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Chromium triiodide is an intrinsically magnetic van der Waals material down to the single-layer limit. Here, we provide a first-principles description of finite-temperature magnetic and spectral properties of monolayer (ML) CrI$_3$ based on…

Van der Waals materials have become a promising building block for future electronics and photonics. The two-dimensional magnet CrSBr came into the spotlight of solid state research due to its intriguing combination of antiferromagnetic…

Stable excitons in semiconductor monolayers such as transition-metal dichalcogenides (TMDCs) enable and motivate fundamental research as well as the development of room-temperature optoelectronics applications. The newly discovered layered…

材料科学 · 物理学 2021-03-17 Magdalena Birowska , Paulo E. Faria Junior , Jaroslav Fabian , Jens Kunstmann

Van der Waals heterostructures (vdWHs) composed of transition-metal dichalcogenides (TMDs) and layered magnetic semiconductors offer great opportunities to manipulate exciton and valley properties of TMDs. Here, we present…

The recent experimental discovery of intrinsic ferromagnetism in single-layer CrI3 opens a new avenue to low-dimensional spintronics. However, the low Curie temperature Tc=45 K is still a large obstacle to its realistic device application.…

材料科学 · 物理学 2019-06-26 Hongxing Li , Yuan-Kai Xu , Kang Lai , Wei-Bing Zhang

We study a capacitor made of three monolayers of transition metal dichalcogenide (TMD) separated by hexagonal Boron Nitride (hBN). We assume that the structure is symmetric with respect to the central layer plane. The symmetry includes the…

介观与纳米尺度物理 · 物理学 2019-04-10 M. Sammon , B. I. Shklovskii

We theoretically examined how the dielectric screening of two-dimensional layered materials affects the dipolar interaction between interlayer excitons in few-layer van der Waals structures. Our analysis indicates that the dipolar…

介观与纳米尺度物理 · 物理学 2024-02-14 Yuhang Hou , Hongyi Yu

Using a combination of density functional theory (DFT) and spin-wave theory methods, we investigate the magnetic interactions and spin excitations in semiconducting VI$_3$. Exchange parameters of monolayer, bilayer, and bulk forms are…

材料科学 · 物理学 2021-09-24 Elijah Gordon , V. V. Mkhitaryan , Haijun Zhao , Y. Lee , Liqin Ke

The optics of dangling-bond-free van der Waals heterostructures containing transition metal dichalcogenides are dominated by excitons. A crucial property of a confined exciton is the quantum confined Stark effect (QCSE). Here, such a…

The discovery of atomically thin two-dimensional (2D) magnetic semiconductors has triggered enormous research interest recently. In this work, we use first-principles many-body perturbation theory to study a prototypical 2D ferromagnetic…

材料科学 · 物理学 2022-02-01 Meng Wu , Zhenglu Li , Steven G. Louie

Van der Waals materials such as thin films of transition-metal dichalcogenides (TMDCs) manifest strongly bound exciton states in the visible spectrum at ambient conditions that provide an ideal platform for exciton-photon couplings.…

光学 · 物理学 2025-07-15 Fatemeh Davoodi , Nahid Talebi

Magnetic proximity effects are crucial ingredients for engineering spintronic, superconducting, and topological phenomena in heterostructures. Such effects are highly sensitive to the interfacial electronic properties, such as electron wave…

Correlated quantum phenomena in one-dimensional (1D) systems that exhibit competing electronic and magnetic order are of strong interest for studying fundamental interactions and excitations, such as Tomonaga-Luttinger liquids and…

The discovery of local-moment magnetism in van der Waals (vdW) semiconductors down to the single-layer limit has led to a paradigm shift in the understanding of two-dimensional (2D) magnets and unleashed their potential for applications in…

Metal monochalcogenide GaSe is a classic layered semiconductor that has received increasing research interest due to its highly tunable electronic and optical properties for ultrathin electronics applications. Despite intense research…

材料科学 · 物理学 2024-05-14 Fanhao Jia , Zhao Tang , Greis J. Cruz , Weiwei Gao , Shaowen Xu , Wei Ren , Peihong Zhang

The van der Waals magnets CrX$_3$ (X = I, Br, and Cl) exhibit highly tunable magnetic properties and are promising candidates for developing novel two-dimensional (2D) magnetic devices such as magnetic tunnel junctions and spin tunneling…

介观与纳米尺度物理 · 物理学 2022-12-06 Jia Wang , Zahra Ahmadi , David Lujan , Jeongheon Choe , Takashi Taniguchi , Kenji Watanabe , Xiaoqin Li , Jeffrey E. Shield , Xia Hong

Chromium tri-halides Cr$X_3$ ($X$ = Cl, Br, and I) have recently become a focal point of research due to their intriguing low-temperature,layer-dependent magnetism that can be manipulated by an electric field. This makes them essential…

Since the celebrated discovery of graphene, the family of two-dimensional (2D) materials has grown to encompass a broad range of electronic properties. Recent additions include spin-valley coupled semiconductors, Ising superconductors that…

The discovery of spontaneous magnetism in van der Waal (vdW) magnetic monolayers has opened up an unprecedented platform for investigating magnetism in purely two-dimensional systems. Recently, it has been shown that the magnetic properties…

介观与纳米尺度物理 · 物理学 2022-01-19 Eliot Heinrich , Xin Li , Benedetta Flebus

The magnetic properties in two-dimensional van der Waals materials depend sensitively on structure. CrI3, as an example, has been recently demonstrated to exhibit distinct magnetic properties depending on the layer thickness and stacking…