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相关论文: Plasmonic Purcell Effect in Organic Molecules

200 篇论文

We study theoretically the quantum optical properties of hybrid molecules composed of an individual quantum dot and a metallic nanoparticle. We calculate the resonance fluorescence of this hybrid system. Its incoherent part, the one arising…

量子物理 · 物理学 2010-04-12 A. Ridolfo , O. Di Stefano , N. Fina , R. Saija , S. Savasta

We theoretically demonstrate the strong Purcell effect in $\varepsilon$-near-zero ultra-anisotropic uniaxial metamaterials with elliptic isofrequency surface. Contrary to the hyperbolic metamaterials, the effect does not rely on the…

光学 · 物理学 2015-06-11 A. V. Chebykin , A. A. Orlov , A. S. Shalin , A. N. Poddubny , P. A. Belov

Plasmonic nanocavities enable the confinement of molecules and electromagnetic fields within nano-metric volumes. As a consequence, the molecules experience a remarkably strong interaction with the electromagnetic field, to such an extent…

The Purcell effect is usually described as a modification of the spontaneous decay rate in the presence of a resonator. In plasmonics, this effect is commonly associated with a large local-field enhancement in "hot spots" due to the…

With recent experiments investigating the optical properties of progressively smaller plasmonic particles, quantum effects become increasingly more relevant, requiring a microscopic description. Using the density matrix formalism we analyze…

介观与纳米尺度物理 · 物理学 2018-10-17 Alexandra Crai , Andreas Pusch , Doris E. Reiter , Lara Román Castellanos , Tilmann Kuhn , Ortwin Hess

Coherent electronic transport through individual molecules is crucially sensitive to quantum interference. Using exact diagonalization techniques, we investigate the zero-bias and zero-temperature conductance through $\pi$-conjugated…

强关联电子 · 物理学 2015-05-14 Julian Rincon , K. Hallberg , S. Ramasesha

The spontaneous emission rate of dipole emitters close to plasmonic dimers are theoretically studied within a nonlocal hydrodynamic model. A nonlocal model has to be used since quantum emitters in the immediate environment of a metallic…

The nonlinear optical dynamics of nano-materials comprised of plasmons interacting with quantum emitters is investigated by a self-consistent model based on the coupled Maxwell-Liouville-von Neumann equations. It is shown that ultra-short…

介观与纳米尺度物理 · 物理学 2013-12-04 Maxim Sukharev , Tamar Seideman , Robert J. Gordon , Adi Salomon , Yehiam Prior

We investigate the quantum optical properties of a single photon emitter coupled to a finite-size metal nanoparticle using a photon Green function technique that rigorously quantizes the electromagnetic fields. We first obtain pronounced…

介观与纳米尺度物理 · 物理学 2012-02-07 C. Van Vlack , Philip Trøst Kristensen , S. Hughes

The optical properties of hybrid molecules composed of semiconductor and metal nanoparticles with a weak probe in a strong pump field are investigated theoretically. Excitons in such a hybrid molecule demonstrate novel optical properties…

介观与纳米尺度物理 · 物理学 2008-03-18 Zhien Lu , Ka-di Zhu

In this thesis we propose new, versatile schemes to control light-matter interactions at the nanoscale. In the first part of the thesis, we envisage a new class of plasmonic cloaks made of magneto-optical (MO) materials. We demonstrate that…

光学 · 物理学 2015-05-12 W. J. M. Kort-Kamp

We calculate the quantum state of the plasmon field excited by an ensemble of molecular emitters, which are driven by exchange of electrons with metallic nano-particle electrodes. Assuming identical emitters that are coupled collectively to…

光学 · 物理学 2016-07-20 Yuan Zhang , Klaus Mølmer , Volkhard May

We consider a hybrid plasmon-exciton system comprised of a resonant molecular subsystem and three Au wires supporting a dipole mode which can be coupled to a dark mode in controllable fashion by variation of a symmetry parameter. The…

光学 · 物理学 2015-03-25 Maxim Sukharev , Paul N. Day , Ruth Pachter

We use an improved version of the standard effective mass approximation model to describe quantum effects in nanometric semiconductor Quantum Dots (QDs). This allows analytic computation of relevant quantities to a very large extent. We…

材料科学 · 物理学 2011-06-21 Baptiste Billaud , T. T. Truong

We consider metamolecule consisting of bosonic mode correlated with the two-level system: it can be, for example, plasmonic mode interacting with the quantum dot. We focus on the parameter range where all the correlations are strong and of…

介观与纳米尺度物理 · 物理学 2015-07-27 E. S. Andrianov , N. M. Chtchelkatchev , A. A. Pukhov

We investigate the conditions yielding plasmon-exciton strong coupling at the single emitter level in the gap between two metal nanoparticles. A quasi-analytical transformation optics approach is developed that makes possible a thorough…

介观与纳米尺度物理 · 物理学 2016-09-07 Rui-Qi Li , D. Hernangómez-Pérez , F. J. García-Vidal , A. I. Fernández-Domínguez

Purcell effect predicts that spontaneous radiation is not an intrinsic property of matter, but is affected by the environment in which it is located, and is the result of the interaction of matter and field. Purcell effect can be inferred…

核理论 · 物理学 2021-04-08 Fei He , Ka-Di Zhu

For almost two decades, it has been believed that the quantum statistical properties of bosons are preserved in plasmonic systems. This idea has been stimulated by experimental work reporting the possibility of preserving nonclassical…

During the long course of evolution, nature has learnt how to exploit quantum effects. In fact, recent experiments reveal the existence of quantum processes whose coherence extends over unexpectedly long time and space ranges. In…

量子物理 · 物理学 2015-07-14 G. L. Giorgi , M. Roncaglia , F. A. Raffa , M. Genovese

The interpretation of the electronic kinetic processes in the quantum zero dimensional nanostructures is considered. The main mechanism of the processes is supposed to be the interaction of electrons with the optical phonons. An emphasis is…

介观与纳米尺度物理 · 物理学 2012-01-05 K. Kral , M. Mensik