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Three-dimensionally (3D) frustrated magnets generally exist in the magnetic diamond and pyrochlore lattices, in which quantum fluctuations suppress magnetic orders and generate highly entangled ground states (GS). LiYbSe2 in a previously…

The emergence of a quantum spin liquid (QSL), a state of matter that can result when electron spins are highly correlated but do not become ordered, has been the subject of a considerable body of research in condensed matter physics. Spin…

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

The synergistic interplay between spin correlations, spin-orbit coupling, and competing exchange interactions provides a promising route to realize exotic quantum states with nontrivial excitations in rare-earth based frustrated magnets.…

We present a comprehensive experimental investigation of the temperature evolution of magnetic states in triangular-lattice delafossite YbCuSe$_2$. Magnetization measurements on high-quality single crystals reveal easy-plane anisotropy.…

强关联电子 · 物理学 2026-04-08 K. Bhattacharya , Y. Tokiwa , M. Majumder

Yb-based magnets, with a perfect triangular lattice of pseudospin-$1/2$ Yb$^{3+}$ ions, have emerged as candidates for realizing a quantum spin-liquid state, with NaYbS$_2$ being a prominent example. Here we present the solid-solution…

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

Spin-orbit coupling is an important ingredient to regulate the many-body physics, especially for many spin liquid candidate materials such as rare-earth magnets and Kitaev materials. The rare-earth chalcogenides NaYbCh$_2$ (Ch = O, S, Se)…

A layered triangular lattice with spin-1/2 ions is an ideal platform to explore highly entangled exotic states like quantum spin liquid (QSL). Here, we report a systematic in-field neutron scattering study on a perfect two-dimensional…

Quantum fluctuations originating phase competition or geometrical frustration of spins lead to novel states such as a quantum critical point and a quantum spin liquid where the strong quantum fluctuations suppress any ordered states even at…

强关联电子 · 物理学 2019-11-28 Y. Saito , H. Nakamura , M. Sawada , T. Yamazaki , S. Fukuoka , N. Matsunaga , K. Nomura , M. Dressel , A. Kawamoto

We investigated the spin dynamics by electron spin resonance (ESR) of the Yb-based, effective spin-1/2 delafossites NaYbO$_{2}$, AgYbO$_{2}$, LiYbS$_{2}$, NaYbS$_{2}$, and NaYbSe$_{2}$ which all show an absence of magnetic order down to…

The cradle of quantum spin liquids, triangular antiferromagnets show strong proclivity to magnetic order and require deliberate tuning to stabilize a spin-liquid state. In this brief review, we juxtapose recent theoretical developments that…

强关联电子 · 物理学 2020-03-13 Yuesheng Li , Philipp Gegenwart , Alexander A. Tsirlin

A quantum spin liquid is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. Such a state of matter is potentially relevant to high-temperature superconductivity and…

We report a comprehensive experimental investigation of the structural, thermodynamic, static, and dynamic properties of a triangular lattice antiferromagnet Rb$_3$Yb(VO$_4$)$_2$. Through the analysis of magnetic susceptibility,…

材料科学 · 物理学 2025-06-10 Sebin J. Sebastian , R. Kolay , Abhidev. B , Q. -P. Ding , Y. Furukawa , R. Nath

We probed the local electronic properties of the mixed-valent Co(+4-x) triangular-lattice in Na{x}CoO{2}-yH{2}O by 59-Co NMR. We observed two distinct types of Co sites for x>=1/2, but the valence seems averaged out for x~1/3. Local spin…

强关联电子 · 物理学 2009-11-10 F. L. Ning , T. Imai , B. W. Statt , F. C. Chou

It is predicted that strongly interacting spins on a frustrated lattice may lead to a quantum disordered ground state or even form a quantum spin liquid with exotic low-energy excitations. However, a thorough tuning of the frustration…

强关联电子 · 物理学 2024-01-08 Jierong Wang , Y. -S. Su , M. Spitaler , P. Puphal , C. Krellner , S. E. Brown , A. Pustogow

We performed high-field magnetization, magnetocaloric effect (MCE), and NMR measurements on the Ising triangular-lattice antiferromagnet Rb$_2$Co(SeO$_3$)$_2$. The observations of the 1/3-magnetization plateau, the split NMR lines, and the…

Na4Ir3O8 is a unique case of a hyperkagome 3D corner sharing triangular lattice which can be decorated with quantum spins. It has spurred a lot of theoretical interest as a spin liquid candidate. We present a comprehensive set of NMR data…

强关联电子 · 物理学 2015-07-29 A. C. Shockley , F. Bert , J-C Orain , Y. Okamoto , P. Mendels

We report a muSR study of LiCrO2, which has a magnetic lattice made up of a stacking of triangular Heisenberg antiferromagnetic (Cr3+, S = 3/2) layers. A static magnetically ordered state is observed below the transition temperature T_N =…

强关联电子 · 物理学 2009-06-09 A. Olariu , P. Mendels , F. Bert , L. K. Alexander , A. V. Mahajan , A. D. Hillier , A. Amato