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As a potential candidate for quantum computation and metrology, the nitrogen vacancy (NV)center in diamond presented both challenges and opportunities resulted from charge state conversion. By utilizing different lasers for the…

量子物理 · 物理学 2014-10-20 Xiangdong Chen , Changling Zou , Zhaojun Gong , Chunhua Dong , Guangcan Guo , Fangwen Sun

Paramagnetic magnetic resonance, a powerful technique for characterizing and identifying chemical targets, is increasingly used for imaging; however, low spin polarization at room temperature and moderate magnetic fields poses challenges…

介观与纳米尺度物理 · 物理学 2019-09-04 C. M. Purser , V. P. Bhallamudi , C. S. Wolfe , H. Yusuf , B. A. McCullian , C. Jayaprakash , M. E. Flatté , P. C. Hammel

We present theoretical proposals for two-dimensional nuclear magnetic resonance spectroscopy protocols based on Nitrogen-vacancy (NV) centers in diamond that are strongly coupled to the target nuclei. Continuous microwave and…

量子物理 · 物理学 2024-10-31 Matthias Kost , Jianming Cai , Martin B. Plenio

Detecting and controlling nuclear spin nano-ensembles is crucial for the further development of nuclear magnetic resonance (NMR) spectroscopy and for the emerging solid state quantum technology. Here we present the fabrication of a…

We propose a method for the estimation of the initial polarization of spinful nuclei of the 13 C isotope in diamond via a measurement of the evolution of the coherence of an NV center spin qubit. Existing polarization measurement methods…

量子物理 · 物理学 2025-04-01 Mateusz Kuniej , Katarzyna Roszak

We report a study of high-resolution microwave spectroscopy of nitrogen-vacancy centers in diamond crystals at and around zero magnetic field. We observe characteristic splitting and transition imbalance of the hyperfine transitions, which…

We report hyperpolarization of the electronic spins associated with substitutional nitrogen defects in bulk diamond crystal. Hyperpolarization is achieved by optical pumping of nitrogen vacancy centers followed by rapid cross relaxation at…

介观与纳米尺度物理 · 物理学 2017-02-22 M. Loretz , H. Takahashi , T. F. Segawa , J. M. Boss , C. L. Degen

We use nominally forbidden electron-nuclear spin transitions in nitrogen-vacancy (NV) centers in diamond to demonstrate coherent manipulation of a nuclear spin ensemble using microwave fields at room temperature. We show that employing an…

量子物理 · 物理学 2021-04-21 P. Huillery , J. Leibold , T. Delord , L. Nicolas , J. Achard , A. Tallaire , G. Hétet

Scanning-probe and wide-field magnetic microscopes based on Nitrogen-Vacancy (NV) centers in diamond have enabled remarkable advances in the study of biology and materials, but each method has drawbacks. Here, we implement an alternative…

Magnetometry using Nitrogen-Vacancy (NV) color centers in diamond predominantly relies on microwave spectroscopy. However, microwaves may hinder certain studies involving biological systems or thin conductive samples. This work demonstrates…

Solid-state spin defects, such as color centers in diamond, are among the most promising candidates for scalable and integrated quantum technologies. In particular, the good optical properties of silicon-vacancy centers in diamond combined…

量子物理 · 物理学 2024-09-20 Marco Klotz , Andreas Tangemann , Alexander Kubanek

The interplay between disorder and transport is a problem central to the understanding of a broad range of physical processes, most notably the ability of a system to reach thermal equilibrium. Disorder and many body interactions are known…

The unpolarized spin environment surrounding a central spin qubit is typically considered as an incoherent source of dephasing, however, precise characterization and control of the spin bath can yield a resource for storing and sensing with…

量子物理 · 物理学 2023-12-01 R. M. Goldblatt , A. M. Martin , A. A. Wood

The nuclear spin in the vicinity of a nitrogen-vacancy (NV) center possesses of long coherence time and convenient manipulation assisted by the strong hyperfine interaction with the NV center. It is suggested for the subsequent quantum…

量子物理 · 物理学 2018-04-18 Yang-Yang Wang , Jing Qiu , Ying-Qi Chu , Mei Zhang , Jianming Cai , Qing Ai , Fu-Guo Deng

Here we report the fabrication of stable, shallow (< 5 nm) nitrogen-vacancy (NV) centers in diamond by nitrogen delta doping at the last stage of the chemical vapor deposition (CVD) growth process. The NVs are stabilized after treating the…

High concentration of negatively charged nitrogen-vacancy ($\text{NV}^{-}$) centers was created in diamond single crystals containing approximately 100 ppm nitrogen using electron and neutron irradiation and subsequent thermal annealing in…

Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…

Due to their large coherent scattering cross section, diamond nanoparticles (DNPs) are considered as a promising candidate material for a new neutron reflector. For investigation of scattering cross sections of packed samples, we have…

仪器与探测器 · 物理学 2020-07-17 Kenji Mishima , Toshiya Otomoa , Kazutaka Ikeda , Hidetoshi Ohshita

Nuclear magnetic resonance (NMR) imaging with shallow nitrogen-vacancy (NV) centers in diamond offers an exciting route toward sensitive and localized chemical characterization at the nanoscale. Remarkable progress has been made to combat…

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…