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The organic conductor $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_{3}$ seems to form a quantum spin liquid, although at low temperatures unusual properties are seen in the charge, spin and lattice degrees of freedom. Here we report results of X-band…

强关联电子 · 物理学 2015-06-22 K. G. Padmalekha , M. Blankenhorn , T. Ivek , L. Bogani , J. A. Schlueter , M. Dressel

Geometrical frustration, quantum entanglement and disorder may prevent long-range order of localized spins with strong exchange interactions, resulting in a novel state of matter. $\kappa$-(BEDT-TTF)$_2$-Cu$_2$(CN)$_3$ is considered the…

The electrodynamic response of the organic spin-liquid candidate $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ has been measured in an extremely wide energy range ($10^{-13}$ to 2 eV) as a function of temperature (5 to 300 K). Below the Mott gap,…

强关联电子 · 物理学 2014-12-16 A. Pustogow , E. Zhukova , B. Gorshunov , M. Pinterić , S. Tomić , J. A. Schlueter , M. Dressel

The magnetic state of the single-component molecular compound, [Cu(tmdt)$_{2}$], is investigated by means of $^{1}$H-NMR. An abrupt spectral broadening below 13 K and a sharp peak in nuclear spin-lattice relaxation rate, $T_{1}^{-1}$, at 13…

强关联电子 · 物理学 2012-05-31 Rina Takagi , Kazuya Miyagawa , Kazushi Kanoda , Biao Zhou , Akiko Kobayashi , Hayao Kobayashi

Utilizing infrared vibrational spectroscopy we have investigated dimerized two-dimensional organic salts in order to search for possible charge redistribution that might cause electronic dipoles and ferroelectricity: the quantum spin liquid…

The spin-liquid candidate $\kappa$-(BEDT-TTF)$_{2}$Cu$_{2}$(CN)$_{3}$ has been studied by measuring the uniaxial expansion coefficients $\alpha_{i}$, the specific heat, and magnetic susceptibility. Special emphasis was placed on the…

强关联电子 · 物理学 2010-01-08 R. S. Manna , M. de Souza , A. Bruehl , J. Schlueter , M. Lang

The quasi-two-dimensional organic charge-transfer salt $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ is one of the prime candidates for a quantum spin-liquid due the strong spin frustration of its anisotropic triangular lattice in combination with…

The spin-liquid candidate $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$ [ET: bis(ethylenedithio)tetrathiafulvalene] does not exhibit magnetic ordering down to a very low temperature, but shows a mysterious anomaly at 6 K. The origin of the so-called 6 K…

强关联电子 · 物理学 2020-11-17 T. Kobayashi , Q. -P. Ding , H. Taniguchi , K. Satoh , A. Kawamoto , Y. Furukawa

We performed $^{13}$C-NMR experiment and measured spin-lattice relaxation rate divided by temperature $1/T_{1}T$ near the superconducting (SC) transition temperature $T_{c}$ in $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Br ($\kappa$-Br salt),…

超导电性 · 物理学 2015-06-19 T. Kobayashi , Y. Ihara , Y. Saito , A. Kawamoto

We investigated the local magnetism of the organic conductor, $\kappa$-(ET)$_{2}$Hg(SCN)$_{2}$Cl, with a quasi-triangular lattice of weakly dimerized molecules through $^{13}$C NMR spectroscopy. The NMR spectra and nuclear relaxation show…

强关联电子 · 物理学 2026-03-31 M. Urai , K. Miyagawa , S. A. Torunova , N. Drichko , E. I. Zhilyaeva , K. Kanoda

The two-dimensional molecular conductor $\kappa$-(BETS)$_2$Mn[N(CN)$_2$]$_3$ undergoes a sharp metal-to-insulator phase transition at $T_{\rm MI}\approx$ 21 K, which has been under scrutiny for many years. We have performed comprehensive…

强关联电子 · 物理学 2025-10-02 Marvin Schmidt , Savita Priya , Zhijie Huang , Mark Kartsovnik , Natalia Kushch , Martin Dressel

Measurements of the coefficient of thermal expansion on the spin-liquid candidate $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ have revealed distinct and strongly anisotropic lattice effects around 6 K - a possible spin-liquid instability. In…

强关联电子 · 物理学 2012-05-09 Rudra Sekhar Manna , Mariano de Souza , John A. Schlueter , Michael Lang

The nature of the magnetic ground state of highly frustrated systems remained puzzling to this day. Here, we have performed multifrequency electron spin resonance (ESR) measurements on a putative quantum spin liquid compound…

The spin excitations from the nonmagnetic charge-ordered insulating state of $\alpha$-(BEDT-TTF)$_2$I$_3$ at ambient pressure have been investigated by probing the static and low-frequency dynamic spin susceptibilities via site-selective…

强关联电子 · 物理学 2016-09-08 Kyohei Ishikawa , Michihiro Hirata , Dong Liu , Kazuya Miyagawa , Masafumi Tamura , Kazushi Kanoda

We study the role played by the magnetic frustration in the antiferromagnetic phase of the organic salt \kappa-(BEDT-TTF)_ 2 Cu [N(CN)_2] Cl. Using the spatially anisotropic triangular Heisenberg model we analyze previous and new performed…

强关联电子 · 物理学 2009-11-11 I. J. Hamad , A. E. Trumper , P. Wzietek , S. Lefebvre , L. O. Manuel

We performed angular and temperature-dependent electron-spin-resonance measurements in the quasi-two-dimensional organic conductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]I. The interlayer spin-diffusion is much weaker compared to the Cl- and…

Electron collisions for a two dimensional Fermi liquid (FL) are shown to give a quasiparticle damping with interesting frequency and temperature variations in the BCS superconducting state. The spin susceptibility which determines the…

凝聚态物理 · 物理学 2009-10-28 Shubha Tewari , John Ruvalds

Motivated by the intrinsic non-Fermi-liquid behavior observed in the heavy-fermion quasicrystal $\mbox{Au}_{51}\mbox{Al}_{34}\mbox{Yb}_{15}$, we study the low-temperature behavior of dilute magnetic impurities placed in metallic…

Recent NMR experiments by Singer et al. [Singer et al. Phys. Rev. Lett. 95, 236403 (2005).] showed a deviation from Fermi-liquid behavior in carbon nanotubes with an energy gap evident at low temperatures. Here, a comprehensive theory for…

强关联电子 · 物理学 2009-11-13 Balázs Dóra , Miklós Gulácsi , Ferenc Simon , Hans Kuzmany

The organic charge-transfer salt $\kappa$-(BEDT-TTF)$_{2}$Hg(SCN)$_{2}$Br is a quasi two-dimensional metal with a half-filled conduction band at ambient conditions. When cooled below $T=80$ K it undergoes a pronounced transition to an…

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