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Colloidal Cadmium Selenide (CdSe) nanoplatelets (NPLs) are a recently developed class of efficient luminescent nanomaterial suitable for optoelectronic device applications. A change in temperature greatly affects their electronic…

介观与纳米尺度物理 · 物理学 2017-10-26 Sumanta Bose , Sushant Shendre , Zhigang Song , Vijay Kumar Sharma , Dao Hua Zhang , Cuong Dang , Weijun Fan , Hilmi Volkan Demir

We report the synthesis and optical characterization of fully inorganic gradientshell CdSe/CdZnS nanocrystals (NCs) with high luminescence quantum yield (QY, 50 percent), which were obtained by replacing native oleic-acid (OA) ligands with…

材料科学 · 物理学 2021-11-03 Justine Baronnier , Benoit Mahler , Christophe Dujardin , Florian Kulzer , Julien Houel

We show theoretically that carriers confined in semiconductor colloidal nanoplatelets (NPLs) sense the presence of neighbor, cofacially stacked NPLs in their energy spectrum. When approaching identical NPLs, the otherwise degenerate energy…

介观与纳米尺度物理 · 物理学 2020-04-21 Jose L. Movilla , Josep Planelles , Juan I. Climente

Luminescent colloidal CdSe nanorings are a new type of semiconductor structure that have attracted interest due to the potential for unique physics arising from their non-trivial toroidal shape. However, the exciton properties and dynamics…

CdSe nanoplatelets (NPLs) are suitable for exploring strong light-matter coupling in semiconductor nanocrystal systems due to their giant oscillator strength and large exciton binding energy. Herein, we report on the facile fabrication and…

材料科学 · 物理学 2023-09-12 Masaru Oda , Kazuaki Yamato , Jyunya Egashira , Hisao Kondo

Colloidal semiconductor nanocrystals are promising building blocks for optoelectronics due to their solution processability, spectral tunability, and ability to self-assemble into complex architectures. However, their use in lasing…

Colloidal semiconductor nanocrystals are promising materials for classical and quantum light sources due to their versatile chemistry and efficient photoluminescence (PL) properties. While visible emitters are well-established, the pursuit…

Recent experiments suggest that the photoluminescence line width of CdSe and CdSe/CdS nanoplatelets (NPLs) may be broadened by the presence of shakeup (SU) lines from negatively charged trions. We carry out a theoretical analysis, based on…

材料科学 · 物理学 2020-11-02 Jordi Llusar , Juan I. Climente

Colloidal nanoplatelets (NPLs) are promising materials for lasing applications. The properties are usually discussed in the framework of 2D materials, where strong excitonic effects dominate the optical properties near the band edge. At the…

The optical properties of transition metal dichalcogenides have previously been modified at the nanoscale by using mechanical and electrical nanostructuring. However, a clear experimental picture relating the local electronic structure with…

Fluorescent semiconductor nanoplatelets (epitaxial quantum wells) can be synthesized with excellent monodispersity and self-assembled in highly-ordered structures. Modifications of their electronic and luminescence properties when stacked,…

Two-dimensional electron-hole gases in colloidal semiconductors have a wide variety of applications. Therefore, a proper physical understanding of these materials is of great importance. In this paper we present a detailed theoretical…

介观与纳米尺度物理 · 物理学 2019-12-18 F. García Flórez , Aditya Kulkarni , Laurens D. A. Siebbeles , H. T. C. Stoof

We propose and demonstrate a method for the construction of highly uniform, multilayered, orientation-controlled superstructures of CdSe/CdZnS core/shell colloidal nanoplatelets (NPLs) using bi-phase liquid interface. These atomically-flat…

Semiconductor nanoplatelets possess exceptional optical properties that make them promising candidates for next-generation optoelectronic applications. However, unlike quantum dots where absorption spectroscopy alone can determine both size…

Atomically flat semiconductor nanostructures have sharp photoluminescence emission, short radiative lifetimes and a well-defined planar structure. However, these nanostructures lack the optical and electronic fine-tuning that justify…

材料科学 · 物理学 2015-09-29 Sébastien Lamarre , Étienne Rochette , Samuel Tremblay , Claudine Nì. Allen

Near-infrared emitting colloidal two-dimensional (2D) PbX (X=S, Se) nanoplatelets have emerged as interesting materials with strong size quantisation in the thickness dimension. They act as model systems for efficient charge carrier…

Colloidal nanoplatelets - quasi-two-dimensional sheets of semiconductor exhibiting efficient, spectrally pure fluorescence - form when liquid-phase syntheses of spherical quantum dots are modified. Despite intense interest in their…

In semiconductors, quantum confinement can greatly enhance the interaction between band carriers (electrons and holes) and dopant atoms. One manifestation of this enhancement is the increased stability of exciton magnetic polarons in…

介观与纳米尺度物理 · 物理学 2017-04-27 W. D. Rice , W. Liu , V. Pinchetti , D. R. Yakovlev , V. I. Klimov , S. A. Crooker

The influence of ligands on the low frequency vibration of different thicknesses cadmium selenide colloidal nanoplatelets is investigated using resonant low frequency Raman scattering. The strong vibration frequency shifts induced by ligand…

Colloidal semiconductor nanoplatelets combine weak lateral confinement with strong Coulomb interactions, enhanced by dielectric confinement. When the platelets are charged with carriers of the same sign, this results in severe Coulomb…

介观与纳米尺度物理 · 物理学 2021-06-01 Jordi Llusar , Juan I. Climente
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