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Experimental studies of high-purity kagome-lattice antiferromagnets (KAFM) are of great importance in attempting to better understand the predicted enigmatic quantum spin-liquid ground state of the KAFM model. However, realizations of this…

强关联电子 · 物理学 2021-06-02 W. Sun , T. Arh , M. Gomilšek , P. Koželj , S. Vrtnik , M. Herak , J. -X. Mi , A. Zorko

Novel magnetic phases are expected to occur in highly frustrated spin systems. Here we study the structurally perfect kagom\'e antiferromagnet CdCu$_3$(OH)$_6$(NO$_3$)$_2\cdot$H$_2$O by magnetization, magnetic torque, and heat capacity…

强关联电子 · 物理学 2017-03-29 Ryutaro Okuma , Takeshi Yajima , Daisuke Nishio-Hamane , Tsuyoshi Okubo , Zenji Hiroi

The neutron diffraction and nuclear magnetic resonance (NMR) measurements have been used to microscopically analyze the magnetic structure in the $S = 1/2$ kagome antiferromagnet CdCu$_{3}$(OH)$_{6}$(NO$_{3}$)$_{2}\cdot $H$_{2}$O. Below the…

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

The ground state of the simple Heisenberg nearest-neighbor quantum kagome antiferromagnetic model is a magnetically disordered spin liquid, yet various perturbations may lead to fundamentally different states. Here we disclose the origin of…

Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we…

强关联电子 · 物理学 2024-08-30 Aini Xu , Qinxin Shen , Bo Liu , Zhenyuan Zeng , Lankun Han , Liqin Yan , Jun Luo , Jie Yang , Rui Zhou , Shiliang Li

We studied the magnetic properties of YCu$_3$(OH)$_6$Br$_2$[Br$_{1-x}$(OH)$_{x}$] ($x$ = 0.33), where Cu$^{2+}$ ions form two-dimensional kagome layers. There is no magnetic order down to 50 mK while the Curie-Weiss temperature is on the…

We present a $^{35}$Cl NMR study for spin $S=1/2$ perfect kagome antiferromagnet Ca-kapellasite (CaCu$_{3}$(OH)$_{6}$Cl$_{2}\cdot$0.6H$_{2}$O) with a magnetic transition at $T^{\ast}=7.2$ K. The static magnetic structure in the ground state…

强关联电子 · 物理学 2020-07-01 Y. Ihara , K. Arashima , H. Yoshida , M. Hirata , T. Sasaki

The quantum kagome antiferromagnets YCu3(OH)6OxCl3-x (x=0,1/3) are produced using a unified solid state synthesis route for polycrystalline samples. From structural refinements based on neutron diffraction data, we clarify the structure of…

Crystal and magnetic structures of the mineral centennialite CaCu$_3$(OH)$_6$Cl$_2\cdot0.6$H$_2$O are investigated by means of synchrotron x-ray diffraction and neutron diffraction measurements complemented by density functional theory…

The search for the experimental evidence of quantum spin liquid (QSL) states is critical but extremely challenging, as the quenched interaction randomness introduced by structural imperfection is usually inevitable in real materials.…

强关联电子 · 物理学 2022-11-08 Fangjun Lu , Long Yuan , Jian Zhang , Boqiang Li , Yongkang Luo , Yuesheng Li

We report a single-crystal neutron diffraction and inelastic neutron scattering study on the spin 1/2 cuprate Cu$_3$Bi(SeO$_3$)$_2$O$_2$Cl, complemented by dielectric and electric polarization measurements. The study clarifies a number of…

High-resolution time-of-flight powder neutron diffraction and high-field magnetization were measured to investigate the magnetic structure and existence of a field-induced magnetic phase transition in the distorted kagome antiferromagnet…

We present the crystal structure and magnetic properties of Y$_{3}$Cu$_{9}$(OH)$_{19}$Cl$_{8}$, a stoichiometric frustrated quantum spin system with slightly distorted kagome layers. Single crystals of Y$_{3}$Cu$_{9}$(OH)$_{19}$Cl$_{8}$…

Motivated by the recent experiments on the new spin half Kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid groundstate and is constructed so as to mimic the…

强关联电子 · 物理学 2009-11-13 R. Chitra , M. J. Rozenberg

Y-kapellasite (Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$), which hosts an original anisotropic kagome sublattice, is a promising candidate for studying elusive and complex correlated physics. It exhibits a theoretically predicted in-plane $(1/3, 1/3)$…

Y{0.5}$Ca{0.5}BaCo4O7 contains kagome layers of Co ions, whose spins are strongly coupled according to a Curie-Weiss temperature of -2200 K. At low temperatures, T = 1.2 K, our diffuse neutron scattering study with polarization analysis…

强关联电子 · 物理学 2015-06-25 W. Schweika , M. Valldor , P. Lemmens

Several Cu$^{2+}$ hydroxide minerals have recently been identified as candidate realizations of the $S=1/2$ kagome Heisenberg model. In this context, we have studied the distorted system KCu$_3$As$_2$O$_7$(OD)$_3$ using neutron scattering…

We report bulk magnetization, and elastic and inelastic neutron scattering measurements under an external magnetic field, $H$, on the weakly coupled distorted kagome system, Cu_{2}(OD)_3Cl. Our results show that the ordered state below 6.7…

强关联电子 · 物理学 2009-11-13 J. -H. Kim , S. Ji , S. -H. Lee , B. Lake , T. Yildirim , H. Nojiri , K. Habicht , Y. Qiu , K. Kiefer

We present a detailed powder and single crystal neutron diffraction study of the spin chain compound Ca3Co2O6. Below 25 K, the system orders magnetically with a modulated partially disordered antiferromagnetic structure. We give a…

强关联电子 · 物理学 2008-09-17 S. Agrestini , L. C. Chapon , A. Daoud-Aladine , J. Schefer , A. Gukasov , C. Mazzoli , M. R. Lees , O. A. Petrenko
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