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The magnetic ground state of perovskite structure CaRuO3 has been enigmatic for decades. Here we show that paramagnetic CaRuO3 can be made ferromagnetic by very small amounts of partial substitution of Ru by Ti. Magnetic hysteresis loops…

凝聚态物理 · 物理学 2009-11-07 T. He , R. J. Cava

We demonstrate how the quantum paraelectric ground state of SrTiO$_3$ can be accessed via a microscopic $ab~initio$ approach based on density functional theory. At low temperature the quantum fluctuations are strong enough to stabilize the…

Here we have experimentally demonstrated spin-correlation-driven ferroelectric quantum criticality in a prototype quantum spin-liquid system, Ba3CuSb2O9, a quantum phenomenon rarely observed. The dielectric constant follows a clear T2…

强关联电子 · 物理学 2026-04-01 Sayan Ghosh , Gourab Roy , Ekta Kushwaha , Mohit Kumar , Tathamay Basu

Here a recently observed weak first order transition in doped SrTiO3 is argued to be a consequence of the coupling between strain and order parameter fluctuations. Starting with a semi-microscopic action, and using renormalization group…

统计力学 · 物理学 2015-05-13 Nabyendu Das

Composites of ferroelectric and paraelectric perovskites have attracted a lot of attention due to their application potential in energy storage as well as novel computing and memory devices. So far the main focus of research has been on…

材料科学 · 物理学 2025-07-23 Sheng-Han Teng , Chinwendu Anabaraonye , Anna Grünebohm

Materials tuned to the neighbourhood of a zero temperature phase transition often show the emergence of novel quantum phenomena. Much of the effort to study these new effects, like the breakdown of the conventional Fermi-liquid theory of…

强关联电子 · 物理学 2014-05-06 S. E. Rowley , L. J. Spalek , R. P. Smith , M. P. M. Dean , G. G. Lonzarich , J. F. Scott , S. S. Saxena

Similar to other perovskites in its family, $\mathrm{SrTiO_{3}}$ exhibits a significant softening of the ferroelectric mode with decreasing temperature, a behavior that typically heralds the onset of a ferroelectric transition. However,…

量子物理 · 物理学 2026-03-02 Francesco Libbi , Lorenzo Monacelli , Boris Kozinsky

CaRuO3 is a perovskite with an orthorhombic distortion and shows the characteristics of spin-glass behavior below TC=87 K. The La3+ substitution for Ca2+ in Ca1-xLaxRuO3 samples, induces a disorder in the Ca site (the A site) and the system…

超导电性 · 物理学 2009-11-07 I. Felner , U. Asaf

We report new observation of cooperative paramagnetic fluctuations of Ru$^{4+}$ spins that coexist with the non-Fermi liquid state in CaRuO$_{3}$ perovskite below T $\simeq$ 22 K. Detailed electrical, magnetic and neutron scattering…

强关联电子 · 物理学 2016-01-06 J. Gunasekera , L. Harriger , T. Heitmann , H. Knoll , D. K. Singh

SrTiO$_{3}$, a quantum paraelectric, becomes a metal with a superconducting instability after removal of an extremely small number of oxygen atoms. It turns into a ferroelectric upon substitution of a tiny fraction of strontium atoms with…

The temperature dependence of static dielectric susceptibility of a system with strongly coupled fluctuating dipoles is calculated within a self consistent mean fluctuation field approximation. Results are qualitatively in good agreement…

材料科学 · 物理学 2015-05-13 Nabyendu Das , Suresh G. Mishra

Ultrasound velocity measurements of the pseudo-cubic spin-crossover cobaltite LaCoO$_3$ and the lightly Ni-substituted La(Co$_{0.99}$Ni$_{0.01}$)O$_3$ reveal two types of symmetry-resolved elastic anomaly in the insulating paramagnetic…

强关联电子 · 物理学 2025-02-03 T. Watanabe , R. Okada , K. Tomiyasu

The perovskite oxide EuTiO3 (ETO) has attracted increased scientific interest due to its potential multiferroic properties and magnetic activity above and below its structural phase transition at TS=282K. Various experiments have indirectly…

We have investigated the dilute magnetic impurity effect on the magnetic properties of a quantum spin liquid candidate Ba3ZnRu2O9 and a spin gapped compound Ba3CaRu2O9. The magnetic ground state of each compound stands against 2%…

强关联电子 · 物理学 2018-08-09 Takafumi D. Yamamoto , Hiroki Taniguchi , Ichiro Terasaki

We report muon spin relaxation measurements on two Ti3+ containing perovskites, LaTiO3 and YTiO3, which display long range magnetic order at low temperature. For both materials, oscillations in the time-dependence of the muon polarization…

强关联电子 · 物理学 2009-11-13 P. J. Baker , T. Lancaster , S. J. Blundell , W. Hayes , F. L. Pratt , M. Itoh , S. Kuroiwa , J. Akimitsu

SrTiO3 is a textbook quantum paraelectric, with ferroelectricity purportedly suppressed by quantum fluctuations of ionic positions down to the lowest temperatures. The precise real space structure of SrTiO3 at low temperature, however, has…

Many functionally relevant ferroic phenomena in quantum materials can be manipulated by driving the lattice coherently with optical and terahertz pulses. New physical phenomena and non-equilibrium phases that have no equilibrium counterpart…

Fluctuating orders in solids are generally considered high-temperature precursors of broken symmetry phases. However, in some cases these fluctuations persist to zero temperature and prevent the emergence of long-range order, as for example…

材料科学 · 物理学 2019-07-24 Tobia Nova , Ankit Disa , Michael Fechner , Andrea Cavalleri

In ABO3 perovskites, oxygen octahedron rotations are common structural distortions that can promote large ferroelectricity in BiFeO3 with an R3c structure [1], but suppress ferroelectricity in CaTiO3 with a Pbnm symmetry [2]. For many…

材料科学 · 物理学 2016-04-05 Hongwei Wang , Jianguo Wen , Dean J. Miller , Qibin Zhou , Mohan Chen , Ho Nyung Lee , Karin M. Rabe , Xifan Wu

Ferroelectricity in perovskites is known to be suppressed by a moderate hydrostatic pressure. The notion that a polar instability should reappear in a higher pressure regime is well accepted theoretically but experiments have failed so far…

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