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Using first-principles density-functional theory calculations, we predict the potential for unprecedented thermoelectric efficiency $zT=5$ at 800 K in $n$-type Ba$_{2}$BiAu full-Heusler compound. Such a high efficiency arises from an…

材料科学 · 物理学 2019-02-06 Junsoo Park , Yi Xia , Vidvuds Ozoliņš

The potential of Fe2TiSn full-Heusler compounds for thermoelectric applications has been suggested theoretically, but not yet grounded experimentally, due to the difficulty of obtaining reproducible, homogeneous, phase pure and defect free…

Heusler compounds have emerged as important thermoelectric materials due to their combination of promising electronic transport properties, mechanical robustness and chemical stability -- key aspects for practical device integration. While…

The thermoelectric properties of 54 different group 4 half-Heusler (HH) alloys have been studied from first principles. Electronic transport was studied with density functional theory using hybrid functionals facilitated by the $\mathbf{k}…

材料科学 · 物理学 2020-01-08 Kristian Berland , Nina Shulumba , Olle Hellman , Clas Persson , Ole Martin Løvvik

In this first-principles study, we investigated the thermoelectric properties of the full-Heusler compound CsK$_2$Sb at different compressive strains. This material exhibits a valence band structure with significant effective mass…

材料科学 · 物理学 2025-05-14 Øven A. Grimenes , G. Jeffrey Snyder , Ole M. Løvvik , Kristian Berland

Heusler compounds with six valence electrons per atom have attracted interest as thermoelectric materials owing to their semimetallic and semiconducting properties. Here, we theoretically and experimentally investigate electronic transport…

材料科学 · 物理学 2024-12-10 Fabian Garmroudi , Michael Parzer , Takao Mori , Andrej Pustogow , Ernst Bauer

The electronic and thermoelectric (TE) transport properties of 13 n-type and p-type half-Heusler alloys are computationally examined using Boltzmann transport. The electronic scattering times resulting from all relevant phonon interactions…

We perform an ab initio computational investigation of the electronic and thermoelectric transport properties of one of the best performance half-Heusler (HH) alloys, NbFeSb. We use Boltzmann Transport equation while taking into account the…

材料科学 · 物理学 2025-10-28 Bhawna Sahni , Yao Zhao , Zhen Li , Rajeev Dutt , Patrizio Graziosi , Neophytos Neophytou

Materials with reduced dimensionality offer beneficial density-of-states (DOS) profiles for thermoelectric energy conversion, but can be impractical in realistic devices. Encouragingly, bulk high-symmetry materials can also exhibit similar…

材料科学 · 物理学 2026-03-10 Øven A. Grimenes , Ole M. Løvvik , Kristian Berland

Heusler type compounds have long been recognized as potential thermoelectric (TE) materials. Here, the experimentally observed TE properties of Fe$_{2}$VAl are understood through electronic structure calculations in the temperature range of…

材料科学 · 物理学 2022-04-20 Shamim Sk , P. Devi , Sanjay Singh , Sudhir K. Pandey

Structural, electronic, and transport properties of ScNiSb, ScPdSb, and ScPtSb were investigated from first principles. Electronic band structures derived within the fully relativistic MBJLDA approach were compared with those obtained from…

材料科学 · 物理学 2018-06-05 Maciej J. Winiarski , Kaja Bilinska , Kamil Ciesielski , Dariusz Kaczorowski

By using ab initio electronic structure calculations here we report the three new full Heusler alloys which are possessing very good thermoelectric behavior and expected to be synthesized in the laboratories. These are Fe2 ScP, Fe2 ScAs and…

材料科学 · 物理学 2015-06-22 Sonu Sharma , Sudhir K. Pandey

The half-Heusler (hH) compounds are currently considered promising thermoelectric (TE) materials due to their favorable thermopower and electrical conductivity. Accurate estimates of these properties are therefore highly desirable and…

材料科学 · 物理学 2026-04-07 Vinod Kumar Solet , Sudhir K. Pandey

The electronic structure and thermoelectric properties of ZrRuTe-based Half-Heusler compounds are studied using density functional theory (DFT) and Boltzmann transport formalism. Based on rigorous computations of electron relaxation time…

材料科学 · 物理学 2020-03-13 Sonu Prasad Keshri , Amal Medhi

The Heusler compound ScInAu$_2$ was previously reported to have a superconducting ground state with a critical temperature of 3.0 K. Recent high throughput calculations have also predicted that the material harbors a topologically…

Half Heusler (HH) thermoelectric alloys provide a wide platform to choose materials with non-toxic and earth abundant elements. This article presents an ab-initio theoretical evaluation of electrical and thermal transport properties of…

材料科学 · 物理学 2016-10-21 Vikram , Jiban Kangsabanik , Enamullah , Aftab Alam

Semiconducting half- and, to a lesser extent, full-Heusler compounds are promising thermoelectric materials due to their compelling electronic properties with large power factors. However, intrinsically high thermal conductivity resulting…

In the quest of new thermoelectric (TE) materials with high power factors, full-Heusler compounds having flat band are found to be promising candidates. In this direction, Fe$_{2}$ScX (X=P,As,Sb) compounds are investigated using mBJ for the…

强关联电子 · 物理学 2019-12-30 Shivprasad S. Shastri , Sudhir K. Pandey

The ScAu$_2$Al superconducting Heusler-type compound was recently characterized to have the highest critical temperature of $T_c = 5.12$ K and the strongest electron-phonon coupling among the Heusler family. In this work, the electronic…

超导电性 · 物理学 2023-12-04 Gabriel Kuderowicz , Bartlomiej Wiendlocha

Half Heusler (HH) alloys with 18 valence electron count have attracted significant interest in the area of research related to thermoelectrics. Understanding the novel transport properties exhibited by these systems with semiconducting…

材料科学 · 物理学 2022-02-15 Kavita Yadav , Saurabh Singh , Tsunehiro Takeuchi , K. Mukherjee
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