相关论文: Doppler-Free Two-Photon Cavity Ring-Down Spectrosc…
We report on the Doppler-free saturation spectroscopy of the nitrous oxide (N$_2$O) overtone transition at 1.28~$\mu$m. This measurement is performed by the noise-immune cavity-enhanced optical heterodyne molecular spectroscopy (NICE-OHMS)…
This paper presents an analysis of near-resonant, ro-vibrational two-photon spectroscopy and the use of cavity ring-down spectroscopy for its detection. Expressions are derived for the photon absorption rate of a three-level system, correct…
Weak transitions in the (2,0) overtone band of the HD molecule at $\lambda = 1.38 \, \mu$m were measured in saturated absorption using the technique of noise-immune cavity-enhanced optical heterodyne molecular spectroscopy. Narrow…
Using a mid-infrared quantum cascade laser and wavelength modulation absorption spectroscopy, we measure the frequencies of ro-vibrational transitions of N$_2$O in the 17 $\mu$m region with uncertainties below 5 MHz. These lines,…
Frequency-stabilized mid-infrared lasers are valuable tools for precision molecular spectroscopy. However, their implementation remains limited by complicated stabilization schemes. Here we achieve optical self-locking of a quantum cascade…
We report on a comb-locked cavity ring-down spectrometer developed for high-precision molecular spectroscopy at 2 ${\mu}$m. It is based on the use of an external-cavity diode laser that is offset-frequency locked to the signal output of a…
In this paper, we describe two complementary non-linear spectroscopy methods which both allow to achieve Doppler-free spectra of atomic gases. First, saturated absorption spectroscopy is used to investigate the structure of the $5{\rm…
The saturated absorption spectrum of the hyperfine-less S(0) quadrupole line in the (2-0) band of H$_2$ is measured at $\lambda=1189$ nm, using the NICE-OHMS technique under cryogenic conditions (72~K). It is for the first time that a Lamb…
We report precision measurement of aluminum atoms ${^{2}P_{1/2}}-{^{2}S_{1/2}}$ transition at 394 nm and ${^{2}P_{3/2}}-{^{2}S_{1/2}}$ transition at 396 nm in a hollow-cathode lamp (HCL). Both absorption spectroscopy and saturated…
Two-photon excitation in the near-infrared (NIR) of colloidal nanocrystalline silicon quantum dots (nc-SiQDs) with photoluminescence also in the NIR has the potential to open up new opportunities in the field of deep biological imaging.…
The $\lambda$ = 2.06 $\mu$m absorption band of CO$_2$ is widely used for the remote sensing of atmospheric carbon dioxide, making it relevant to many important top-down measurements of carbon flux. The forward models used in the retrieval…
The features of Doppler-free resonances detected by probing the $^{133}$Cs atom $6S_{1/2}-7P_{3/2}$ transition at 456 nm in a nanometric-thick vapor layer are investigated. The matrix element of this transition is about 11 times smaller…
In this paper, two-photon absorption resonance has been investigated . We studied this phenomenon in three-level system with common upper level, two lower long-life levels and two quasi-resonant laser fields with different frequency…
Using an Electrically Focus Tunable Lens (EFTL), an integrating sphere and a tunable femtosecond-pulse laser (Mai Tai HP), we were able to measure the degenerate two-photon absorption coefficient (in transmission) of CdS and ZnSe in a long…
We present a reliable, narrow linewidth (100 kHz) continuous-wave optical parametric oscillator (OPO) suitable for high-resolution spectroscopy applications. The OPO is based on a periodically-poled lithium-niobate crystal and features a…
The parity-allowed two-photon transitions between the ground state 3A2(T2) of the configuration 3d8 in cubical symmetry and the excited states of the same configuration are obtained via a simple model. This model is developed in a symmetry…
We report observation of the $\rm 5S_{1/2} \rightarrow 5D_{5/2}$ two-photon transition in Rb vapor at 778 nm, using an external cavity diode laser system and a heated vapor cell. The spectra in the two isotopes show well-resolved hyperfine…
We report on Doppler-free continuous-wave optical UV-spectroscopy resolving the hyperfine structure of the $\mathrm{A}\,^2\Sigma^+ \leftarrow \mathrm{X}\,^2\Pi_{3/2}$ transition in nitric oxide for total angular momenta $J_X=1.5-19.5$ on…
Vapour cell spectroscopy is an essential technique in many fields; in particular, nearly all atom and ion trapping experiments rely on simultaneous spectroscopy of two atomic transitions, traditionally employing separate apparatus for each…
A combination of optical feedback self-locking of a continuous-wave distributed feedback diode laser to a V-shaped high finesse cavity, laser phase modulation at a frequency equal to the free spectral range of the V-cavity and detection of…