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Frontiers of attosecond science are constantly shifting, thus addressing more and more intricate effects with increasing resolution. Ultrashort pulses offer a practical way to prepare complex superpositions of quantum states, follow, and…

量子物理 · 物理学 2019-05-16 Huihui Wang , Tobias Möhle , Oliver Kühn , Sergey I. Bokarev

Recent developments in attosecond spectroscopy yield access to the correlated motion of electrons on their intrinsic time scales. Spin-flip dynamics is usually considered in the context of valence electronic states, where spin-orbit…

原子与分子团簇 · 物理学 2017-08-02 H. Wang , S. I. Bokarev , S. G. Aziz , O. Kühn

Understanding the nature of magnetic interactions in ultra-small magnetic ensembles and their intrinsic properties is vital to uncover the dynamics therein. In this study we reveal the spin dynamics of hexagonally arranged Fe atoms on…

介观与纳米尺度物理 · 物理学 2018-08-21 Tamene R. Dasa , Valeri S. Stepanyuk

Recent advances in attosecond physics provide access to the correlated motion of valence and core electrons on their intrinsic timescales. For valence excitations, processes related to the electron spin are usually driven by nuclear motion.…

化学物理 · 物理学 2017-01-18 Huihui Wang , Sergey I. Bokarev , Saadullah G. Aziz , O. Kühn

Laser radiation incident on a ferromagnetic sample produces excited electrons and currents whose spin polarization must not be aligned with the magnetization -- an effect due to spin-orbit coupling that is ubiquitous in spin- and…

材料科学 · 物理学 2023-11-03 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

Induced by an ultra-short laser pulse, the electronic structure of a material undergoes strong modifications leading to a fast demagnetization in magnetic materials. Induced spin-flip transitions are one of the reasons for demagnetization,…

材料科学 · 物理学 2024-04-29 Sergiy Mankovsky , Svitlana Polesya , Hubert Ebert

Recent experimental advances in ultrafast science put different processes occurring on the electronic timescale below a few femtoseconds in focus. In the present theoretical work, we demonstrate how the transformation and propagation of the…

计算物理 · 物理学 2023-06-13 Thies Romig , Vladislav Kochetov , Sergey I. Bokarev

Different energy shifts for majority and minority electrons occur. Thus, for example in case of (laser) excited ferromagnetic metals majority and minority electrons may respond differently in time during closing the exchange splitting. Spin…

介观与纳米尺度物理 · 物理学 2013-05-27 M. Avignon , K. H. Bennemann

Transition-metal oxides have been a central subject of condensed matter physics for decades. In addition to novel electronic states driven by the influence of strong correlation, relativistic spin-orbit coupling effects have recently…

材料科学 · 物理学 2025-05-22 Satoshi Okamoto , Narayan Mohanta , Ho Nyung Lee , Adriana Moreo , Elbio Dagotto

Transition-metal phthalocyanine molecules have attracted considerable interest in the context of spintronics device development due to their amenability to diverse bonding regimes and their intrinsic magnetism. The latter is highly…

强关联电子 · 物理学 2024-12-19 Sumanta Bhandary , Emiliano Poli , Gilberto Teobaldi , David D. O'Regan

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

材料科学 · 物理学 2010-07-06 Adrian Glaubitz

The spin dynamics of a hydrogen atom during the passage of a periodic magnetic structure is discussed. The occupation numbers of the components of the hyperfine structure are considered as a function of time. The characteristic…

原子物理 · 物理学 2020-05-13 A. I. Milstein , Yu. V. Shestakov , D. K. Toporkov

It is well known that non-central nuclear forces, such as the spin-orbital coupling and the tensor force, play important roles in understanding many interesting features of nuclear structures. However, their dynamical effects in nuclear…

核理论 · 物理学 2015-11-17 Jun Xu , Bao-An Li , Wen-Qing Shen , Yin Xia

The mechanism behind fast intersystem crossing in transition-metal complexes is shown to be a result of the dephasing of the photoexcited state to the phonon continuum of a different state with a significantly different transition…

强关联电子 · 物理学 2010-02-11 Michel van Veenendaal , Jun Chang , A. J. Fedro

Spin injection across interfaces driven by ultrashort optical pulses on femtosecond timescales constitutes a new way to design spintronics applications. Targeted utilization of this phenomenon requires knowledge of the efficiency of…

材料科学 · 物理学 2022-12-29 P. Elliott , A. Eschenlohr , J. Chen , S. Shallcross , U. Bovensiepen , J. K. Dewhurst , S. Sharma

The spin dynamics in Ni is studied by an exact diagonalization method on the ultrafast time scale. It is shown that the femtosecond relaxation of the magneto-optical response results from exchange interaction and spin-orbit coupling. Each…

材料科学 · 物理学 2009-10-30 W. Hubner , G. P. Zhang

Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

强关联电子 · 物理学 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

A joint theoretical and experimental investigation is performed to understand the underlying physics of laser-induced demagnetization in Ni and Co films. Experimentally dynamics of spins is studied by determining the time-dependent…

Ultrafast magnetization dynamics probes the most fundamental properties of magnetic materials, exploring questions about the fundamental interactions responsible for magnetic phenomena. Thermal effects are known to be extremely important…

材料科学 · 物理学 2019-08-26 Daniel Meilak , Sarah Jenkins , Rory Pond , Richard F. L. Evans

We present an ab initio method for eletcronic structure calculations, which accounts for the interaction of electrons and magnons in ferromagnets. While it is based on a many body perturbation theory we approximate numerically complex…

材料科学 · 物理学 2023-04-19 S. Paischer , G. Vignale , M. I. Katsnelson , A. Ernst , P. Buczek
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