相关论文: The Shape of the Electric Dipole Function Determin…

Surprisingly large spontaneous electric dipole moments recently observed in homonuclear niobium clusters below 100 K (Moro el. al. Science 300, 1265 (2003)) are explained using first-principles electronic structure calculations. The…

We propose a q-deformed model of the anharmonic vibrations in diatomic molecules. We analyse the applicability of the model to the phenomenological Dunham's expansion by comparing with experimental data. Our methodology involves a global…

The dynamics of charge carriers in lattices of quantum spins is a long standing and fundamental problem. Recently, a new generation of quantum simulation experiments based on atoms in optical lattices has emerged that gives unprecedented…

Multipole moments are the first order responses of the energy to spatial derivatives of the electric field strength. The quality of density functional theory (DFT) prediction of molecular multipole moments thus characterizes errors in…

Here we present different approaches to ultrafast pulse and polarization shaping, based on a ``quantum fluid'' platform of polaritons. Indeed we exploit the normal modes of two dimensional polariton fluids made of strong coupled quantum…

We report Brownian dynamics (BD) simulation and theoretical results for a system of spherical colloidal particles with permanent dipole moments in a rotating magnetic field. Performing simulations at a fixed packing fraction and dipole…

We have perfomed Time Dependant Hartree-Fock (TDHF) calculations on the non linear response of nuclei. We have shown that quadrupole (and dipole) motion produces monopole (and quadrupole) oscillations in all atomic nuclei. We have shown…

We study quantum droplets emerging in a quasi-one-dimensional asymmetric mixture of two atomic species with different intra-component coupling constants. We find that such mixtures support a rich variety of multipole quantum droplets, where…

Recent experiments on trilayer transition-metal dichalcogenide heterostructures have revealed the rich behavior of dipolar excitons. Motivated by these experimental observations, we investigate the collective dynamics of planar quantum…

The vibrational motion equations of both homo and hetero-nuclei diatomic molecules are here derived for the first time. A diatomic molecule is first considered as a one dimensional quantum mechanics oscillator. The second and third-order…

We show that the electric dipole-dipole interaction between a pair of polar molecules undergoes an all-out transformation when superimposed by a far-off resonant optical field. The combined interaction potential becomes tunable by variation…

Microcavity polaritons are bosonic light-matter particles that can emit coherent radiation without electronic population inversion via bosonic scattering. This phenomenon, known as polariton lasing, strongly depends on the polaritons'…

We investigate the depletion of single-electron states in small molecules under the influence of very short XUV pulses. In N$_2$, for a certain window of XUV energies around 50 eV, we observe a marked occupation inversion, i.e. a situation…

Molecular hydrogen normally has only weak, quadrupole transitions between its rovibrational states, but in a static electric field it acquires a dipole moment and a set of allowed transitions. Here we use published ab initio calculations of…

We study collective excitations of rotational and spin states of an ensemble of polar molecules, which are prepared in a dipolar crystalline phase, as a candidate for a high fidelity quantum memory. While dipolar crystals are formed in the…

The molecular Hubbard Hamiltonian (MHH) naturally arises for ultracold ground state polar alkali dimer molecules in optical lattices. We show that, unlike ultracold atoms, different molecules display different many-body phases due to…

We assess the cavity molecular dynamics method for the calculation of vibrational polariton spectra, using liquid water as a specific example. We begin by disputing a recent suggestion that nuclear quantum effects may lead to a broadening…

We report the properties of a novel type of sub-proton scale magnetic hole found in two dimensional PIC simulations of decaying turbulence with a guide field. The simulations were performed with a realistic value for ion to electron mass…

The strengths and short-comings of the point-dipole model for polar fluids of spherical molecules are illustrated by considering the physically more relevant case of extended dipoles formed by two opposite charges $\pm q$ separated by a…

The Dicke-Ising model describes cavity quantum electrodynamics setups in which dipoles couple not only with the photonic cavity field but also to each other through dipole-dipole interaction. In this work we diagonalise such a model in…