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We present a new theoretical approach to the study of second and third harmonic generation from metallic nanostructures and nanocavities filled with a nonlinear material, in the ultrashort pulse regime. We model the metal as a two-component…

Monolayer transition metal dichalcogenides, coupled to metal plasmonic nanocavities, have recently emerged as new platforms for strong light-matter interactions. These systems are expected to have nonlinear optical properties that will…

Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…

Remarkable optical and electrical properties of two-dimensional (2D) materials, such as graphene and transition-metal dichalcogenide (TMDC) monolayers, offer vast technological potential for novel and improved optoelectronic nanodevices,…

光学 · 物理学 2016-07-22 Martin Weismann , Nicolae C. Panoiu

Optical properties of periodic arrays of nanoholes of a triangular shape with experimentally realizable parameters are examined in both linear and nonlinear regimes. Utilizing fully vectorial three-dimensional approach based on the…

介观与纳米尺度物理 · 物理学 2020-03-18 Elena Drobnyh , Maxim Sukharev

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

光学 · 物理学 2021-05-11 Muhammad Khalid , Cristian Ciracì

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of…

We show that second harmonic generation can be enhanced by Fano resonant coupling of asymmetric plasmonic metal nanostructures. We develop a theoretical model examining the effects of electromagnetic interaction between two metal…

Understanding how light interacts at the nanoscale with metals, semiconductors, or ordinary dielectrics is pivotal if one is to properly engineer nano-antennas, filters and, more generally, devices that aim to harness the effects of new…

We develop a quantitative mathematical theory that offers new perspectives on nonlinear harmonic generation in plasmonic structures arising from symmetry breaking. Focusing on second harmonic generation--the most fundamental process and the…

偏微分方程分析 · 数学 2026-05-04 Hongyu Liu , Zhi-Qiang Miao , Jingfeng Yao , Chengxun Yuan , Guang-Hui Zheng

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

光学 · 物理学 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa

Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…

Second and third harmonic signals have been usually generated by using nonlinear crystals, but that method suffers from the low efficiency in small thicknesses. Metamaterials can be used to generate harmonic signals in small thicknesses.…

光学 · 物理学 2016-07-28 Iman Sajedian , Inki Kim , Abdolnasser Zakery , Junsuk Rho

Monolayer transition metal dichalcogenides (TMDs) exhibit high nonlinear optical (NLO) susceptibilities. Experiments on MoS$_2$ have indeed revealed very large second-order ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) optical…

We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…

Plasmons in atomically thin materials offer a compelling route to trigger nonlinear light-matter interactions through extreme optical confinement in the two-dimensional (2D) limit. However, optical nonlocality in plasmons is typically…

介观与纳米尺度物理 · 物理学 2025-12-23 Line Jelver , Joel D. Cox

We explore the outcomes of detailed microscopic models by calculating second- and third-harmonic generation from thin film surfaces with discontinuous free-electron densities. These circumstances can occur in structures consisting of a…

We theoretically investigate the second harmonic generation and photon drag effect induced by an incident plane wave to a doped graphene placed on a two-dimensional diffraction grating. The relevant nonlinear conductivity of the graphene is…

光学 · 物理学 2018-10-04 Tetsuyuki Ochiai

Recent advances in nanofabrication technology now enable unprecedented control over 2D heterostructures, in which single- or few-atom thick materials with synergetic opto-electronic properties can be combined to develop next-generation…

材料科学 · 物理学 2019-06-10 A. Rodríguez Echarri , Joel D. Cox , F. Javier García de Abajo

A combined analytical and numerical study of the modes in two distinct plasmonic nanowire systems is presented. The computations are based on a Discontinuous Galerkin Time-Domain approach and a fully nonlinear and nonlocal hydrodynamic…

光学 · 物理学 2018-02-26 M. Moeferdt , T. Kiel , T. Sproll , F. Intravaia , K. Busch
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