相关论文: Direct Numerical Observation of Real-Space Recolli…
High harmonic generation (HHG) from gas phase atoms (or molecules) has opened up a new frontier in ultrafast optics, where attosecond time resolution and Angstrom spatial resolution are accessible. The fundamental physical pictures of HHG…
We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…
High-harmonic generation (HHG) is a coherent optical process in which the incident photon energy is up-converted to the multiples of its initial energy. In solids, under the influence of a strong laser field, electron-hole (e-h) pairs are…
Acting as a highly nonlinear response to the strong laser field, high harmonic generation (HHG) naturally contains the fingerprints of atomic and electronic properties of materials. Electronic properties of a solid such as band structure…
We study numerically the Bloch electron wavepacket dynamics in periodic potentials to simulate laser-solid interactions. We introduce a new perspective in the coordinate space combined with the motion of the Bloch electron wavepackets…
High harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C$_{60}$, with 240 valence electrons engaging harmonic generation at each crystal momentum, the…
We revisit the mechanism of high harmonic generation (HHG) from solids by comparing HHG in laser fields with different ellipticities but constant maximum amplitude. It is shown that the cutoff of HHG is strongly extended in a circularly…
We investigate the high harmonic generation (HHG) from solids by simulating the dynamics of a single active electron in periodic potentials. The corresponding time-dependent Schr\"odinger equations (TDSE) are solved numerically by using…
High-harmonic generation (HHG) in solids has emerged in recent years as a rapidly expanding and interdisciplinary field, attracting attention from both the condensed-matter and the atomic, molecular, and optics communities. It has exciting…
We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…
An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…
State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…
We investigate the orientation dependence of molecular high-order harmonic generation (HHG) both numerically and analytically. We show that the molecular recollision electronic wave packets (REWPs) in the HHG are closely related to the…
High harmonic generation (HHG) in solids has emerged as a powerful spectroscopic method for resolving ultrafast electron dynamics and band structure properties across a wide range of materials. However, quantitative HHG studies require…
Non-perturbative high-harmonic generation (HHG) has recently been observed in the liquid phase, where it was demonstrated to have a different physical mechanism compared to gas and solid phases of matter. The currently best physical picture…
We develop and demonstrate a fully real-space perspective on HHG in crystals. Due to Wannier-Stark localization induced on sub-cycle timescales in the presence of a strong field, real-space descriptions are natural for strongly driven…
High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…
Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…
We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…
High harmonic generation (HHG) in solids has recently emerged as a powerful all-optical approach for probing material properties and ultrafast electron dynamics in quantum systems. It has been widely applied for studying two-dimensional and…