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Nanocomposites are promising candidates for the next generation of thermoelectric materials since they exhibit extremely low thermal conductivities as a result of phonon scattering on the boundaries of the various material phases. The…

介观与纳米尺度物理 · 物理学 2017-12-06 Samuel Foster , Mischa Thesberg , Neophytos Neophytou

Some of the most promising candidates for next generation thermoelectrics are nanocomposites due to their low thermal conductivities that result from phonon scattering on the boundaries of the various material phases. However, in order to…

材料科学 · 物理学 2019-03-04 Samuel Foster , Mischa Thesberg , Neophytos Neophytou

Silicon carbide nanoparticles with diameters around 8 nm and with narrow size distribution have been finely mixed with doped silicon nanopowders and sintered into bulk samples to investigate the influence of nanoinclusions on electrical and…

材料科学 · 物理学 2021-10-27 S. Aria Hosseini , Devin Coleman , Sabah Bux , P. Alex Greaney , Lorenzo Mangolini

Low band gap thermoelectric materials suffer from bipolar effects at high temperatures, with increased electronic thermal conductivity and reduced Seebeck coefficient, leading to reduced power factor and low ZT figure of merit. In this work…

材料科学 · 物理学 2022-03-14 Patrizio Graziosi , Zhen Li , Neophytos Neophytou

We investigate the electric and thermoelectric transport coefficients of nanocomposites using the Non-Equilibrium Greens Function (NEGF) method, which can accurately capture the details of geometry and disorder in these structures. We…

介观与纳米尺度物理 · 物理学 2018-10-17 Vassilios Vargiamidis , Samuel Foster , Neophytos Neophytou

Bipolar carrier transport is often a limiting factor in the thermoelectric efficiency of narrow bandgap materials at high temperatures due to the reduction in the Seebeck coefficient and the introduction of an additional term to the thermal…

材料科学 · 物理学 2019-03-27 Samuel Foster , Neophytos Neophytou

The correlated couple of electrical and thermal property is the challenge to realize a substantial leap in thermoelectric materials.Synthesis of semiconductor and metal composites is a significant and versatile design strategy to optimize…

应用物理 · 物理学 2018-05-23 Wenwen Zheng , Peng Bi , Fengming Liu , Yong Liu , Jing Shi , Rui Xiong , Ziyu Wang

Based on the concept of band bending at metal/semiconductor interfaces as an energy filter for electrons, we present a theory for the enhancement of the thermoelectric properties of semiconductor materials with metallic nanoinclusions. We…

材料科学 · 物理学 2008-07-03 Sergey V. Faleev , François Léonard

The addition of porosity to thermoelectric materials can significantly increase the figure of merit, ZT, by reducing the thermal conductivity. Unfortunately, porosity is also detrimental to the thermoelectric power factor in the numerator…

介观与纳米尺度物理 · 物理学 2021-03-29 S. Aria Hosseini , Giuseppe Romano , P. Alex Greaney

Introducing hierarchical disorder from multiple defects into materials through nanostructuring is one of the most promising directions to achieve extremely low thermal conductivities and thus improve thermoelectric performance. The success…

材料科学 · 物理学 2019-09-16 Laura de Sousa Oliveira , Vassilios Vargiamidis , Neophytos Neophytou

The Seebeck coefficient is an important quantity in determining the thermoelectric efficiency of a material. Phosphorene is a two-dimensional material with a puckered structure, which makes its properties anisotropic. In this work, a…

材料科学 · 物理学 2023-01-05 M. Amir Bazrafshan , Farhad Khoeini

We report here metal to insulator transition, colossal Seebeck coefficient and ultralow thermal conductivity (0.0057th of its bulk value, significantly smaller than many well-known thermoelectric materials and silicon, showing potential…

材料科学 · 物理学 2020-01-28 Vikash Sharma , Gunadhor Singh Okram , Yung-Kang Kuo

The present study demonstrates a large enhancement in the Seebeck coefficient and ultralow thermal conductivity (TE) in Sb$_2$Te$_3$-AgSbTe$_2$ nanocomposite thin film. The addition of Ag leads to the in-situ formation of AgSbTe$_2$…

It has been demonstrated that InSb nanoinclusions, which are formed in situ, can simultaneously improve all three individual thermoelectric properties of the n-type half Heusler compound (Ti,Zr,Hf)(Co,Ni)Sb [Xie et al., Acta Mater. 58, 4795…

Nanostructured materials and nanocomposites have shown great promise for improving the efficiency of thermoelectric materials. Herein, Fe nanoparticles were imbedded into a CrN matrix by combining two physical vapor deposition approaches,…

It is suggested that low dimensionality can improve the thermoelectric (TE) power factor of a device, offering an enhancement of the ZT figure of merit. In this work the atomistic sp3d5s*-spin-orbit-coupled tight-binding model and the…

介观与纳米尺度物理 · 物理学 2011-06-13 Neophytos Neophytou , Hans Kosina

We theoretically unveil the unconventional possibility to achieve extremely high thermoelectric power factors in lightly doped narrow gap semiconductors with asymmetric conduction/valence bands operated in the bipolar transport regime.…

材料科学 · 物理学 2020-08-05 Patrizio Graziosi , Neophytos Neophytou

Low dimensional structures have demonstrated improved thermoelectric (TE) performance because of a drastic reduction in their thermal conductivity, {\kappa}l. This has been observed for a variety of materials, even for traditionally poor…

材料科学 · 物理学 2012-01-31 Neophytos Neophytou , Hans Kosina

We investigate the thermoelectric properties of a hybrid nanodevice composed by a 2D carbon based material and a superconductor. This system presents nonlinear bipolar thermoelectricity as induced by the spontaneous breaking of the…

介观与纳米尺度物理 · 物理学 2023-04-11 Lorenzo Bernazzani , Giampiero Marchegiani , Francesco Giazotto , Stefano Roddaro , Alessandro Braggio

Engineering materials to include nanoscale porosity or other nanoscale structures has become a well-established strategy for enhancing the thermoelectric performance of dielectrics. However, the approach is only considered beneficial for…

材料科学 · 物理学 2021-10-14 Hosseini , S. Aria , Romano , Giuseppe , Greaney , P. Alex
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