相关论文: Observation of strong nonlinear interactions in pa…
We show that the nonlinear interactions between x rays and longer wavelengths in crystals depend strongly on the band structure and related properties. Consequently, these types of interactions can be used as a powerful probe for…
We present a combined theoretical and experimental study of X-ray optical wave mixing. This class of nonlinear phenomena combines the strengths of spectroscopic techniques from the optical domain, with the high-resolution capabilities of…
X-ray parametric down-conversion is a fundamental nonlinear effect that promises a wide range of possible applications. Nevertheless, it has been scarcely investigated and unequivocal evidence of the effect is still missing for certain…
We present measurements of the polarization dependencies of the x-ray signal photons generated by the effect of parametric down-conversion of x rays into ultraviolet radiation. The results exhibit pronounced discrepancies with the classical…
The interaction of high-energy electrons and X-ray photons with soft semiconductors such as halide perovskites is essential for the characterisation and understanding of these optoelectronic materials. Using nano-probe diffraction…
Nonlinear optical responses provide a powerful way to understand the microscopic interactions between laser fields and matter. They are critical for plenty of applications, such as in lasers, integrated photonic circuits, biosensing and…
Interaction of non-relativistic electrons with single crystal target may produce coherent x-rays. That is the result of interference between two known x-ray generation mechanisms having orientational behavior, namely parametric x-rays and…
Nonlinear optics is of crucial importance in several fields of science and technology with applications in frequency conversion, entangled-photon generation, self-referencing of frequency combs, crystal characterization, sensing, and…
We theoretically examine neon atoms in ultrashort and intense x rays from free electron lasers and compare our results with data from experiments conducted at the Linac Coherent Light Source (LCLS). For this purpose, we treat in detail the…
We report a phase-sensitive nonlinear x-ray response in the charge-density-wave material 1T-TaS2, revealed through x-ray parametric down-conversion into the ultraviolet. Extending nonlinear x-ray wave mixing beyond conventional crystalline…
We study the scattering of electromagnetic waves in anisotropic energetic materials. Nonlinear light-matter interactions in molecular crystals result in frequency-conversion and polarization changes. Applied electromagnetic fields of…
We investigate the nonlinear interaction between a relativistically strong laser beam and a plasma in the quantum regime. The collective behavior of the electrons is modeled by a Klein-Gordon equation, which is nonlinearly coupled with the…
Intense efforts have been made in recent years to realize nonlinear optical interactions at the single-photon level. Much of this work has focused on achieving strong third-order nonlinearities, such as by using single atoms or other…
The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…
Graphene is known to possess strong optical nonlinearity. Its nonlinear response can be further enhanced by graphene plasmons. Here, we report a novel nonlinear electro-absorption effect observed in nanostructured graphene due to excitation…
Semiclassical methods are used to study the nonlinear interaction of light in vacuum in the context of four wave mixing. This study is motivated by a desire to investigate the possibility of using recently developed powerful ultrashort…
Nonlinear optical processes rely on the intrinsically weak interactions between photons enabled by their coupling with matter. Unfortunately, many applications in nonlinear optics are severely hindered by the small response of conventional…
Optical pulses are routinely used to drive dynamical changes in the properties of solids. In quantum materials, many new phenomena have been discovered, including ultrafast transitions between electronic phases, switching of ferroic orders…
We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…
Advances in our ability to understand and utilize the world around us have always relied on the development of advanced tools for probing and manipulating materials properties. X-ray matter interactions played a critical role in the…