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Broadband coherent anti-Stokes Raman scattering (CARS) spectroscopy plays a vital role in chemical sensing and label-free vibrational imaging, yet conventional methods suffer from limited acquisition speeds and complex detection schemes.…

光学 · 物理学 2025-07-23 Jing Hu , Tianjian Lv , Zhaoyang Wen , Wending Huang , Ming Yan , Heping Zeng

We apply coherent anti-Stokes Raman Scattering (CARS) microscopy to characterize director structures in liquid crystals.

软凝聚态物质 · 物理学 2016-09-08 A. V. Kachynski , A. N. Kuzmin , P. N. Prasad , I. I. Smalyukh

We propose a new technique for comparing two Raman active samples. The method employs optical interference of the signals generated via coherent anti-Stokes Raman scattering (CARS) of broadband laser pulses with noisy spectra. It does not…

量子物理 · 物理学 2015-05-27 Evgeny A. Shapiro , Stanislav O. Konorov , Valery Milner

We report stimulated Raman spectroscopy of the G phonon in both single and multi-layer graphene, through Coherent anti-Stokes Raman Scattering (CARS). The signal generated by the third order nonlinearity is dominated by a vibrationally…

介观与纳米尺度物理 · 物理学 2019-09-11 A. Virga , C. Ferrante , G. Batignani , D. De Fazio , A. D. G. Nunn , A. C. Ferrari , G. Cerullo , T. Scopigno

Coherent Raman scattering (CRS) spectroscopy techniques have been widely developed and optimized for different applications in biomedicine and fundamental science. The most utilized CRS technique has been coherent anti-Stokes Raman…

光学 · 物理学 2020-03-05 Pavel Kolesnichenko , Jonathan O. Tollerud , Jeffrey A. Davis

Coherent anti-Stokes Raman scattering (CARS) and, in particular, femtosecond adaptive spectroscopic techniques (FAST CARS) have been successfully used for molecular spectroscopy and microscopic imaging. Recent progress in ultrafast…

Airborne contaminants, e.g., bacterial spores, are usually analyzed by time consuming microscopic, chemical and biological assays. Current research into real time laser spectroscopic detectors of such contaminants is based on e.g. resonant…

Coherent Anti-Stokes Raman Scattering (CARS) processes are ``coherent,'' but the phase of the anti-Stokes radiation is usually lost by most incoherent spectroscopic CARS measurements. We propose a novel Raman microscopy imaging method…

光学 · 物理学 2009-11-10 D. L. Marks , S. A. Boppart

We demonstrate coherent anti-Stokes Raman scattering (CARS) microscopy in a wide-field setup with nanosecond laser pulse excitation. In contrast to confocal setups, the image of a sample can be recorded with a single pair of excitation…

光学 · 物理学 2009-11-11 Christoph Heinrich , Stefan Bernet , Monika Ritsch-Marte

Coherent Raman scattering spectroscopy is studied purposely, with the Gaussian ultrashort pulses as a hands-on elucidatory extraction tool of the clean coherent Raman resonant spectra from the overall measured data contaminated with the…

光学 · 物理学 2017-04-05 Gombojav O. Ariunbold , Narangerel Altangerel

We demonstrate a novel technique of coherent Raman spectroscopy with a femtosecond laser. We apply to a molecular sample a sequence of pairs of ultrashort excitation and probe pulses, with a linearly increasing time delay between the two…

Chemical imaging enabled by Raman processes is crucial to investigating biological and chemical samples in a label-free manner. Stimulated Raman spectroscopy (SRS) overcomes the key limitation associated with low signal levels in…

光学 · 物理学 2026-03-25 Florian M. Schweizer , Hannah Terrasa , Manish Garg

Nonlinear optical methods, such as coherent anti-Stokes Raman scattering (CARS) and stimulated Raman scattering (SRS), are able to perform label free imaging, with chemical bonds specificity. Here, we demonstrate that the use of circularly…

We have developed a coherent Raman imaging platform using broadband coherent anti-Stokes Raman scattering (BCARS) that provides an unprecedented combination of speed, sensitivity, and spectral breadth. The system utilizes a unique…

We present a theoretical investigation of coherent anti-Stokes Raman scattering (CARS) that is modulated by periodically depleting the ground state population through Rabi oscillations driven by an additional control laser. We find that…

Coherent anti-Stokes Raman scattering (CARS) microscope system was built and applied to a non-intrusive gas concentration measurement of a mixing flow in a millimeter-scale channel. Carbon dioxide and nitrogen were chosen as test fluids and…

流体动力学 · 物理学 2015-08-07 Ken Yamamoto , Yuki Yamagata , Madoka Moriya , Reiko Kuriyama , Yohei Sato

Raman spectroscopy is one of the key techniques in the study of vibrational modes and molecular structures. In Coherent Anti-Stokes Raman Scattering (CARS) spectroscopy, a molecular vibrational spectrum is resolved via the third-order…

光学 · 物理学 2010-12-02 Ori Katz , Jonathan M. Levitt , Eran Grinvald , Yaron Silberberg

We propose an all-fiber-generated dual-soliton pulses based scheme for the background-free detection of coherent anti-Stokes Raman spectroscopy under the spectral focusing mechanism. Due to the strong birefringence and high nonlinearity of…

光学 · 物理学 2016-05-30 Kun Chen , Tao Wu , Haoyun Wei , Yan Li

Coherent anti-Stokes Raman Spectroscopy (CARS) is a laser-based measurement technique widely applied across many science and engineering disciplines to perform non-intrusive gas diagnostics. CARS is often used to study combustion, where the…

机器学习 · 计算机科学 2022-05-25 Gregory J. Hunt , Cody R. Ground , Andrew D. Cutler

Far field radiation pattern under tight focusing condition is investigated in Coherent Anti-stokes Raman Scattering (CARS) microscopy both in the forward (F-CARS) and backward (E-CARS) directions. While we assume no refraction index…

光学 · 物理学 2009-11-11 D. Gachet , N. Sandeau , H. Rigneault