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Non-equilibrium transport properties and energy conversion performance of a molecular photo-voltaic cell are analyzed using the Lindblad master equation within the open quantum systems approach. The method allows us to calculate the…

介观与纳米尺度物理 · 物理学 2015-04-09 Shigeru Ajisaka , Bojan Zunkovic , Yonatan Dubi

Transport of excitons through transfer networks is a unique example where the interplay between quantum coherence and environment-induced dephasing leads to non-trivial effects. One exciting example is the "environment-assisted quantum…

生物物理 · 物理学 2020-05-12 Elinor Zerah-Harush , Yonatan Dubi

Understanding how the effectiveness of natural photosynthetic energy harvesting systems arises from the interplay between quantum coherence and environmental noise represents a significant challenge for quantum theory. Recently it has begun…

生物物理 · 物理学 2015-06-16 E. K. Irish , R. Gómez-Bombarelli , B. W. Lovett

Transport phenomena at the nanoscale are of interest due to the presence of both quantum and classical behavior. In this work, we demonstrate that quantum transport efficiency can be enhanced by a dynamical interplay of the system…

量子物理 · 物理学 2009-05-22 Patrick Rebentrost , Masoud Mohseni , Ivan Kassal , Seth Lloyd , Alán Aspuru-Guzik

Decoherence is mostly detrimental in quantum information and quantum optics applications. However, the interplay between environment-induced incoherent dynamics and unitary evolution can give rise to novel quantum many-body phenomena that…

量子物理 · 物理学 2026-05-28 Eric Sánchez-Llorente , Helmut Ritsch , Maria Moreno-Cardoner

Electron capture by {\it isolated} atoms and ions proceeds by photorecombination. In this process a species captures a free electron by emitting a photon which carries away the excess energy. It is shown here that in the presence of an {\it…

量子物理 · 物理学 2010-03-18 Kirill Gokhberg , Lorenz S. Cederbaum

Transport phenomena are fundamental in Physics. They allow for information and energy to be exchanged between individual constituents of communication systems, networks or even biological entities. Environmental noise will generally hinder…

量子物理 · 物理学 2009-11-13 M. B. Plenio , S. F. Huelga

Electron-hole pairs in organic photovoltaics dissociate efficiently despite their Coulomb-binding energy exceeding thermal energy at room temperature. The electronic states involved in charge separation couple to structured vibrational…

介观与纳米尺度物理 · 物理学 2023-08-15 Alejandro D. Somoza , Nicola Lorenzoni , James Lim , Susana F. Huelga , Martin B. Plenio

Light-harvesting via the transport and trapping of optically-induced electronic excitations is of fundamental interest to the design of new energy efficient quantum technologies. Using a paradigmatic quantum optical model, we study the…

量子物理 · 物理学 2024-08-08 Jonah S. Peter , Raphael Holzinger , Stefan Ostermann , Susanne F. Yelin

The investigation of the phenomenon of dephasing assisted quantum transport, which happens when the presence of dephasing benefits the efficiency of this process, has been mainly focused on Markovian scenarios associated with constant and…

量子物理 · 物理学 2022-01-27 Saulo V. Moreira , Breno Marques , Fernando L. Semião

Single-molecule electronics has been envisioned as the ultimate goal in the miniaturisation of electronic circuits. While the aim of incorporating single-molecule junctions into modern technology still proves elusive, recent developments in…

介观与纳米尺度物理 · 物理学 2017-11-22 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

The soft character of organic materials leads to strong coupling between molecular nuclear and electronic dynamics. This coupling opens the way to control charge transport in organic electronic devices by inducing molecular vibrational…

Energy transfer within photosynthetic systems can display quantum effects such as delocalized excitonic transport. Recently, direct evidence of long-lived coherence has been experimentally demonstrated for the dynamics of the…

量子物理 · 物理学 2008-12-06 Masoud Mohseni , Patrick Rebentrost , Seth Lloyd , Alán Aspuru-Guzik

We present a theoretical analysis of the efficiency and rate of excitation transport on a network described by a complete graph in which every site is connected to every other. The long-time transport properties are analytically calculated…

量子物理 · 物理学 2025-07-16 Sam Alterman , Justin Berman , Frederick W. Strauch

The efficiencies of light-harvesting complexes in biological systems can be much higher than the current efficiencies of artificial solar cells. In this paper, we therefore propose and analyse an energy transport mechanism which employs…

化学物理 · 物理学 2020-03-11 Arend G. Dijkstra , Almut Beige

Enhanced interaction between two two-level emitters (e.g., atoms) by nonreciprocal photonic media can be of benefit to broad areas, from quantum information science to biological detection. Here we provide a detailed analysis on why…

量子物理 · 物理学 2022-09-14 S. Ali Hassani Gangaraj , Lei Ying , Francesco Monticone , Zongfu Yu

Effect of a complicated many-body environment is analyzed on the electron random scattering by a 2D mesoscopic open ballistic structure. A new mechanism of decoherence is proposed. The temperature of the environment is supposed to be zero…

介观与纳米尺度物理 · 物理学 2015-03-13 Valentin V. Sokolov

The conversion of an absorbed photon from the exciton energy into the reaction centre in the photosynthetic complex has a near unit efficiency. It is becoming clear that any classical model, where the exciton hopping is modeled by a…

量子物理 · 物理学 2010-06-21 Vlatko Vedral , Tristan Farrow

Noise-assisted transport in quantum systems occurs when quantum time-evolution and decoherence conspire to produce a transport efficiency that is higher than what would be seen in either the purely quantum or purely classical cases. In…

量子物理 · 物理学 2012-08-30 Ivan Kassal , Alán Aspuru-Guzik

Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…

量子物理 · 物理学 2015-02-12 Arend G. Dijkstra , Chen Wang , Jianshu Cao , Graham R. Fleming
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