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Exciton-photon hybridization is typically realised in geometrically defined optical cavities, where tunability is achieved by modifying either the cavity or the excitonic medium. Here we investigate transition-radiation interferences in…

We study experimentally and theoretically the exciton-phonon interaction in MoSe2 monolayers encapsulated in hexagonal BN, which has an important impact on both optical absorption and emission processes. The exciton transition linewidth…

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

The optical responses of semiconducting transition metal dichalcogenides are dominated by excitons. Being able to strongly interact with light and other materials excitations, excitons in semiconductors are prototypes for investigating…

介观与纳米尺度物理 · 物理学 2021-01-28 Xuke Jiang , Masoud Taleb , Florian Diekmann , Kai Rossnagel , Nahid Talebi

The concept of \textit{optical} exciton - a photo-excited bound electron-hole pair within a crystal - is routinely used to interpret and model a wealth of excited-state phenomena in semiconductors. Beside originating sub-band gap signatures…

材料科学 · 物理学 2022-09-21 Fulvio Paleari , Andrea Marini

Exciton-polaritons - coherently hybridized states of excitons and photons - are instrumental for solid-state nonlinear optics and quantum simulations. To enable engineered polariton energy landscapes and interactions, local control over the…

The common model to describe exciton-plasmon interaction phenomenologically is the coupled oscillator model. Originally developed for atomic systems rather than solid-state matter, this model treats both excitons and plasmons as single…

介观与纳米尺度物理 · 物理学 2024-10-23 Lara Greten , Robert Salzwedel , Diana Schutsch , Andreas Knorr

Phonon interactions in solid-state photonics systems cause intrinsic quantum decoherence and often present the limiting factor in emerging quantum technology. Due to recent developments in nanophotonics, exciton-cavity structures with very…

量子物理 · 物理学 2021-01-04 Emil V. Denning , Matias Bundgaard-Nielsen , Jesper Mork

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

材料科学 · 物理学 2022-02-17 Gabriel Antonius , Steven G. Louie

Recent experiments have demonstrated strong light-matter coupling between electromagnetic nanoresonators and pristine sheets of two-dimensional semiconductors, and it has been speculated whether these systems can enter the quantum regime…

量子物理 · 物理学 2022-02-23 E. V. Denning , M. Wubs , N. Stenger , J. Mork , P. T. Kristensen

We study theoretically the Coulomb interaction between excitons in transition metal dichalcogenide (TMD) monolayers. We calculate direct and exchange interaction for both ground and excited states of excitons. The screening of the Coulomb…

介观与纳米尺度物理 · 物理学 2017-09-13 V. Shahnazaryan , I. Iorsh , I. A. Shelykh , O. Kyriienko

We investigate the correction of interlayer exciton binding energy in transition metal dichalcogenides double layers arising from the exciton-optical phonon coupling using the method of Lee-Low-Pines unitary transformation. We find that the…

介观与纳米尺度物理 · 物理学 2018-11-14 Zi-Wu Wang , Xi-Ying Dong , Run-Ze Li , Yao Xiao , Zhi-Qing Li

Multi-exciton correlations shape the photo-induced response of nanostructured materials, particularly when interactions are enhanced by light confinement. Here multidimensional coherent spectroscopy is used to quantify biexciton and…

介观与纳米尺度物理 · 物理学 2025-07-11 Giuseppe Fumero , Jagannath Paul , Jared K. Wahlstrand , Alan D. Bristow

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

材料科学 · 物理学 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

Due to a strong Coulomb interaction, excitons dominate the excitation kinetics in 2D materials. While Coulomb-scattering between electrons has been well studied, the interaction of excitons is more challenging and remains to be explored. As…

材料科学 · 物理学 2021-01-27 Daniel Erkensten , Samuel Brem , Ermin Malic

Embedding a monolayer of a transition metal dichalcogenide in a high-Q optical cavity results in the formation of distinct exciton polariton modes. The polaritons are affected by the strong exciton-phonon interaction in the monolayer. We…

介观与纳米尺度物理 · 物理学 2021-12-22 Frank Lengers , Tilmann Kuhn , Doris E. Reiter

Localized excitons play a vital role in the optical response of monolayers of transition metal dichalcogenides and can be exploited as single photon sources for quantum information technology. While the optical properties of such localized…

介观与纳米尺度物理 · 物理学 2020-11-04 F. Lengers , T. Kuhn , D. E. Reiter

The strong excitonic effect in monolayer transition metal dichalcogenide (TMD) semiconductors has enabled many fascinating light-matter interaction phenomena. Examples include strongly coupled exciton-polaritons and nearly perfect atomic…

介观与纳米尺度物理 · 物理学 2021-04-13 Hongchao Xie , Shengwei Jiang , Daniel A. Rhodes , James C. Hone , Jie Shan , Kin Fai Mak

Monolayer transition metal dichalcogenides feature Coulomb-bound electron-hole pairs (excitons) with exceptionally large binding energy and coupled spin and valley degrees of freedom. These unique attributes have been leveraged for…

Strong spatial confinement and highly reduced dielectric screening provide monolayer transition metal dichalcogenides (TMDCs) with strong many-body effects, thereby possessing optically forbidden excitonic states (i.e., dark excitons) at…

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