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The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

Time-domain analysis of harmonic fields with sub-cycle resolution is now experimentally viable due to the emergence of sensitive, on-chip techniques for petahertz-scale optical-field sampling. We demonstrate how such a time-domain,…

We investigate the generation of higher-order harmonics from a quantum optics perspective via the interaction of a semiconductor with a coherent pump field focusing on the regime where strong-field intraband excitations dominate. The…

Strong-field methods in solids enable new strategies for ultrafast nonlinear spectroscopy and provide all-optical insights into the electronic properties of condensed matter in reciprocal and real space. Additionally, solid-state media…

We propose a novel picture of high-harmonic generation (HHG) in solids based on the concept of temporally changing band structures. To demonstrate the utility of this picture, we focus on the high-order sideband generation (HSG) caused by…

材料科学 · 物理学 2019-08-14 Tomohiro Tamaya , Takeo Kato

We study intraband high-order harmonic generation arising from a band-gap material driven by a linearly polarized laser field. We factorize the intraband high-order harmonic-generation signal into intracycle and intercycle terms. The…

Over the past decade, ultrafast electron dynamics in the solid state have been extensively studied using various strong light-matter interaction techniques, such as high-harmonic generation. These studies lead to multiple interpretations of…

Solids in an intense laser field show high-harmonic generation (HHG), which can provide information on carrier dynamics and band structures in weakly correlated systems. In strongly correlated systems, a laser field can induce a transition…

强关联电子 · 物理学 2025-08-04 Ryohei Ikeda , Yuta Murakami , Daiki Sakai , Tatsuya Miyamoto , Toshimitsu Ito , Hiroshi Okamoto

High-harmonic generation by a laser-driven solid slab is simulated using time-dependent density functional theory. Multiple harmonic plateaus up to very high harmonic orders are observed already at surprisingly low field strengths. The full…

原子物理 · 物理学 2017-11-29 Kenneth K. Hansen , Tobias Deffge , Dieter Bauer

The development of sources delivering non-classical states of light is one of the main needs for applications of optical quantum information science. Here, we demonstrate the generation of non-classical states of light using strong-laser…

A new nonlinear scheme of high harmonics generation in a wide class of time-reversal invariant materials with broken spatial inversion symmetry (where recently the nonlinear Hall effect has been established) due to the nontrivial topology…

介观与纳米尺度物理 · 物理学 2021-01-04 H. K. Avetissian , G. F. Mkrtchian

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Anomalous high-harmonic generation (HHG) arises in certain solids when irradiated by an intense laser field, as the result of a nonlinear perpendicular current akin to a Hall current. Here, we theoretically characterize the anomalous HHG…

光学 · 物理学 2023-05-03 Lun Yue , Mette B. Gaarde

In the framework of linear optics, light fields do not interact with each other in a medium. Yet, when their field amplitude becomes comparable to the electron binding energies of matter, the nonlinear motion of these electrons emits new…

High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…

光学 · 物理学 2025-10-20 Marcelo F. Ciappina

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…

We consider a quantum mechanical model for the high-order harmonic generation in bulk solids. The bandgap is assumed to be considerably larger than the exciting photon energy. Using dipole approximation, the dynamical equations for…

量子物理 · 物理学 2017-11-09 Viktor Szaszkó-Bogár , Katalin Varjú , Péter Földi

We investigate theoretically the strong-field regime of light-matter interactions in the topological-insulator class of quantum materials. In particular, we focus on the process of non-perturbative high-order harmonic generation from the…

介观与纳米尺度物理 · 物理学 2022-01-24 Denitsa Baykusheva , Alexis Chacón , Dasol Kim , Dong Eon Kim , David A. Reis , Shambhu Ghimire

In the field of high-order harmonic generation from solids, the electron motion typically exceeds the edge of the first Brillouin zone. In conventional nonlinear optics, on the other hand, the excursion of band electrons is negligible.…

光学 · 物理学 2022-12-28 Jan Reislöhner , Doyeong Kim , Ihar Babushkin , Adrian N. Pfeiffer

The long standing issue of separating resonant from non-resonant processes in extreme nonlinear optics is resolved. The theoretical formalism is applied to high harmonic generation (HHG) in solids and reveals a deeper view into the dominant…

光学 · 物理学 2022-06-03 A. Thorpe , N. Boroumand , A. M. Parks , E. Goulielmakis , T. Brabec
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