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Temperature-responsive properties of surface-attached poly(N-isopropylacrylamide) (PNIPAM) network films with well-controlled chemistry are investigated. The synthesis consists of cross-linking and grafting preformed ene-reactive polymer…

材料科学 · 物理学 2016-04-13 Mengxing Li , Bruno Bresson , F Cousin , Christian Fretigny , Yvette Tran

We developed functional surfaces of laser-microstructured silicon coated with blends of polystyrene (PS) and poly(N-isopropylacrylamide) (PNIPAM) and we study their switching wetting behavior between hydrophilicity and hydrophobicity. Large…

Nanostructured polymer-metal oxide composites are a current research area of great importance due to its highlight applications in sensors, optics, catalysts and drug delivery. Particularly the use of thermoresponsive polymers gives more…

软凝聚态物质 · 物理学 2020-07-21 Hong Xu

Thermoresponsive poly(N-isopropylacrylamide) (PNIPAM) particles of different sizes are synthesized by varying the concentration of sodium dodecyl sulphate (SDS) in a one-pot method. The sizes, size polydispersities and the…

软凝聚态物质 · 物理学 2020-09-23 Chandeshwar Misra , Sanjay Kumar Behera , Ranjini Bandyopadhyay

Poly(N-isopropylacrylamide) (PNIPAM) is a synthetic polymer that is widely studied for its thermoresponsive character. However, recent works also reported evidence of a low temperature (protein-like) dynamical transition around 225 K in…

We synthesize thermoresponsive poly(N-isopropylacrylamide) (PNIPAM) colloidal microgel particles of different stiffnesses by controlling the concentration of crosslinker in a one-pot synthesis method. We employ oscillatory rheology and…

软凝聚态物质 · 物理学 2024-02-12 Chandeshwar Misra , Sanjay Kumar Behera , Sonali Vasant Kawale , Ranjini Bandyopadhyay

Temperature-sensitive hydrogels based on polymers such as poly(N-isopropylacrylamide) (PNIPAM) undergo a volume phase transition in response to changes in temperature. During this transition, distinct changes in both thermal and mechanical…

软凝聚态物质 · 物理学 2017-07-19 Frank J. Aangenendt , Johan Mattsson , Wouter G. Ellenbroek , Hans M. Wyss

Polyimide (PI) thin films are widely used in advanced technologies, yet accurate characterization of their thermal properties remains challenging, as evidenced by significant inconsistencies in reported data and an incomplete understanding…

应用物理 · 物理学 2026-04-15 Bingjiang Zhang , Dihui Wang , Tao Chen , Heng Ban , Puqing Jiang

We probe, using the Surface Forces Apparatus, the thermal response of poly(N-isopropylacrylamide) (PNIPAM) brushes of various grafting densities, grown from plasma-activated mica by means of surface-initiated polymerization. We thus show…

软凝聚态物质 · 物理学 2009-10-09 Ibrahim Bou Malham , Lionel Bureau

Hypotheses: Additives are commonly used to tune macromolecular conformational transitions. Among additives, trehalose is an excellent bioprotectant and among responsive polymers, PNIPAM is the most studied material. Nevertheless, their…

The viscoelastic properties of thin polymeric films represent a central issue, especially for nanotechnological applications. In particular, it is highly relevant the dependence of viscoelasticity on the temperature. For polystyrene it is…

Density of the polyacrylamide ultrathin films has been studied using X-ray reflectivity technique. Two sources (one powder and another aqueous solution) of polyacrylamide were used to prepare spin coated films on silicon substrate. Light…

软凝聚态物质 · 物理学 2009-04-14 Mojammel H. Mondal , M. Mukherjee , K. Kawashima , K. Nishida , T. Kanaya

The effect of annealing on the dynamical behavior of swelling for ultrathin polyacrylamide films deposited on silicon substrates have been studied using X-ray reflectivity technique. The spin coated polyacrylamide films of similar…

软凝聚态物质 · 物理学 2009-04-14 Mojammel H. Mondal , M. Mukherjee

The thermosensitive behavior of microgel particles suspended in solvents, i.e. their temperature-dependent swelling properties, has triggered ongoing interest in industry and academia over the past forty years. The most-studied polymer is…

软凝聚态物质 · 物理学 2026-04-23 Domenico Truzzolillo , Thomas Hellweg , Julian Oberdisse

The crystal growth of isotactic polystyrene (it-PS) is investigated in very thin, 11 nm thick films. The it-PS crystals grown in the thin films show quite different morphology from that in the bulk. With decreasing crystallization…

软凝聚态物质 · 物理学 2016-08-31 Ken Taguch , Hideki Miyaji , Kunihide Izumi , Akitaka Hoshino , Yoshihisa Miyamoto , Ryohei Kokawa

Poly-N-isopropylacrylamide (PNIPAM) is a thermoresponsive polymer, an essential building block of a large family of soft smart materials. In neat water it undergoes upon heating at $\approx$305K a phase transition from swollen to collapsed…

化学物理 · 物理学 2018-06-15 Vladimir Palivec , Denis Zadrazil , Jan Heyda

Poly(N-isopropylacrylamide), PNIPAM, is a widely studied polymer, which serves as a key constituent of nanostructured soft materials with responsive properties. Upon increasing temperature the PNIPAM polymer chain undergoes a reversible…

软凝聚态物质 · 物理学 2019-10-22 Letizia Tavagnacco , Emanuela Zaccarelli , Ester Chiessi

We describe the design of micropatterned surfaces for single cell studies, based on thermoresponsive polymer brushes. We show that brushes made of poly(N-isopropylacrylamide) grafted at high surface density display excellent protein and…

软凝聚态物质 · 物理学 2012-06-04 Kalpana Mandal , Martial Balland , Lionel Bureau

The advances in new technologies have prompted the need for functional systems smaller than the gyration radius of polymer chains. Thus, understanding how nanoconfinement affects polymer properties has been the focus of a lot of research…

软凝聚态物质 · 物理学 2010-07-27 Fabrice Cousin , Jérémie Gummel , Daniel Clemens , Isabelle Grillo , François Boué

Wrinkling patterns at the metallized surface of thin polymer films are shown to be sensitive to the sticky or slippery character of the polymer/substrate interface (titanium coating, polystyrene film and coated silicon substrate). Selective…

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