相关论文: Nitrogen Oxide Concentrations in Natural Waters on…
A key challenge in origin-of-life studies is understanding the environmental conditions on early Earth under which abiogenesis occurred. While some constraints do exist (e.g., zircon evidence for surface liquid water), relatively few…
One of the proposed scenarios for the origin of life is the primordial RNA world, which considers that RNA molecules were likely responsible for the storage of genetic information and the catalysis of biochemical reactions in primitive…
The emergence of life on the Earth has required a prior organic chemistry leading to the formation of prebiotic molecules. The origin and the evolution of the organic matter on the early Earth is not yet firmly understood. Several…
Rocky planets may acquire a primordial atmosphere by outgassing of volatiles from their magma ocean. The distribution of O between H$_2$O, CO and CO$_2$ in chemical equilibrium subsequently changes significantly with decreasing temperature.…
Earth is expected to have acquired a reduced proto-atmosphere enriched in H2 and CH4 through the accretion of building blocks that contain metallic Fe and/or the gravitational trapping of surrounding nebula gas. Such an early, wet, reduced…
Any search for present or past life beyond Earth should consider the initial processes and related environmental controls that might have led to its start. As on Earth, such an understanding lies well beyond how simple organic molecules…
Ultraviolet (UV) light plays a key role in surficial theories of the origin of life, and numerous studies have focused on constraining the atmospheric transmission of UV radiation on early Earth. However, the UV transmission of the natural…
The origin of life on Earth would benefit from a prebiotic atmosphere that produced nitriles, like HCN, which enable ribonucleotide synthesis. However, geochemical evidence suggests that Hadean air was relatively oxidizing with negligible…
The emergence of habitable conditions on the early Earth and on rocky exoplanets requires persistent energy sources that can drive both prebiotic chemistry and climate warming under magnetically active young G to M stars. To quantify the…
Atmospheric nitrogen may be a necessary ingredient for the habitability of a planet since its presence helps to prevent water loss from a planet. The present day nitrogen isotopic ratio, $^{15}$N/$^{14}$N, in the Earth's atmosphere is a…
The origin of the Earth's ocean has been discussed on the basis of deuterium/hydrogen ratios (D/H) of several sources of water in the solar system. The average D/H of carbonaceous chondrites (CC's) is known to be close to the current D/H of…
Earth's mantle nitrogen (N) content is comparable to that found in its N-rich atmosphere. Mantle N has been proposed to be primordial or sourced by later subduction, yet its origin has not been elucidated. Here we model N partitioning…
There are two dominant and contrasting classes of origin of life scenarios: those predicting that life emerged in submarine hydrothermal systems, where chemical disequilibrium can provide an energy source for nascent life; and those…
The isotopic compositions of terrestrial hydrogen and nitrogen are clearly different from those of the nebular gas from which the solar system formed, and also differ from most of cometary values. Terrestrial N and H isotopic compositions…
The dominant form of nitrogen provided to most solar system bodies is currently unknown, though available measurements show that the detected nitrogen in solar system rocks and ices is depleted with respect to solar abundances and the…
Bioavailable nitrogen is thought to be a requirement for the origin and sustenance of life. Before the onset of biological nitrogen fixation, abiotic pathways to fix atmospheric N2 must have been prominent to provide bioavailable nitrogen…
The search for life beyond the Solar System is a major activity in exoplanet science. However, even if an Earth-like planet were to be found, it is unlikely to be at a similar stage of evolution as the modern Earth. It is therefore of…
Ancient Venus and Earth may have been similar in crucial ways for the development of life, such as liquid water oceans, land-ocean interfaces, favorable chemical ingredients and energy pathways. If life ever developed on, or was transported…
Planet Earth has evolved from an entirely anoxic planet with possibly a different tectonic regime to the oxygenated world with horizontal plate tectonics that we know today. For most of this time, Earth has been inhabited by a purely…
How life started on Earth is an unsolved mystery. There are various hypotheses for the location ranging from outer space to the seafloor, subseafloor or potentially deeper. Here, we applied extensive ab initio molecular dynamics (AIMD)…