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Recent techniques have allowed transition metal dichalcogenides (TMD) monolayers to be grown and adequately characterised. Of particular interest, their nonlinear optical response presents many promising opportunities for future…

介观与纳米尺度物理 · 物理学 2020-03-06 David N. Carvalho , Fabio Biancalana

Monolayer transition metal dichalcogenide semiconductors, with versatile experimentally accessible exciton species, offer an interesting platform for investigating the interaction between excitons and a Fermi sea of charges. Using hexagonal…

介观与纳米尺度物理 · 物理学 2020-08-18 Thomas Goldstein , Yueh-Chun Wu , Shao-Yu Chen , Takashi Taniguchi , Kenji Watanabe , Kalman Varga , Jun Yan

Exciton effects on conjugated polymers and the resulting optical nonlinearities are investigated in soliton lattice systems. The magnitude of the THG at the 10 percent doping increases by the factor about 10^2 from that of the neutral…

凝聚态物理 · 物理学 2016-08-31 Kikuo Harigaya

Integrating two-dimensional van der Waals materials with optical cavities has revealed a fascinating platform to study exciton-polariton physics. Manipulating exciton polaritons often requires external control over the electrical and…

光学 · 物理学 2023-11-08 Zhi Wang , Li He , Bumho Kim , Bo Zhen

A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

We study a 2D system of trion-polaritons at the quantum level and demonstrate that for monolayer semiconductors they can exhibit a strongly nonlinear optical response. The effect is due to the composite nature of trion-based excitations…

量子物理 · 物理学 2020-11-11 O. Kyriienko , D. N. Krizhanovskii , I. A. Shelykh

Monolayer transition metal dichalcogenides (TMDs) are direct gap semiconductors emerging promising applications in diverse optoelectronic devices. To improve performance, recent investigations have been systematically focused on the tuning…

Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that…

介观与纳米尺度物理 · 物理学 2022-03-02 Valentin Walther , Lida Zhang , Susanne F. Yelin , Thomas Pohl

Excitons in monolayer transition-metal dichalcogenides (TMDs) have garnered significant attention because of their large binding energies due to weakly screened Coulomb interaction, and direct bandgap at the K/K$^\prime$ point in the…

Strong coupling between light and matter in an optical cavity provides a pathway to giant polariton nonlinearity, where effective polariton-polariton interactions are mediated by materials' nonlinear responses. The pursuit of such enhanced…

光学 · 物理学 2024-11-26 Zhi Wang , Li He , Bumho Kim , Bo Zhen

Atomically thin materials such as graphene and monolayer transition metal dichalcogenides (TMDs) exhibit remarkable physical properties resulting from their reduced dimensionality and crystal symmetry. The family of semiconducting…

Atomically thin crystals of transition metal dichalcogenides (TMDs) host excitons with strong binding energies and sizable light-matter interactions. Coupled to optical cavities, monolayer TMDs routinely reach the regime of strong…

Just as photons are the quanta of light, plasmons are the quanta of orchestrated charge-density oscillations in conducting media. Plasmon phenomena in normal metals, superconductors and doped semiconductors are often driven by…

材料科学 · 物理学 2017-11-22 Dinh Van Tuan , Benedikt Scharf , Igor Žutić , Hanan Dery

Nonlinear light sources are central to a myriad of applications, driving a quest for their miniaturisation down to the nanoscale. In this quest, nonlinear metasurfaces hold a great promise, as they enhance nonlinear effects through their…

Excitons in monolayer transition metal dichalcogenide (TMD) provide a paradigm of composite Boson in 2D system. This letter reports a photoluminescence and reflectance study of excitons in monolayer molybdenum diselenide (MoSe2) with…

介观与纳米尺度物理 · 物理学 2020-08-26 Ke Xiao , Tengfei Yan , Qiye Liu , Siyuan Yang , Chiming Kan , Ruihuan Duan , Zheng Liu , Xiaodong Cui

We propose an analytical approach for calculating the linear and nonlinear optical (NLO) responses of monolayer transition metal dichalcogenides (TMDs) including excitonic effects. An effective Hamiltonian reproducing the trigonal warping…

介观与纳米尺度物理 · 物理学 2019-07-03 Alireza Taghizadeh , T. G. Pedersen

Recently reported large values of exciton-polariton nonlinearity of transition metal dichalcogenide (TMD) monolayers coupled to optically resonant structures approach the values characteristic for GaAs-based systems in the regime of strong…

介观与纳米尺度物理 · 物理学 2022-05-10 F. A. Benimetskiy , A. Yulin , A. O. Mikhin , V. Kravtsov , I. Iorsh , M. S. Skolnick , I. A. Shelykh , D. N. Krizhanovskii , A. Samusev

We demonstrate the integration of a thin BaTiO$_3$ (BTO) membrane with monolayer MoSe$_2$ in a dual gate device that enables in-situ manipulation of the BTO ferroelectric polarization with a voltage pulse. While two-dimensional (2D)…

Excitons, composite electron-hole quasiparticles, are known to play an important role in optoelectronic phenomena in many semiconducting materials. Recent experiments and theory indicate that the band-gap optics of the newly discovered…

介观与纳米尺度物理 · 物理学 2015-09-02 Yuri N. Gartstein , Xiao Li , Chuanwei Zhang

We present a proposal for achieving light-induced superconductivity using exciton polaritons - hybrid light-matter particles of excitons (bound electron-hole pairs) and microcavity photons. In contrast to previous theories of…

介观与纳米尺度物理 · 物理学 2025-08-14 Kenneth Choo , Olivier Bleu , Meera M. Parish , Jesper Levinsen