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Massively parallel ionization of many atoms in a cluster or bio-molecule is identified as new phenomenon of light-matter interaction which becomes feasible through short and intense FEL pulses. Almost simultaneously emitted from the…

原子与分子团簇 · 物理学 2012-04-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

The angular distribution of the emitted electrons, following the two-photon ionization of the hydrogen-like ions, is studied within the framework of second order perturbation theory and the Dirac equation. Using a density matrix approach,…

原子物理 · 物理学 2007-05-23 Peter Koval , Stephan Fritzsche , Andrey Surzhykov

We study strong-field double ionization in a three-electron atom by applying a simplified, reduced-dimensionality model with three active electrons. The influence of the spin-induced symmetry of the spatial part of the wavefunction on the…

Polyatomic molecules in strong laser fields can undergo substantial nuclear motion within tens of femtoseconds. Ion imaging methods based on dissociation or Coulomb explosion therefore have difficulty faithfully recording the geometry…

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…

The angular distribution of the emitted electrons, following the two--photon ionization of the hydrogen--like ions, is studied within the framework of second order perturbation theory \textit{and} the Dirac equation. Using a density matrix…

原子物理 · 物理学 2007-05-23 Peter Koval , Stephan Fritzsche , Andrey Surzhykov

Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…

原子物理 · 物理学 2015-05-27 C. Müller , A. B. Voitkiv

Molecules show a much increased multiple ionization rate in a strong laser field as compared to atoms of similar ionization energy. A widely accepted model attributes this to the action of the joint fields of the adjacent ionic core and the…

原子物理 · 物理学 2013-05-16 J. Wu , M. Meckel , L. Ph. H. Schmidt , M. Kunitski , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

The temporal dynamics of double ionization of H2 has been investigated both experimentally and theoretically with few-cycle laser pulses. The main observables are the proton spectra associated to the H^+ + H^+ fragmentation channel. The…

量子物理 · 物理学 2008-09-23 Sébastien Saugout , Eric Charron , Christian Cornaggia

We theoretically investigate the mechanism of enhanced ionization in two-electron molecules by analyzing Bohmian trajectories for a one-dimensional H2 in an intense laser field. We identify both types of ionizing trajectories corresponding…

量子物理 · 物理学 2015-06-17 Ryohto Sawada , Takeshi Sato , Kenichi L. Ishikawa

Using the recently developed concept of the 2-electron streak camera (see NJP 12, 103024 (2010)), we have studied the energy-sharing between the two ionizing electrons in single-photon double ionization of He(1s2s). We find that the most…

原子物理 · 物理学 2015-05-28 H. Price , A. Staudte , A. Emmanouilidou

We study ionization dynamics of aligned diatomic molecules N$_2$ in strong elliptical laser fields experimentally and theoretically. The alignment dependence of photoelectron momentum distributions (PMDs) of N$_2$ measured in experiments is…

We investigate theoretically the dissociative ionization of a H2+ molecule using two ultrashort laser (pump-probe) pulses. The pump pulse prepares a dissociating nuclear wave packet on an ungerade surface of H2+. Next, an UV (or XUV) probe…

量子物理 · 物理学 2013-05-29 Szczepan Chelkowski , André D. Bandrauk

We analyzed the two-dimensional (2D) electron momentum distributions of high-energy photoelectrons of atoms in an intense laser field using the second-order strong field approximation (SFA2). The SFA2 accounts for the rescattering of the…

原子物理 · 物理学 2009-11-13 Zhangjin Chen , Toru Morishita , Anh-Thu Le , C. D. Lin

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the…

原子物理 · 物理学 2009-02-14 Denys I. Bondar , Wing-Ki Liu , Misha Yu. Ivanov

We investigate the photoionization dynamics of atoms subjected to intense, ultrashort laser pulses through the use of quantum trajectories. This method provides a unique and consistent framework for examining electron dynamics within a…

原子物理 · 物理学 2024-08-01 Taylor Moon , Klaus Bartschat , Nicolas Douguet

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

化学物理 · 物理学 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

We present the first theoretical treatment of the formation of highly excited neutral H atoms (H$^{*}$) for strongly driven H$_{2}$. This process, with one electron ionizing and one captured in a Rydberg state, was recently reported in an…

原子物理 · 物理学 2015-05-28 A. Emmanouilidou , D. Tchitchekova , C. Lazarou , U. Eichmann

Signatures of the Coulomb corrections in the photoelectron momentum distribution during laser-induced ionization of atoms or ions in tunneling and multiphoton regimes are investigated analytically in the case of an one-dimensional problem.…

We use a quantum trajectory-based semi-classical method to account for Coulomb interaction between the photoelectron and the parent ion in the classically forbidden, sub-barrier region during strong-field tunneling ionization processes. We…

原子物理 · 物理学 2017-11-21 Tian-Min Yan , D. Bauer