018-06-06 Ben Whitenack , Devan Tormey , Michael Crescimanno , Andrew C. Funk , Shannon OLeary

Laser-assisted electron scattering (LAES), a light-matter interaction process that facilitates energy transfer between strong light fields and free electrons, has so far been observed only in gas phase. Here we report on the observation of…

Recent developments in experiments with vibrational electron energy loss spectroscopy (EELS) have revealed spectral shape variations at spatial resolutions down to sub-atomic scale. Interpretation in terms of local phonon density of states…

材料科学 · 物理学 2021-09-15 Paul M. Zeiger , Ján Rusz

Here, we demonstrate the radiative polarization of high-energy electron beams in collisions with ultrashort pulsed bi-chromatic laser fields. Employing a Boltzmann kinetic approach for the electron distribution allows us to simulate the…

等离子体物理 · 物理学 2019-12-06 Daniel Seipt , Dario Del Sorbo , Christopher P. Ridgers , Alec G. R. Thomas

Van der Waals (vdW) materials exhibit intriguing structural, electronic and photonic properties. Electron Energy Loss Spectroscopy (EELS) within Scanning Transmission Electron Microscope (STEM) allows for nanoscale mapping of such…

Recent SO(3)-equivariant models embedded a molecule as a set of single atoms fixed in the three-dimensional space, which is analogous to a ball-and-stick view. This perspective provides a concise view of atom arrangements, however, the…

化学物理 · 物理学 2025-08-26 Bumju Kwak , Jeonghee Jo