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Generation of ultrabroadband isolated attosecond pulses (IAPs) is essential for time-resolved applications in chemical and material sciences, as they have the potential to access the spectral water window region of chemical elements, which…

介观与纳米尺度物理 · 物理学 2022-04-20 Younes Adnani , Abdelmalek Taoutioui , Abdelkader Makhoute , Károly Tökési , Hicham Agueny

We report theoretical calculations of high-order harmonic generation (HHG) of Xe with the inclusion of multi-electron effects and macroscopic propagation of the fundamental and harmonic fields in an ionizing medium. By using the…

原子物理 · 物理学 2011-10-11 Cheng Jin , Anh-Thu Le , Carlos A. Trallero-Herrero , C. D. Lin

High-order harmonic generation (HHG) arising from the non-perturbative interaction of intense light fields with matter constitutes a well-established tabletop source of coherent extreme-ultraviolet and soft X-ray radiation, which is…

Isolated attosecond pulses (IAPs) generated by few-cycle femtosecond lasers are essential for capturing ultrafast dynamics in atoms, molecules, and solids. Nonetheless, the advancement of attosecond science critically depends on achieving…

Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to…

光学 · 物理学 2025-06-04 Zhaopin Chen , Mark Levit , Yuval Kern , Basabendra Roy , Adi Goldner , Michael Krüger

We present experimental results showing the appearance of a near-continuum in the high-order harmonic generation (HHG) spectra of atomic and molecular species as the driving laser intensity of an infrared pulse increases. Detailed…

We investigate the production of an isolated attosecond pulse~(IAP) via the phase-matching gating of high-harmonic generation by intense laser pulses. Our study is based on the integration of the propagation equation for the fundamental and…

光学 · 物理学 2023-09-12 Vasily V. Strelkov , Margarita A. Khokhlova

Isolated attosecond pulses (IAP) generated by high-order harmonic generation are valuable tools that enable dynamics to be studied on the attosecond time scale. The applicability of these IAP would be widened drastically by increasing their…

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…

The bottleneck for an attosecond science experiment is concluded to be the lack of a high-peak-power isolated attosecond pulse source. Therefore, currently, generating an intense attosecond pulse would be one of the highest priority goals.…

We present a novel approach named as pumping ionizing gating (PIG) for the generation of isolated attosecond pulses (IAPs). In this regime, a short laser is used to ionize a pre-existing gas grating, creating a fast-extending plasma…

We theoretically investigate high-order harmonic generation (HHG) and its ellipticity in gapped graphene, driven by a femtosecond short-pulse laser at various orientation angles, employing the two-band density-matrix equations within the…

原子物理 · 物理学 2025-05-21 Xinru Song , Xiaoyu Bu , Xiaohui Zhao , Rongxiang Zhang , Shang Wang , Fulong Dong

An all-optical method for directly reconstructing the spectral phase of isolated attosecond pulse (IAP) has been proposed recently [New J. Phys. 25, 083003 (2023)]. This method is based on the high-harmonic generation (HHG) streaking…

光学 · 物理学 2023-09-07 Kan Wang , Yong Fu , Baochang Li , Xiangyu Tang , Zhong Guan , Bincheng Wang , C. D. Lin , Cheng Jin

The mechanism underlying high harmonic generation (HHG) in gases has been well clarified, characterizing attosecond pulse trains (APT) in the time domain, significantly advances the synthesis of isolated attosecond pulse (IAP). However, the…

光学 · 物理学 2025-07-25 Qing-Guo Fan , Kang Lai , Wen-hao Liu , Zhi Wang , Lin-Wang Wang , Jun-Wei Luo

Attosecond pulse trains (APTs) are indispensable for probing electron dynamics at their intrinsic timescales. High harmonic generation (HHG) has long been a successful and widely used technique in producing extreme ultraviolet APTs. While…

加速器物理 · 物理学 2025-10-16 Lanpeng Ni , Junhao Liu , Zheng Qi , Chao Feng

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

原子物理 · 物理学 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…

原子物理 · 物理学 2026-04-23 Aaron T. Bondy , Klaus Bartschat

High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet…

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…

One of the main difficulties to efficiently generating high-order harmonics in long neutral-gas targets is to reach the phase-matching conditions. One issue is that the medium cannot be sufficiently ionized by the driving laser due to…

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