相关论文: Key signal contributions in photothermal deflectio…
Adsorption processes play a fundamental role in molecular transport through nanofluidic systems, but their signatures in measured signals are often hard to distinguish from other processes like diffusion. In this paper, we derive an…
Time-domain thermoreflectance (TDTR) and frequency-domain thermoreflectance (FDTR) have been widely used for non-contact measurement of anisotropic thermal conductivity of materials with high spatial resolution. However, the requirement of…
Ultra-fast and multi-dimensional spectroscopy gives a powerful looking glass into the dynamics of molecular systems. In particular two-dimensional electronic spectroscopy (2DES) provides a probe of coherence and the flow of energy within…
Photoreflectance is used for the characterisation of semiconductor samples, usually by sweeping the monochromatized probe beam within the energy range comprised between the highest value set by the pump beam and the lowest absorption…
We analyze the optical pump-probe reflection and transmission coefficients when the photoinduced response depends nonlinearly on the incident pump intensity. Under these conditions, we expect the photoconductivity depth profile to change…
Ta$_{3}$N$_{5}$ is among the most intensively studied photoanode materials for solar-driven water oxidation, yet its performance often remains limited by short carrier lifetimes and defect mediated recombination. Although transient…
We have used a photothermal technique, in which chopped light heats the front surface of a small ( ~ 1 mm2) sample and the chopping frequency dependence of thermal radiation from the back surface is measured with a liquid nitrogen cooled…
The nonlinear response of materials, an increasingly important aspect of light-matter interaction, can be challenging to measure in highly absorbing materials. Here, we introduce an interferometric technique that enables a direct…
Two-pulse correlation experiments performed using pulses of different intensities on Pd(111) with different CO coverages showed that the CO photodesorption probability depends on whether the strong or the weak pulse arrives first to the…
In the present work I analyze the factors that affect signal generation in the measurement of photothermal expansion with an atomic force microscopy probe. I discuss the general properties of the signal transduction mechanism considering…
Inconclusive photon subtraction (IPS) is a conditional measurement scheme to force nonlinear evolution of a given state. In IPS the input state is mixed with the vacuum in a beam splitter and then the reflected beam is revealed by ON/OFF…
Nanomechanical spectroscopy (NMS) is a recently developed approach to determine optical absorption spectra of nanoscale materials via mechanical measurements. It is based on measuring changes in the resonance frequency of a membrane…
The amplification obtained using weak values is quantified through a detailed investigation of the signal to noise ratio for an optical beam deflection measurement. We show that for a given deflection, input power and beam radius, the use…
The photonic density of states (PDS) of the eigen polarizations (EPs) in cholesteric liquid crystal (CLC) cells are calculated. The exact analytic expressions for the reflection and transmission matrices for the finite thickness CLC layer…
In this technical review we give an introduction to optical spectroscopy for layered materials as a powerful, non-invasive tool to access details of the electronic band structure and crystal quality. Potential applications in photonics and…
The photon statistics of Spontaneous Parametric Down Conversion (SPDC) exhibit dependencies on wavelength, pump power, and coincidence time. Notably, the average photon numbers were found to asymmetrically increase with increasing pump…
Optical pump-probe spectroscopy is a powerful tool for the study of non-equilibrium electronic dynamics and finds wide applications across a range of fields, from physics and chemistry to material science and biology. However, a shortcoming…
A method of measuring the relative phase of the energy gap in a high-temperature superconductor is suggested for electron energy loss spectroscopy. Energy-resolved measurements of off-specular scattering should show a feature similar to the…
The analysis of high spectral resolution spectroscopic and spectropolarimetric observations constitute a very powerful way of inferring the dynamical, thermodynamical, and magnetic properties of distant objects. However, these techniques…
Thermoreflectance techniques, including time-domain thermoreflectance (TDTR), frequency-domain thermoreflectance (FDTR), and the square-pulsed source (SPS) method, are powerful tools for characterizing the thermal properties of bulk and…