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Strong coupling between vibrational transitions in molecules within a resonant optical microcavity leads to the formation of collective, delocalized vibrational polaritons. There are many potential applications of "polaritonic chemistry,"…

化学物理 · 物理学 2021-11-05 Rong Duan , Joseph N. Mastron , Yin Song , Kevin J. Kubarych

The anisotropic nature of the new two-dimensional (2D) material phosphorene, in contrast to other 2D materials such as graphene and transition metal dichalcogenide (TMD) semiconductors, allows excitons to be confined in a…

Recent techniques have allowed transition metal dichalcogenides (TMD) monolayers to be grown and adequately characterised. Of particular interest, their nonlinear optical response presents many promising opportunities for future…

介观与纳米尺度物理 · 物理学 2020-03-06 David N. Carvalho , Fabio Biancalana

We present an approach for exponentially enhancing the single-photon coupling strength in an optomechanical system using only additional linear resources. It allows one to reach the quantum nonlinear regime of optomechanics, where nonlinear…

量子物理 · 物理学 2016-05-04 Marc-Antoine Lemonde , Nicolas Didier , Aashish A. Clerk

Molecular polaritons have gained considerable attention due to their potential to control nanoscale molecular processes by harnessing electromagnetic coherence. Although recent experiments with liquid-phase vibrational polaritons have shown…

Monolayer photonic materials offer a tremendous potential for on-chip optoelectronic devices. Their realization requires knowledge of optical coherence properties of excitons and trions that have so far been limited to nonlinear optical…

介观与纳米尺度物理 · 物理学 2017-12-20 Gabriella D. Shepard , Jenny V. Ardelean , Daniel A. Rhodes , X. -Y. Zhu , James C. Hone , Stefan Strauf

Transition metal dichalcogenides (TMD) monolayers, holding potential as good sunlight absorbers, are promising materials for next-generation optoelectronic devices. They may enable ultrathin photovoltaic(PV) devices thanks to their…

材料科学 · 物理学 2022-11-28 C. Attaccalite , M. S. Prete , M. Palummo , O. Pulci

Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…

材料科学 · 物理学 2024-12-05 Simone Grillo , Elena Cannuccia , Maurizia Palummo , Olivia Pulci , Claudio Attaccalite

Photonic integrated circuits with second-order ($\chi^{(2)}$) nonlinearities are rapidly scaling to remarkably low powers. At this time, state-of-the-art devices achieve saturated nonlinear interactions with thousands of photons when driven…

Deeply sub-wavelength two-dimensional films may exhibit extraordinarily strong nonlinear effects. Here we show that 2D films exhibit the remarkable property of a phase-controllable nonlinearity, i.e., the amplitude of the nonlinear…

We study solitons in one-dimensional quadratic nonlinear photonic crystals with modulation of both the linear and nonlinear susceptibilities. We derive averaged equations that include induced cubic nonlinearities and numerically find…

斑图形成与孤子 · 物理学 2009-10-31 Joel F. Corney , Ole Bang

We investigate the steady states of a lossy array of nonlinear optical resonators that are driven by lasers and interact via mutual photon tunneling. For weak nonlinearities, we find two-mode squeezing of polaritons in modes whose…

介观与纳米尺度物理 · 物理学 2015-05-14 Michael J. Hartmann

Large exciton-polariton optical nonlinearities present a key mechanism for photonics-based communication, ultimately in the quantum regime. Enhanced nonlinear response from various materials hosting excitons and allowing for their strong…

介观与纳米尺度物理 · 物理学 2024-08-05 Anna M. Grudinina , Nina S. Voronova

We develop a rigorous quantum-mechanical theory of the nonlinear optical process of difference frequency generation of surface plasmon-polaritons in Landau-quantized graphene. Although forbidden in the electric-dipole approximation, the…

介观与纳米尺度物理 · 物理学 2018-09-12 A. Ryan Kutayiah , Mikhail Tokman , Yongrui Wang , Alexey Belyanin

There are a variety of nonlinear optical effects including higher harmonic generations, photovoltaic effects, and nonlinear Kerr rotations. They are realized by the strong light irradiation to materials that results in nonlinear…

介观与纳米尺度物理 · 物理学 2016-05-26 Takahiro Morimoto , Naoto Nagaosa

Harnessing nonlinearities strong enough to allow two single photons to interact with one another is not only a fascinating challenge but is central to numerous advanced applications in quantum information science. Currently, all known…

Second-order nonlinearity in solids gives rise to a plethora of unique physical phenomena ranging from piezoelectricity and optical rectification to optical parametric amplification, spontaneous parametric down-conversion, and the…

We analyze the photon statistics of a weakly driven optomechanical system and discuss the effect of photon blockade under single photon strong coupling conditions. We present an intuitive interpretation of this effect in terms of displaced…

量子物理 · 物理学 2015-05-27 Peter Rabl

We propose a method to study the quantum nonlinearity and observe the multiphoton transitions in a multiatom CQED system. We show that by inducing simultaneously destructive quantum interference for the single-photon and two-photon…

光学 · 物理学 2015-10-28 Guoqing Yang , Wen-ju Gu , Gaoxiang Li , Bichen Zou , Yifu Zhu

Photons are ideal carriers of quantum information, as they can be easily created and can travel long distances without being affected by decoherence. For this reason, they are well suited for quantum communication. However, the interaction…

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