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We review the current state of tabletop extreme ultraviolet (XUV) sources based on high harmonic generation (HHG) in femtosecond enhancement cavities (fsEC). Recent developments have enabled generation of high photon flux (1014 photons/sec)…

光学 · 物理学 2015-06-05 Arthur K Mills , TJ Hammond , Matthew HC Lam , David J Jones

We present a table-top extreme ultraviolet (XUV) beamline for measuring time- and frequency-resolved XUV excited optical luminescence (XEOL) with additional femtosecond-resolution XUV transient absorption spectroscopy functionality. XUV…

Many atomic and molecular systems of fundamental interest possess resonance frequencies in the extreme ultraviolet (XUV) where laser technology is limited and radiation sources have traditionally lacked long-term phase coherence. Recent…

Time- and Angle-resolved photoelectron spectroscopy from surfaces can be used to record the dynamics of electrons and holes in condensed matter on ultrafast time scales. However, ultrafast photoemission experiments using extreme-ultraviolet…

The VOXES project's goal is to realize the first prototype of a high resolution and high precision X-ray spectrometer for diffused sources, using Highly Annealed Pyrolitic Graphite (HAPG) crystals combined with precision position detectors.…

仪器与探测器 · 物理学 2019-03-08 A. Scordo , H. Shi , C. Curceanu , M. Miliucci , F. Sirghi , J. Zmeskal

Novel methods for diagnostics of molecular hydrogen plasma processes, such as ionization, production of high vibrational levels, dissociation of molecules via excitation to singlet and triplet states and production of metastable states, are…

等离子体物理 · 物理学 2015-07-10 J. Komppula , O. Tarvainen

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

We demonstrate a new technique in velocity map imaging (VMI) that allows spatial gating of the laser focal overlap region in time resolved pump-probe experiments. This significantly enhances signal-to-noise ratio by eliminating background…

We present a new velocity map imaging instrument for studying molecular beam surface scattering in a near-ambient pressure (NAP-VMI) environment. The instrument offers the possibility to study chemical reaction dynamics and kinetics where…

化学物理 · 物理学 2022-08-10 Tzu-En Chien , Lea Hohmann , Dan J. Harding

We present an approach that combines photon spectrum correlation analysis with the reconstruction of three-dimensional momentum distribution from velocity map images in an efficient, single-step procedure. We demonstrate its efficacy with…

High-harmonic generation (HHG) is used as a source for various imaging applications in the extreme ultraviolet spectral range. It offers spatially coherent radiation and unique elemental contrast with the potential for attosecond time…

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

The ongoing development of intense high-harmonic generation (HHG) sources has recently enabled highly nonlinear ionization of atoms by the absorption of at least 10 extreme-ultraviolet (XUV) photons within a single atom [Senfftleben…

Recent progress in laser-based high-repetition rate extreme ultraviolet (EUV) lightsources and multidimensional photoelectron spectroscopy enable the build-up of a new generation of time-resolved photoemission experiments. Here, we present…

X-ray free electron laser (XFEL) experiments have brought unique capabilities and opened new directions in research, such as creating new states of matter or directly measuring atomic motion. One such area is the ability to use finely…

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

强关联电子 · 物理学 2025-11-03 Takeshi Suzuki , Kozo Okazaki

The remarkable progress in the field of laser spectroscopy induced by the invention of the frequency-comb laser has enabled many new high-precision tests of fundamental theory and searches for new physics. Extending frequency-comb based…

原子物理 · 物理学 2021-01-20 L. S. Dreissen , C. Roth , E. L. Gründeman , J. J. Krauth , M. G. J. Favier , K. S. E. Eikema

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

Neuromorphic event-based cameras are bio-inspired visual sensors with asynchronous pixels and extremely high temporal resolution. Such favorable properties make them an excellent choice for solving state estimation tasks under aggressive…

机器人学 · 计算机科学 2024-06-03 Xiuyuan Lu , Yi Zhou , Junkai Niu , Sheng Zhong , Shaojie Shen

Cavity-based x-ray free-electron lasers (CBXFELs) represent a possible realization of fully coherent hard x-ray sources having high spectral brilliance along with a narrow spectral bandwidth of $\simeq 1 - 50$~meV, a high repetition pulse…

光学 · 物理学 2025-03-25 Keshab Kauchha , Peifan Liu , Paresh Pradhan , Yuri Shvyd'ko