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The photogalvanic effect (PGE) occurring in noncentrosymmetric materials enables the generation of a dc photocurrent at zero bias with a high polarization sensitivity, which makes it very attractive in photodetection. However, the magnitude…

应用物理 · 物理学 2021-06-28 Liyu Qian , Juan Zhao , Yiqun Xie

We perform photoluminescence measurements on vacancy-related emitters in hexagonal boron nitride (hBN) that are notorious for their low quantum yields. The gating of these emitters via few-layer graphene electrodes reveals a reproducible,…

Organic bulk-heterojunctions (BHJ) and solar cells containing the trimetallic nitride endohedral fullerene 1-[3-(2-ethyl)hexoxy carbonyl]propyl-1-phenyl-Lu3N@C80 (Lu3N@C80-PCBEH) show an open circuit voltage (VOC) 0.3 V higher than similar…

In this study, we investigate the bulk electronic structure of Pb-substituted LaO$_{0.5}$F$_{0.5}$BiS$_2$ single crystals, using two types of hard-x-ray spectroscopy. High-energy-resolution fluorescence-detected x-ray absorption…

Understanding the transport of photogenerated charge carriers in semiconductors is crucial for applications in photovoltaics, optoelectronics and photo-detectors. While recent experimental studies using scanning ultrafast electron…

材料科学 · 物理学 2023-02-22 Wenkai Ouyang , Xiangying Zuo , Bolin Liao

We present first-principles many-body perturbation theory calculations of the quasiparticle electronic structure and of the optical response of HfO$_2$ polymorphs. We use the $GW$ approximation including core electrons by the projector…

材料科学 · 物理学 2018-11-14 Benoît Sklénard , Alberto Dragoni , François Triozon , Valerio Olevano

We present angle-resolved photoemission experiments on 1T-TiSe2 at temperatures ranging from 13K to 288K. The data evidence a dramatic renormalization of the conduction band below 100K, whose origin can be explained with the exciton…

Significant excitonic effects were observed in graphene by measuring its optical conductivity in a broad spectral range including the two-dimensional {\pi}-band saddle-point singularities in the electronic structure. The strong…

材料科学 · 物理学 2015-05-20 Kin Fai Mak , Jie Shan , Tony F. Heinz

Extensive efforts have been undertaken on the photoelectric physics of hybrid organolead halide perovskites to unveil the reason for the attractive photovoltaic performance. Yet, the resulting evidences are far from being fully conclusive.…

In this work we employ the $GW$ approximation in the framework of the SternheimerGW method to investigate the effects of many-body corrections to the band structures and Fermi surfaces of bulk and monolayer NbS$_2$. For the bulk system, we…

材料科学 · 物理学 2018-08-13 Christoph Heil , Martin Schlipf , Feliciano Giustino

BiFeO$_{3}$ is multiferroic material with space group Pbnm exhibits coupling of both magnetic and electric orders under strain force. To analyze band gap Tauc plot extrapolation method is used $\&$ remarkably smaller than some reported…

材料科学 · 物理学 2021-03-04 Tewodros Eyob , Kenate Nemera , Lemi Demeyu

The bulk photovoltaic effect is a long-known but poorly understood phenomenon. Recently, however, the multiferroic bismuth ferrite has been observed to produce strong photovoltaic response to visible light, suggesting that the effect has…

材料科学 · 物理学 2015-08-25 Steve M. Young , Fan Zheng , Andrew M. Rappe

Ferroelectric and photovoltaic properties of BiFeO3/LaFeO3 superlattices grown by pulsed laser deposition have been investigated being the bilayer thickness). For a high concentration of BiFeO3 a ferroelectric state is observed…

材料科学 · 物理学 2020-12-11 J. Belhadi , S. Yousfi , M. El Marssi , D. C. Arnold , H. Bouyanfif

We present a microscopic theory of a photon drag effect that appears in a Bose-Einstein condensate of neutral particles, considering indirect excitons in a double quantum well nanostructure under the action of a circularly polarized…

介观与纳米尺度物理 · 物理学 2018-08-02 V. M. Kovalev , M. V. Boev , I. G. Savenko

We investigate the excitonic transitions in single- and few-layer MoSe2 phototransistors by photocurrent spectroscopy. The measured spectral profiles show a well-defined peak at the optically active (bright) A0 exciton resonance. More…

The calculated quasiparticle band structure of bulk hexagonal boron nitride using the all-electron GW approximation shows that this compound is an indirect-band-gap semiconductor. The solution of the Bethe-Salpeter equation for the…

材料科学 · 物理学 2009-11-11 B. Arnaud , S. Lebègue , P. Rabiller , M. Alouani

Following the recent discovery of a bulk photovoltaic effect in the Pb[(Mg1/3Nb2/3)0.68Ti0.32]O3 crystal, we report here more than one order of magnitude improvement of photovoltaicity as well as its poling dependence in the related…

材料科学 · 物理学 2019-06-14 A. S. Makhort , G. Schmerber , B. Kundys

Shift current is a photovoltaic current in bulk noncentrosymmetric insulator. Studies on shift current have so far focused on the extended Bloch waves, such as in semiconductors and perovskites. In contrast, it is unknown whether the…

介观与纳米尺度物理 · 物理学 2021-08-31 Hiroaki Ishizuka , Naoto Nagaosa

Multiferroic materials, characterized by the coexistence of ferroelectricity and ferromagnetism, may unveil band structures suggestive of complex phenomena and new functionalities. In this Letter, we analyze the band structure of EuO in its…

The ab initio prediction of Raman intensities for bulk solids usually relies on the hypothesis that the frequency of the incident laser light is much smaller than the band gap. However, when the photon frequency is a sizeable fraction of…

材料科学 · 物理学 2015-06-17 Yannick Gillet , Matteo Giantomassi , Xavier Gonze