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The inclusion of atomic inversion in Raman scattering can significantly alter field dynamics in plasmonic settings. Our calculations show that large local fields and femtosecond pulses combine to yield: (i) population inversion within hot…

光学 · 物理学 2015-06-15 M. Scalora , M. A. Vincenti , D. de Ceglia , M. Grande , J. W. Haus

We demonstrate low-frequency interferometric impulsive stimulated Raman scattering (ISRS) imaging with high robustness to distortions by optical scattering. ISRS is a pump-probe coherent Raman spectroscopy that can capture Raman vibrational…

High-gain resonant nonlinear Raman scattering on trapped cold atoms within a high-fineness ring optical cavity is simply explained under a nonlinear opto-mechanical mechanism, and a proposal using it to detect frequency of micro-trap on…

原子物理 · 物理学 2014-03-24 Lin Zhang

We discuss layout and performance of a high-resolution Stimulated Raman Loss spectrometer that has been newly developed for accurate studies of spectral lineshapes and line center frequencies of hydrogen isotopologues and in general of…

光学 · 物理学 2023-04-06 M. Lamperti , L. Rutkowski , D. Gatti , R. Gotti , L. Moretti , D. Polli , G. Cerullo , M. Marangoni

The evolution versus pump power of the spectrum of a singly resonant optical parametric oscillator based on an MgO-doped periodically poled stoichiometric lithium tantalate crystal is observed. The onset of cascade Raman lasing due to…

光学 · 物理学 2015-05-13 T-H. My , O. Robin , O. Mhibik , C. Drag , F. Bretenaker

We revisit laser intensity noise in the context of stimulated Raman scattering (SRS), which has recently proved to be a key technique to provide label free images of chemical bonds in biological and medical samples. Contrary to most…

仪器与探测器 · 物理学 2019-10-29 Xavier Audier , Sandro Heuke , Peter Volz , Ingo Rimke , Hervé Rigneault

Transient absorption and Raman scattering measurements on noble metal nanoparticles offer complimentary information on their vibrational modes and mechanical interactions with their surroundings. We have developed a comprehensive modeling…

介观与纳米尺度物理 · 物理学 2024-10-29 Rachel Gelfand , Matthew Pelton

The inelastic scatterings of matter systems, such as Raman scattering, contain rich information on mechanical vibrations like as resonant frequencies, which lead to various applications, for example, a sensor for specific molecules.…

量子物理 · 物理学 2021-10-04 Sho Tamaki , Tomohiro Yokoyama , Hajime Ishihara

Near-field enhanced, nano-Raman spectroscopy has been successfully used to probe the surface chemistry of silicon prepared using standard wafer cleaning and processing techniques. The results demonstrate the utility of this measurement for…

材料科学 · 物理学 2010-02-16 P. G. Spizzirri , J. -H. Fang , S. Rubanov , E. Gauja , S. Prawer

The vibrational and electronic properties of 2-dimensinal (2D) materials can be efficiently tuned by external strain due to their good stretchability. Resonant Raman spectroscopy is a versatile tool to study the physics of phonons,…

We report a shot noise limited high speed stimulated Raman microscopy platform allowing to acquire molecular vibrational spectra over \SI{200}{\per \cm} in \SI{12}{\micro \second} at a scan rate of 40kHz. Using spectral focusing together…

光学 · 物理学 2019-05-29 Xavier Audier , Nicolas Forget , Hervé Rigneault

Brillouin and Raman scattering spectroscopy are established techniques for the nondestructive contactless and label-free readout of mechanical, chemical and structural properties of condensed matter. Brillouin-Raman investigations currently…

Stimulated Raman scattering (SRS) microscopy has emerged as a powerful technique for probing the spatiotemporal dynamics of molecular bonds with exceptional sensitivity, resolution, and speed. However, classically, its performance remains…

Stimulated Raman scattering (SRS) microscopy is a powerful label-free imaging technique that probes the vibrational response of chemicals with high specificity and sensitivity. High-power, quantum-enhanced SRS microscopes have been recently…

A theoretical model describing the Raman scattering process in atomic vapors is constructed. The treatment investigates the low-excitation regime suitable for modern experimental applications. Despite the incorporated decoherence effects…

量子物理 · 物理学 2012-07-16 Jan Kolodynski , Jan Chwedenczuk , Wojciech Wasilewski

A simple physical mechanism of stimulated light scattering on nanoscale objects in water suspension similar to Langmuir waves mechanism in plasma is proposed. The proposed mechanism is based on a dipole interaction between the light wave…

We demonstrate stimulated Raman gain using a broadband LED Stokes source to measure vibrational spectra of aqueous glucose solutions. This versatile and cost-effective method increases Raman signal for a variety of applications. We measured…

应用物理 · 物理学 2018-09-14 Peter Bullen , Ioannis Kymissis , Adler Perotte

Backward stimulated Raman scattering in gases provides a promising route to compression and amplification of a Stokes seed-pulse by counter-propagating against a pump-pulse, as has been already demonstrated in various platforms, mainly in…

光学 · 物理学 2018-05-08 Manoj K. Mridha , David Novoa , Philip St. J. Russell

Strain is prominent in fabricated samples of two-dimensional semiconductors and it also serves as an exploitable tool for engineering their properties. However, quantifying strain and characterizing its spatially inhomogeneous distribution…

材料科学 · 物理学 2014-09-01 Ruixiang Fei , Li Yang

The random lasing (RL) emission of dyed vesicular polymeric films in diffusive regime of light propagation was investigated under helium temperature. It represents itself the coupling effect of stimulated emission and stimulated Raman…

光学 · 物理学 2010-08-27 V. P. Yashchuk , E. A. Tikhonov , O. A. Prygodiuk