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Because of their unique and rich physical properties, transition metal dichalcogenides (TMDs) materials have attracted much interest. Many studies suggest that introducing the degree of freedom of anisotropy, which may be brought about by…

材料科学 · 物理学 2025-02-11 T. T. Lin , J. W. Ma , H. C. Deng , L. Z. Liu

Monolayer transition metal dichalcogenides (TMDs) exhibit high nonlinear optical (NLO) susceptibilities. Experiments on MoS$_2$ have indeed revealed very large second-order ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) optical…

Monolayer transition-metal dichalcogenides (TMDCs) present high second-order optical nonlinearity, which is extremely desirable for, e.g., frequency conversion in nonlinear photonic devices. On the other hand, the atomic thickness of 2D…

介观与纳米尺度物理 · 物理学 2020-11-17 Pilar G. Vianna , Aline dos S. Almeida , Rodrigo M. Gerosa , Dario A. Bahamon , Christiano J. S. de Matos

The in-plane anisotropic properties of two-dimensional (2D) group IV monochalcogenides provide an additional degree of freedom which can be used in future optoelectronic devices. Here, it is shown that the third harmonic generation (THG)…

We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologically-protected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by…

Remarkable optical and electrical properties of two-dimensional (2D) materials, such as graphene and transition-metal dichalcogenide (TMDC) monolayers, offer vast technological potential for novel and improved optoelectronic nanodevices,…

光学 · 物理学 2016-07-22 Martin Weismann , Nicolae C. Panoiu

Rigorous electrodynamical simulations based on the nonlinear Drude model are performed to investigate the influence of strong coupling on high harmonic generation by periodic metal gratings. It is shown that a thin dispersive material with…

介观与纳米尺度物理 · 物理学 2019-08-13 Elena Drobnyh , Ruth Pachter , Maxim Sukharev

Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…

光学 · 物理学 2025-08-25 Navdeep Rana , M. S. Mrudul , Amar Bharti , Sucharita Giri , Gopal Dixit

In transition metal dichalcogenides (TMDCs), charge carriers have spin, pseudospin, and valley degrees of freedom associated with magnetic moments. The monolayers and bilayers of the TMDCs, in particular, MoS$_2$, lead strong couplings…

材料科学 · 物理学 2021-11-29 Yeon Lee , Dasol Kim , Dong Eon Kim , Alexis Chacón

We study a system of a transition metal dichalcogenide (TMD) monolayer placed in an optical resonator, where strong light-matter coupling between excitons and photons is achieved. We present quantitative theory of the nonlinear optical…

介观与纳米尺度物理 · 物理学 2020-10-09 V. Shahnazaryan , V. K. Kozin , I. A. Shelykh , I. V. Iorsh , O. Kyriienko

Two-dimensional Transition-Metal Dichalcogenides (TMDs) are of great interest for second harmonic (SH) generation due to their large second-order susceptibility, atomically thin structure, and relaxed phase-matching conditions. TMDs are…

Frequency conversion processes, such as second- and third-harmonic generation, are one of the most common effects in nonlinear optics which offer many opportunities for photonics, chemistry, material science, characterization, and…

光学 · 物理学 2017-06-26 Alexander Krasnok , Mykhailo Tymchenko , Andrea Alu

Monolayer transition metal dichalcogenides, coupled to metal plasmonic nanocavities, have recently emerged as new platforms for strong light-matter interactions. These systems are expected to have nonlinear optical properties that will…

We report observation of strong and anisotropic third harmonic generation (THG) in monolayer and multilayer ReS$_2$. The third-order nonlinear optical susceptibility of monolayer ReS$_2$, $\left| \chi^{(3)} \right|$ is on the order of…

材料科学 · 物理学 2017-04-12 Qiannan Cui , Rodrigo A. Muniz , J. E. Sipe , Hui Zhao

Providing quantitative interpretation of coherent nonlinear microscopy images, such as third-harmonic generation (THG), is generally hampered by the complex phase-matching conditions, especially in the presence of sample linear…

光学 · 物理学 2026-03-09 Mohammad Reza Farhadinia , Nicolas Olivier

In this paper we explore the capabilities of MoS2 and WS2 2D monolayers to produce radiation in the terahertz range by generation of high-order harmonics. This phenomenon, which is a result of the non-linear response of the electronic…

应用物理 · 物理学 2024-02-13 Jose Manuel Iglesias , Elena Pascual , Maria J. Martin , Raul Rengel

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

光学 · 物理学 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

Resonant structures in modern nanophotonics are non-Hermitian (leaky and lossy), and support quasinormal modes. Moreover, contemporary cavities frequently include 2D materials to exploit and resonantly enhance their nonlinear properties or…

计算物理 · 物理学 2023-01-25 Thomas Christopoulos , Emmanouil E. Kriezis , Odysseas Tsilipakos

We experimentally explore the fingerprint of the microscopic electron dynamics in second-order harmonic generation (SHG). It is shown that the interbond electron hopping induces a novel source of nonlinear polarization and plays an…

We theoretically investigate detuning-dependent properties of high-order harmonic generation (HHG) in monolayer transition metal dichalcogenides (TMDCs). In contrast to HHG in conventional materials, TMDCs show both parallel and…

材料科学 · 物理学 2018-04-18 Tomohiro Tamaya , Satoru Konabe , Shiro Kawabata
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