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The Yb based triangular lattice delafossites $A$Yb$X_2$ ($A$ = alkali metal, $X$ = O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe$_2$ with a perfect…

强关联电子 · 物理学 2025-09-23 Barkha Khattar , Anzar Ali , Masahiko Isobe , Yogesh Singh

We introduce the rare-earth delafossite compound TlYbSe$_2$ -- extending the search for quantum spin liquids in frustrated triangular lattice magnets. While the DC magnetisation suggests magnetic exchange interactions in the order of…

强关联电子 · 物理学 2025-09-16 Bishnu P. Belbase , Arjun Unnikrishnan , Shi Feng , Eun Sang Choi , Johannes Knolle , Arnab Banerjee

A layered triangular lattice with spin-1/2 ions is an ideal platform to explore highly entangled exotic states like quantum spin liquid (QSL). Here, we report a systematic in-field neutron scattering study on a perfect two-dimensional…

The ytterbium-based delafossite NaYbSe$_2$ is discussed as a prototype for a spin-orbit entangled, effective spin-1/2 triangular spin lattice with emerging antiferromagnetic correlations and a quantum-spin-liquid (QSL) ground state. We…

强关联电子 · 物理学 2025-01-08 S. Luther , K. M. Ranjith , Th. Doert , J. Wosnitza , H. Kühne , M. Baenitz

High-quality single crystals of NaYbSe$_2$, which resembles a perfect triangular-lattice antiferromagnet without the intrinsic disorder, are investigated by magnetization and specific heat, as well as the local probe techniques nuclear…

The triangular lattice compound TlYbS$_2$ was prepared as large single crystals via a molten flux growth technique using sodium chloride. Anisotropic magnetic susceptibility measurements down to 0.4 K indicate a complete absence of…

材料科学 · 物理学 2020-03-10 Timothy Ferreira , Jie Xing , Liurukara D. Sanjeewa , Athena S. Sefat

A triangular lattice selenide series of rare earth (RE), CsRESe2, were synthesized as large single crystals using a flux growth method. This series stabilized in either trigonal (R-3m) or hexagonal (P63/mmc) crystal systems. Physical…

The two-dimensional triangular-lattice antiferromagnet (TLAF) is a textbook example of frustrated magnetic systems. Despite its simplicity, the TLAF model exhibits a highly rich and complex magnetic phase diagram, featuring numerous…

We report neutron scattering, pressure-dependent AC calorimetry, and AC magnetic susceptibility measurements of triangular lattice NaYbSe$_2$. We observe a continuum of scattering, which is reproduced by matrix product simulations, and no…

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

强关联电子 · 物理学 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa

Spintronics has emerged as a field of vast applicability, and layered magnetic materials have served as a ground for advancement in this direction. Here, we report the synthesis and detailed magnetic and specific heat studies on NdSbSe, (a…

强关联电子 · 物理学 2025-01-22 Prabuddha Kant Mishra , Priyanka Nehla , Rishabh Shukla , Rie Umetsu , Ashok Kumar Ganguli

Antiferromagnetically coupled S=1/2 spins on an isotropic triangular lattice is the paradigm of frustrated quantum magnetism, but structurally ideal realizations are rare. Here we investigate NaYbO$_2$, which hosts an ideal triangular…

A quantum spin liquid (QSL) is a state of matter characterized by fractionalized quasiparticle excitations, quantum entanglement, and a lack of long-range magnetic order. However, QSLs have evaded definitive experimental observation.…

Square-lattice systems offer a direct route for realizing 2D quantum magnetism with frustration induced by competing interactions. In this work, the square-lattice materials YbBi2IO4 and YbBi2ClO4 were investigated using a combination of…

强关联电子 · 物理学 2024-01-26 Pyeongjae Park , G. Sala , Th. Proffen , Matthew B. Stone , Andrew D. Christianson , Andrew F. May

Three-dimensionally (3D) frustrated magnets generally exist in the magnetic diamond and pyrochlore lattices, in which quantum fluctuations suppress magnetic orders and generate highly entangled ground states (GS). LiYbSe2 in a previously…

We report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field…

强关联电子 · 物理学 2013-06-25 Y. Tokiwa , T. Radu , R. Coldea , H. Wilhelm , Z. Tylczynski , F. Steglich

Currently under active study in condensed matter physics, both theoretically and experimentally, are quantum spin liquid (QSL) states, in which no long-range magnetic ordering appears at low temperatures due to strong quantum fluctuations…

强关联电子 · 物理学 2019-07-04 Ruidan Zhong , Shu Guo , Guangyong Xu , Zhijun Xu , Robert J. Cava

Competing magnetic interactions, frustration driven quantum fluctuations, and spin correlations offer an ideal route for the experimental realization of emergent quantum phenomena and exotic quasi particle excitations in 3D frustrated…

强关联电子 · 物理学 2024-07-09 J. Khatua , Suheon Lee , Gyungbin Ban , Marc Uhlarz , Kwang-Yong Choi , P. Khuntia

Platelike high-quality NaYbS$_{2}$ rhombohedral single crystals with lateral dimensions of a few mm have been grown and investigated in great detail by bulk methods like magnetization and specific heat, but also by local probes like nuclear…

Some strongly frustrated magnets such as the "spin-ice" compounds fail to produce any magnetic order at finite temperatures even in the presence of magnetic field. Still they have very unusual low-temperature thermodynamic properties…

材料科学 · 物理学 2010-05-18 P. N. Timonin
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