相关论文: Bond strengthening in dense H2O and implications t…
We propose three new phases of H2O under ultrahigh pressure. Our structural search was performed using an adaptive genetic algorithm which allows an extensive exploration of crystal structure. The new sequence of pressure-induced…
The HDO/H2O abundance ratio is thought to be a key diagnostic on the evolution of water during the star- and planet-formation process and thus on its origin on Earth. We here present millimeter-wavelength high angular resolution…
Detection of water vapor in the atmosphere of temperate rocky exoplanets would be a major milestone on the path towards characterization of exoplanet habitability. Past modeling work has shown that cloud formation may prevent the detection…
The supra-molecular structure of a liquid is strongly connected to its dynamics which in turn controls macroscopic properties such as viscosity. Consequently, detailed knowledge about how this structure changes with temperature is essential…
The ice-albedo feedback is a potentially important de-stabilizing effect for the climate of terrestrial planets. It is based on the positive feedback between decreasing surface temperatures, an increase of snow and ice cover and an…
This paper reviews recent observations of water in Galactic interstellar clouds and nearby galactic nuclei. Two results are highlighted: (1) Multi-line H$_2$O mapping of the Orion Bar shows that the water chemistry in PDRs is driven by…
An understanding of the abundance and distribution of water vapor in the innermost region of protoplanetary disks is key to understanding the origin of habitable worlds and planetary systems. Past observations have shown H2O to be abundant…
Earth-like, potentially habitable exoplanets are prime targets in the search for extraterrestrial life. Information about their atmosphere and surface can be derived by analyzing light of the parent star reflected by the planet. We…
A direct measure of hydrogen bonding in water under conditions ranging from the normal state to the supercritical regime is derived from the Compton scattering of inelastically-scattered X-rays. First, we show that a measure of the number…
H2O is the most abundant component of astrophysical ices. In most lines of sight it is not possible to fit both the H2O 3 um stretching, the 6 um bending and the 13 um libration band intensities with a single pure H2O spectrum. Recent…
The atmospheric C/O ratio of exoplanets is widely used to constrain their formation. To guarantee that the C/O ratio provides robust information, we need to accurately quantify the amount of C and O in exoplanetary atmospheres. In the case…
Tidal dissipation in planetary interiors is one of the key physical mechanisms that drive the evolution of star-planet and planet-moon systems. New constraints are now obtained both in the Solar and exoplanetary systems. Tidal dissipation…
Data suggest that most rocky exoplanets with orbital period $p$ $<$ 100 d ("hot" rocky exoplanets) formed as gas-rich sub-Neptunes that subsequently lost most of their envelopes, but whether these rocky exoplanets still have atmospheres is…
Water-rich planets such as Earth are expected to become eventually uninhabitable, because liquid water does not remain stable at the surface as surface temperatures increase with the solar luminosity over time. Whether a large increase of…
Hydrogen bond is often assumed to be a purely electrostatic interaction between a electron-deficient hydrogen atom and a region of high electron density. Here, for the first time, we directly image hydrogen bond in real space by…
Many parameters constraining the spectral appearance of exoplanets are still poorly understood. We therefore study the properties of irradiated exoplanet atmospheres over a wide parameter range including metallicity, C/O ratio and host…
C-H-N-O system is central for organic chemistry and biochemistry, and plays a major role in planetary science (dominating the composition of "ice giants" Uranus and Neptune). The inexhaustible chemical diversity of this system at normal…
The high-pressure behavior of monoclinic VO$_2$ is revisited by a combination of Raman spectroscopy and X-ray diffraction on a single crystal under hydrostatic conditions at room temperature. A soft mode is observed up to P$_c$ = 13.9(1)…
A combination of the temporally and spatially resolved phonon spectroscopy has enabled calibration of hydrogen bond transition from the vibration mode of heavy water to the core/shelled nanodroplet and the subnanosized ionic hydration shell…
Most experimentally known high-pressure ice phases have a body-centred cubic (bcc) oxygen lattice. Our atomistic simulations show that, amongst these bcc ice phases, ices VII, VII' and X are the same thermodynamic phase under different…