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Utilization of triplet excitons, which generally emit poorly, is always fundamental to realize highly efficient organic light-emitting diodes (LEDs). While triplet harvest and energy transfer via electron exchange between triplet donor and…

Two-dimensional halide perovskites host strongly bound excitons whose fine structure controls polarization selection rules and radiative recombination, yet several spectral features in (PEA)$_2$PbI$_4$ remain controversially assigned. Here,…

介观与纳米尺度物理 · 物理学 2026-04-22 Patrick Grenzer , Fabian Lie , Klaus H. Eckstein , Tobias Hertel , Linn Leppert

Halide perovskite materials raised tremendous interest in recent years since their cheap fabrication, superior performance in both solar cell and light emitting diode (LED). Due to the existence of layered quantum well structure, quasi…

材料科学 · 物理学 2021-11-23 Wei Tang , Liting Tao , Tian Zhang , Yanjun Fang , Deren Yang , Linjun Li

Hybrid organic-inorganic semiconductors feature complex lattice dynamics due to the ionic character of the crystal and the softness arising from non-covalent bonds between molecular moieties and the inorganic network. Here we establish that…

A theoretical model for excitons confined in layered metal halide perovskites is presented. The model accounts for polaronic effects, dielectric and quantum confinement by means of effective mass theory, image charges and Haken potentials.…

介观与纳米尺度物理 · 物理学 2023-08-08 Jose L. Movilla , Josep Planelles , Juan I. Climente

The family of hybrid organic-inorganic lead-halide perovskites are the subject of intense interest for optoelectronic applications, from light-emitting diodes to photovoltaics to X-ray detectors. Due to the inert nature of most organic…

Understanding how dielectric anisotropy governs excitonic behavior in two-dimensional (2D) halide perovskites is critical for predicting and engineering their optoelectronic properties. In this work, we investigate Cs(n+1)PbnBr3n+1…

The bound electron-hole pairs known as excitons govern the optical properties of insulating solids. While their behavior in equilibrium is well-understood theoretically, the nonequilibrium regime at high excitation densities-where phenomena…

介观与纳米尺度物理 · 物理学 2025-10-31 Pushpendra Yadav

Exciton transport in molecular aggregates with magic-angle orientation is expected to be strongly suppressed due to their negligible dipole-dipole interactions. However, recent reports show that light-matter interactions can significantly…

化学物理 · 物理学 2026-03-10 Siwei Wang , Liang-Yan Hsu , Hsing-Ta Chen

The great variety of lead halide perovskite semiconductors represents an outstanding platform for studying crystal symmetry effects on the spin-dependent properties. Access to them is granted through optical orientation of exciton and…

Tightly bound excitons in monolayer semiconductors represent a versatile platform to study two-dimensional propagation of neutral quasiparticles. Their intrinsic properties, however, can be severely obscured by spatial energy fluctuations…

The nature of trions and their interaction with light has remained a puzzle. The composition and dispersion of polaritons involving trions provide insights into this puzzle. Trions and excitons in doped two-dimensional (2D) materials are…

介观与纳米尺度物理 · 物理学 2021-07-28 Okan Koksal , Minwoo Jung , Christina Manolatou , A. Nick Vamivakas , Gennady Shvets , Farhan Rana

Excitons play an essential role in the optical response of two-dimensional materials. These are bound states showing up in the band gaps of many-body systems and are conceived as quasiparticles formed by an electron and a hole. By…

光学 · 物理学 2024-06-21 Mikhail Malakhov , Giovanni Cistaro , Fernando Martín , Antonio Picón

Topological exciton-polaritons are a burgeoning class of topological photonic systems distinguished by their hybrid nature as part-light, part-matter quasiparticles. Their further control over novel valley degree of freedom (DOF) has…

Optical nonlinearities are crucial for advanced photonic technologies since they allow photons to be managed by photons. Exciton-polaritons resulting from strong light-matter coupling are hybrid in nature: they combine small mass and high…

Atomistically detailed computational studies of nanocrystals, such as those derived from the promising lead-halide perovskites, are challenging due to the large number of atoms and lack of symmetries to exploit. Here, focusing on…

材料科学 · 物理学 2022-10-05 Giulia Biffi , Yeongsu Cho , Roman Krahne , Timothy C. Berkelbach

Exciton dissociation plays a crucial role in the performance of optoelectronic devices based on two-dimensional (2D) transition metal dichalcogenides (TMDs). In this work, we investigate the effect of an in-plane electric field on the…

材料科学 · 物理学 2024-10-11 Tao Zhu , Chenhang Zheng , Lei Xu , Ming Yang

With strongly bound and stable excitons at room temperature, single-layer, two-dimensional organic-inorganic hybrid perovskites are viable semiconductors for light-emitting quantum optoelectronics applications. In such a technological…

Excitons in two dimensional Ruddlesden Popper perovskites (RPPs) exhibit large and tunable binding energies, making them promising candidates for optoelectronic applications. In particular, long-range exciton energy transfer in these…

Two-dimensional group-VI transition metal dichalcogenide semiconductors, such as MoS2, WSe2 and others, exhibit strong light-matter coupling and possess direct band gaps in the infrared and visible spectral regimes, making them potentially…

介观与纳米尺度物理 · 物理学 2020-03-03 Thomas Mueller , Ermin Malic