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The toolbox for imaging molecules is well-equipped today. Some techniques visualize the geometrical structure, others the electron density or electron orbitals. Molecules are many-body systems for which the correlation between the…

The two-dimensional sub-cycle-time to electron momentum mapping provided by orthogonal two-color laser fields is applied to photoelectron spectroscopy. Using neon as the example we gain experimental access to the dynamics of emitted…

Multipath holographic interference in strong-field quantum tunnel ionization is key to revealing sub-Angstrom attosecond dynamics for molecular movies. This critical sub-cycle motion is often obscured by longer time-scale effects such as…

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

Ionization by relativistically intense laser pulses of finite duration is considered in the framework of strong-field quantum electrodynamics. Our main focus is on the formation of ionization supercontinua. More specifically, when studying…

原子物理 · 物理学 2016-07-13 K. Krajewska , J. Z. Kamiński

The interaction of intense laser pulses with nano-scale particles leads to the production of high-energy electrons, ions, neutral atoms, neutrons and photons. Up to now, investigations have focused on near-infrared to X-ray laser pulses…

Phase-of-the-phase spectroscopy using two-color colinearly polarized laser pulses has been introduced and experimentally applied to strong-field tunneling ionization in S. Skruszewicz et al., Phys. Rev. Lett. 115, 043001 (2015) and recently…

原子物理 · 物理学 2018-12-05 V. Tulsky , M. A. Almajid , D. Bauer

We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…

A three-dimensional semiclassical model is used to study double ionization of Ar when driven by a near-infrared and near-single-cycle laser pulse for intensities ranging from 0.85$\times$10$^{14}$ W/cm$^{2}$ to 5$\times$10$^{14}$…

原子物理 · 物理学 2017-02-15 A. Chen , M. Kübel , B. Bergues , M. F. Kling , A. Emmanouilidou

H-atoms in H$_2$O are rearranged by strong optical fields generated by intense, 10 fs laser pulses to form H$_2^+$, against prevailing wisdom that strong fields inevitably lead to multiple molecular ionization and the subsequent Coulomb…

化学物理 · 物理学 2015-05-13 F. A. Rajgara , D. Mathur , A. K. Dharmadhikari , C. P. Safvan

Ionization rates and Stark shifts of H$_2$, CO, O$_2$, H$_2$O, and CH$_4$ in static electric fields have been computed with coupled-cluster methods in a basis set of atom-centered Gaussian functions with complex-scaled exponent.…

化学物理 · 物理学 2018-06-13 Thomas-C. Jagau

Using a three-dimensional quasiclassical technique we explore molecular double ionization by a linearly polarized, infrared (800 nm) and ultrashort (6 fs) laser pulse. We first focus on intensities corresponding to the tunneling regime and…

原子物理 · 物理学 2015-05-14 A. Emmanouilidou , A. Staudte

In this work we report ab initio calculations for the $H_2^+$ molecule interacting with ultrashort intense laser pulses. We analyse several observables that can, in principle, be available experimentally, in order to get a deeper…

原子物理 · 物理学 2017-05-25 R. E. F. Silva

We report on strong field ionization of S- and R-propylene oxide in circularly polarized two-color laser fields. We find that the relative helicity of the two single color laser fields affects the photoelectron circular dichroism (PECD).…

We propose a novel mechanism of electron localization and molecular symmetry breaking in dissociative photoionization of the H$_2$ molecule. The Coulomb field of the ejected electron can induce transition of the remaining H$_2^+$ ion from…

原子物理 · 物理学 2014-03-12 Vladislav V. Serov , A. S. Kheifets

We present a study of multiphoton dissociative ionization from molecules. By solving the time-dependent Schr\"{o}dinger equation for H$_2^+$ and projecting the solution onto double continuum scattering states, we observe the correlated…

原子物理 · 物理学 2012-07-03 C B Madsen , F Anis , L B Madsen , B D Esry

With a classical ensemble model that including electron correlations during the whole ionization process, we investigated strong-field sequential double ionization of Ar by elliptically polarized pulses at the quantitative level. The…

原子物理 · 物理学 2015-06-04 Yueming Zhou , Cheng Huang , Qing Liao , Peixiang Lu

A detailed theory-versus-experiment comparison is worked out for H$_2^+$ intense laser dissociation, based on angularly resolved photodissociation spectra recently recorded in H.Figger's group. As opposite to other experimental setups, it…

量子物理 · 物理学 2009-11-10 Vassili Serov , Arne Keller , Osman Atabek , Nicolas Billy

The analysis of an angular distribution of the emission intensity of a two-level atom (dipole) in a photonic crystal reveals an enhancement of the emission rate in some observation directions. Such an enhancement is the result of the…

光学 · 物理学 2009-11-13 Dmitry N. Chigrin

Double-slit diffraction studies with photons or massive particles rank among the most beautiful experiments in physics. In particular, measurements at very low intensities demonstrate the particle-wave duality and the coherent superposition…